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921.
Yunpeng Wang Zhaoyun Wang Changyi Zhao Hongjun Wang Jinzhong Liu Jialan Lu Dehan Liu 《Journal of Petroleum Geology》2007,30(4):339-356
In this paper we derive kinetic parameters for the generation of gaseous hydrocarbons (C1‐5) and methane (C1) from closed‐system laboratory pyrolysis of selected samples of marine kerogen and oil from the SW Tarim Basin. The activation energy distributions for the generation of both C1‐5 (Ea = 59‐72kcal, A = 1.0×1014 s?1) and C1 (Ea = 61‐78kcal, A = 6.06×1014 s?1) hydrocarbons from the marine oil are narrower than those for the generation of these hydrocarbons from marine kerogen (Ea = 50‐74kcal, A = 1.0×1014 s?1 for C1‐5; and Ea = 48‐72kcal, A=3.9×1013 s?1 for C1, respectively). Using these kinetic parameters, both the yields and timings of C1‐5 and C1 hydrocarbons generated from Cambrian source rocks and from in‐reservoir cracking of oil in Ordovician strata were predicted for selected wells along a north‐south profile in the SW of the basin. Thermodynamic conditions for the cracking of oil and kerogen were modelled within the context of the geological framework. It is suggested that marine kerogen began to crack at temperatures of around 120°C (or 0.8 %Ro) and entered the gas window at 138°C (or 1.05 %Ro); whereas the marine oil began to crack at about 140 °C (or 1.1 %Ro) and entered the gas window at 158 °C (or 1.6%Ro). The main geological controls identified for gas accumulations in the Bachu Arch (Southwest Depression, SW Tarim Basin) include the remaining gas potential following Caledonian uplift; oil trapping and preservation in basal Ordovician strata; the extent of breaching of Ordovician reservoirs; and whether reservoir burial depths are sufficiently deep for oil cracking to have occurred. In the Maigaiti Slope and Southwest Depression, the timing of gas generation was later than that in the Bachu Arch, with much higher yields and generation rates, and hence better prospects for gas exploration. It appears from the gas generation kinetics that the primary source for the gases in the Hetianhe gasfield was the Southwest Depression. 相似文献
922.
923.
Biofiltration is an efficient technology for treatment of gaseous waste. Its disadvantages, however, include large volume of bioreactor and slow adaptation to fluctuating concentrations in waste gas. Catalytic oxidation offers a high destructive efficiency at relatively low operating temperature and small unit. A bench scale system integrated with a biofilter and a catalytic oxidation unit for the treatment of gases containing o-xylene was investigated in this study. The catalytic oxidation unit was packed with Cu/Al2O3 catalyst. The results showed that 90% of o-xylene could be removed in the biofilter at the load below 38.2 g m−3 h−1. High o-xylene concentration in inlet gas resulted in an overload of the biofilter. Using the Cu/Al2O3 catalytic oxidation unit, the concentration of o-xylene could be reduced evidently. The combination of the chemical and microbial processes not only led to a high and stable efficiency of o-xylene conversion, but also improved capacity resisting the shock loads. The Cu/Al2O3 was studied for o-xylene oxidation in temperature range of 90–320 °C. The o-xylene conversion was improved correspondingly with the increasing of oxidation temperature. The reaction mechanism of o-xylene oxidation on Cu/Al2O3 was also investigated using diffuse reflectance infrared Fourier transform spectroscopy (DRIFTS). 相似文献
924.
为适应城市发展需要,必须加强城市水利工作,通过对舒兰市水资源现状分析,对解决城市供水水源工程建设的措施进行探讨。 相似文献
925.
926.
927.
Lanthanum doped nickel and YSZ composite anode (LaNi–YSZ) exhibited a greatly reduced polarization resistance and high performance for electrochemical oxidation of hydrogen and methane, which resulted from a fine anode structure with a high dispersion of nickel catalyst and a high catalytic activity towards methane. 相似文献
928.
929.
多计数管流向探头;;单孔;;总流向;;局部流向;;滤水管 掌握地下水的流动方向,有助于研究地下水的运动规律。利用放射性单孔法可以测定地下水流某一点流动方向。 应用放射性指示剂在单孔中测定地下水流向的方法由奥地利的梅尔霍费于1963年首先提出,1964年波兰的鲍劳斯齐克等把这种方法用于现场测量。放射性单孔流向测量方法有若干种,其原理基本相同,仅测量装置结构有区别,早期有单管旋转式探头。我们从1983年7月 相似文献
930.
Ying Bai Yanfeng Yin Na Liu Bingkun Guo Hongjun Shi Jianyong Liu Zhaoxiang Wang Liquan Chen 《Journal of power sources》2007
As the continuance of our series study on LiCoO2 surface modification, the complicated traditional surface coating method is replaced with simple addition of amorphous YPO4 and Al2O3 in commercial LiCoO2 or in commercial electrolyte based on our understanding to the improvement mechanism of surface modification. Comprehensive studies by X-ray photoelectron spectroscopy (XPS), gas chromatography and mass spectroscopy (GC–MS), inductively coupled plasma (ICP) and Fourier transformed infrared (FTIR) indicate that the products of spontaneous reaction between the additive and the LiPF6 based electrolyte are responsible for the performance improvements. 相似文献