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排序方式: 共有8137条查询结果,搜索用时 15 毫秒
91.
Lingping Kong Jue Gong Qingyang Hu Francesco Capitani Anna Celeste Takanori Hattori Asami Sano-Furukawa Nana Li Wenge Yang Gang Liu Ho-kwang Mao 《Advanced functional materials》2021,31(9):2009131
The soft nature of organic–inorganic halide perovskites renders their lattice particularly tunable to external stimuli such as pressure, undoubtedly offering an effective way to modify their structure for extraordinary optoelectronic properties. Here, using the methylammonium lead iodide as a representative exploratory platform, it is observed that the pressure-driven lattice disorder can be significantly suppressed via hydrogen isotope effect, which is crucial for better optical and mechanical properties previously unattainable. By a comprehensive in situ neutron/synchrotron-based analysis and optical characterizations, a remarkable photoluminescence (PL) enhancement by threefold is convinced in deuterated CD3ND3PbI3, which also shows much greater structural robustness with retainable PL after high peak-pressure compression–decompression cycle. With the first-principles calculations, an atomic level understanding of the strong correlation among the organic sublattice and lead iodide octahedral framework and structural photonics is proposed, where the less dynamic CD3ND3+ cations are vital to maintain the long-range crystalline order through steric and Coulombic interactions. These results also show that CD3ND3PbI3-based solar cell has comparable photovoltaic performance as CH3NH3PbI3-based device but exhibits considerably slower degradation behavior, thus representing a paradigm by suggesting isotope-functionalized perovskite materials for better materials-by-design and more stable photovoltaic application. 相似文献
92.
In IEEE 802.15.4/ZigBee Wireless Sensor Networks (WSNs) a specific node (called the PAN coordinator or sink) controls the whole network. When the network operates in a multi-hop fashion, the position of the PAN coordinator has a significant impact on the performance: it strongly affects network energy consumption for both topology formation and data routing. The development of efficient self-managing, self-configuring and self-regulating protocols for the election of the node that coordinates and manages the IEEE 802.15.4/ZigBee WSN is still an open research issue. In this paper we present a cross-layer approach to address the problem of PAN coordinator election on topologies formed in accordance with the IEEE 802.15.4. Our solution combines the network formation procedure defined at the MAC layer by the IEEE 802.15.4 standard with a topology reconfiguration algorithm operating at the network layer. We propose a standard-compliant procedure (named PAN coordinator ELection – PANEL) to self-configure a IEEE 802.15.4/ZigBee WSN by electing, in a distributed way, a suitable PAN coordinator. A protocol implementing this solution in IEEE 802.15.4 is also provided. Performance results show that our cross-layer approach minimizes the average number of hops between the nodes of the network and the PAN coordinator allowing to reduce the data transfer delay and determining significant energy savings compared with the performance of the IEEE 802.15.4 standard. 相似文献
93.
A Roadmap for Controlled and Efficient n‐Type Doping of Self‐Assisted GaAs Nanowires Grown by Molecular Beam Epitaxy 下载免费PDF全文
Marta Orrù Eva Repiso Stefania Carapezzi Alex Henning Stefano Roddaro Alfonso Franciosi Yossi Rosenwaks Anna Cavallini Faustino Martelli Silvia Rubini 《Advanced functional materials》2016,26(17):2836-2845
N‐type doping of GaAs nanowires has proven to be difficult because the amphoteric character of silicon impurities is enhanced by the nanowire growth mechanism and growth conditions. The controllable growth of n‐type GaAs nanowires with carrier density as high as 1020 electron cm?3 by self‐assisted molecular beam epitaxy using Te donors is demonstrated here. Carrier density and electron mobility of highly doped nanowires are extracted through a combination of transport measurement and Kelvin probe force microscopy analysis in single‐wire field‐effect devices. Low‐temperature photoluminescence is used to characterize the Te‐doped nanowires over several orders of magnitude of the impurity concentration. The combined use of those techniques allows the precise definition of the growth conditions required for effective Te incorporation. 相似文献
94.
Hierarchically Structured Magnetic Nanoconstructs with Enhanced Relaxivity and Cooperative Tumor Accumulation 下载免费PDF全文
Ayrat Gizzatov Jaehong Key Santosh Aryal Jeyarama Ananta Antonio Cervadoro Anna Lisa Palange Matteo Fasano Cinzia Stigliano Meng Zhong Daniele Di Mascolo Adem Guven Eliodoro Chiavazzo Pietro Asinari Xuewu Liu Mauro Ferrari Lon J. Wilson Paolo Decuzzi 《Advanced functional materials》2014,24(29):4584-4594
Iron oxide nanoparticles are formidable multifunctional systems capable of contrast enhancement in magnetic resonance imaging, guidance under remote fields, heat generation, and biodegradation. Yet, this potential is underutilized in that each function manifests at different nanoparticle sizes. Here, sub‐micrometer discoidal magnetic nanoconstructs are realized by confining 5 nm ultra‐small super‐paramagnetic iron oxide nanoparticles (USPIOs) within two different mesoporous structures, made out of silicon and polymers. These nanoconstructs exhibit transversal relaxivities up to ≈10 times (r 2 ≈ 835 mm ?1 s?1) higher than conventional USPIOs and, under external magnetic fields, collectively cooperate to amplify tumor accumulation. The boost in r 2 relaxivity arises from the formation of mesoscopic USPIO clusters within the porous matrix, inducing a local reduction in water molecule mobility as demonstrated via molecular dynamics simulations. The cooperative accumulation under static magnetic field derives from the large amount of iron that can be loaded per nanoconstuct (up to ≈65 fg) and the consequential generation of significant inter‐particle magnetic dipole interactions. In tumor bearing mice, the silicon‐based nanoconstructs provide MRI contrast enhancement at much smaller doses of iron (≈0.5 mg of Fe kg?1 animal) as compared to current practice. 相似文献
95.
Raul D. Rodriguez Sergey Shchadenko Gennadiy Murastov Anna Lipovka Maxim Fatkullin Ilia Petrov Tuan-Hoang Tran Alimzhan Khalelov Muhammad Saqib Nelson E. Villa Vladimir Bogoslovskiy Yan Wang Chang-Gang Hu Alexey Zinovyev Wenbo Sheng Jin-Ju Chen Ihsan Amin Evgeniya Sheremet 《Advanced functional materials》2021,31(17):2008818
Polyethylene terephthalate (PET) is the most widely used polymer in the world. For the first time, the laser-driven integration of aluminum nanoparticles (Al NPs) into PET to realize a laser-induced graphene/Al NPs/polymer composite, which demonstrates excellent toughness and high electrical conductivity with the formation of aluminum carbide into the polymer is shown. The conductive structures show an impressive mechanical resistance against >10000 bending cycles, projectile impact, hammering, abrasion, and structural and chemical stability when in contact with different solvents (ethanol, water, and aqueous electrolytes). Devices including thermal heaters, carbon electrodes for energy storage, electrochemical and bending sensors show this technology's practical application for ultra-robust polymer electronics. This laser-based technology can be extended to integrating other nanomaterials and create hybrid graphene-based structures with excellent properties in a wide range of flexible electronics’ applications. 相似文献
96.
97.
98.
In this study, we first analyse energy-efficiency measures in existing electrically heated houses in Sweden from a societal economic perspective. Measures to a house envelopes and to energy supply chains are evaluated through a system analysis approach and we include the external costs of climate change and the effect of different Swedish climatic zones. We find that in a typical house from the 1970s, conversion from electric heating is highly motivated since the mitigation cost of conversion is lower than the estimated external costs of emitted CO2. Both conversions and house envelope measures are more motivated in the northern part of the country, where there is a higher heat demand. A successful implementation of changes requires them to be attractive for consumers to adopt. We therefore secondly analyse the economic conditions for Swedish house owners to implement societal economic cost-efficient measures. We include the economic influence of an investment subsidy for heating system conversion, an income tax deduction for changing windows, customer electricity tax, real estate tax and of the cost of purchased energy from different energy suppliers. Apart from the economics, several other factors affect a house owner's decision to change heating systems. We therefore thirdly analyse house owners’ perceptions of different heating supply alternatives based on the results of two comprehensive questionnaires. These different perspectives are combined in a discussion whether the studied policy instruments encourage house owners to implement changes in accordance with the energy-efficiency goals of decision makers. We find that the investment subsidy could be useful to break the lock-in effect of resistance heaters, which house owners seemed to experience. The electricity tax makes heating systems in line with national goals more competitive and efficiency measures to the house envelope more profitable. The reduction of the electricity tax in the northern part of the country has the opposite effect. Also, the increase in real estate tax when implementing energy-efficiency measures gives a contradictory message. The price differences between energy suppliers has a larger impact on the house owners’ economic conditions than both subsidies and tax rate changes, and possibly also affect the house owner's attitudes towards various systems. 相似文献
99.
The emissivity of foam-covered water surface at L-band: theoretical modeling and experimental results from the FROG 2003 field experiment 总被引:1,自引:0,他引:1
100.
Vall-llossera M. Camps A. Corbella I. Torres F. Duffo N. Monerris A. Sabia R. Selva D. Antolin C. Lopez-Baeza E. Ferrer J.F. Saleh K. 《Geoscience and Remote Sensing, IEEE Transactions on》2005,43(5):973-982
The goal of the Soil Moisture and Ocean Salinity mission over land is to infer surface soil moisture from multiangular L-band radiometric measurements. As the canopy affects the microwave emission of land, it is necessary to characterize different vegetation layers. This paper presents the Reference Pixel L-Band Experiment (REFLEX), carried out in June-July 2003 at the Vale/spl grave/ncia Anchor Station, Spain, to study the effects of grapevines on the soil emission and on the soil moisture retrieval. A wide range of soil moisture (SM), from saturated to completely dry soil, was measured with the Universitat Polite/spl grave/cnica de Catalunya's L-band Automatic Radiometer (LAURA). Concurrently with the radiometric measurements, the gravimetric soil moisture, temperature, and roughness were measured, and the vines were fully characterized. The opacity and albedo of the vineyard have been estimated and found to be independent on the polarization. The /spl tau/--/spl omega/ model has been used to retrieve the SM and the vegetation parameters, obtaining a good accuracy for incidence angles up to 55/spl deg/. Algorithms with a three-parameter optimization (SM, albedo albedo, and opacity) exhibit a better performance than those with one-parameter optimization (SM). 相似文献