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21.
A single-electron transistor (SET) can be used as an extremely sensitive charge detector. Mechanical displacements can be converted into charge, and hence, SETs can become sensitive detectors of mechanical oscillations. For studying small-energy oscillations, an important approach to realize the mechanical resonators is to use piezoelectric materials. Besides coupling to traditional electric circuitry, the strain-generated piezoelectric charge allows for measuring ultrasmall oscillations via SET detection. Here, we explore the usage of SETs to detect the shear-mode oscillations of a 6-mm-diameter quartz disk resonator with a resonance frequency around 9 MHz. We measure the mechanical oscillations using either a conventional DC SET, or use the SET as a homodyne or heterodyne mixer, or finally, as a radio-frequency single-electron transistor (RF-SET). The RF-SET readout is shown to be the most sensitive method, allowing us to measure mechanical displacement amplitudes below \(10^{-13}\) m. We conclude that a detection based on a SET offers a potential to reach the sensitivity at the quantum limit of the mechanical vibrations.  相似文献   
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Fe-modified mordenite, ferrierite, Y, ZSM-5, ZSM-12 and beta zeolite catalysts were prepared by solid state ion-exchange and conventional liquid phase ion-exchange methods from aqueous solutions. Sn- modified H-beta-300 zeolite catalyst was prepared by the later method. The characterization of proton form, Fe and Sn modified zeolites was carried out using X-ray powder diffraction, scanning electron microscopy, Mössbauer spectroscopy with magnetic measurements, transmission electron microscopy, nitrogen adsorption, X-ray absorption spectroscopy, X-ray photoelectron spectroscopy, inductively coupled plasma spectroscopy, thermo-gravimetric analysis and FTIR spectroscopy using pyridine as a probe molecule. Isomerization of α-pinene oxide over the Fe and Sn modified zeolite catalysts was carried out in the liquid phase using a batch-wise glass reactor. Formation of campholenic aldehyde and fencholenic aldehyde were observed to be influenced by the structure, acidity of zeolite and contents of Fe and Sn, reaction temperature and the catalysts pretreatment.  相似文献   
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This study investigates the feasibility of enhanced electrokinetic Fenton process for the remediation of hexachlorobenzene (HCB) in low permeable soil. Laboratory scale experiments were carried out in two different type of experimental setup to evaluate the influence of electrode positions in the system. Kaolin was artificially contaminated with HCB and treated by electrokinetic Fenton process. beta-Cyclodextrin was used to enhance the solubility of HCB in pore fluid. Results show that the position of electrodes in the system and the way in which Fenton's reagent was added to the system has a significant influence on the treatment efficiency.  相似文献   
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Electrokinetic soil remediation--critical overview   总被引:14,自引:0,他引:14  
In recent years, there has been increasing interest in finding new and innovative solutions for the efficient removal of contaminants from soils to solve groundwater, as well as soil, pollution. The objective of this review is to examine several alternative soil-remediating technologies, with respect to heavy metal remediation, pointing out their strengths and drawbacks and placing an emphasis on electrokinetic soil remediation technology. In addition, the review presents detailed theoretical aspects, design and operational considerations of electrokinetic soil-remediation variables, which are most important in efficient process application, as well as the advantages over other technologies and obstacles to overcome. The review discusses possibilities of removing selected heavy metal contaminants from clay and sandy soils, both saturated and unsaturated. It also gives selected efficiency rates for heavy metal removal, the dependence of these rates on soil variables, and operational conditions, as well as a cost-benefit analysis. Finally, several emerging in situ electrokinetic soil remediation technologies, such as Lasagna, Elektro-Klean, electrobioremediation, etc., are reviewed, and their advantages, disadvantages and possibilities in full-scale commercial applications are examined.  相似文献   
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We describe recent experiments developed for investigating the interactions between superconducting phase quantum bits (qubits) and resonant cavities. Two-level system (TLS) defects within the junction barrier also couple to the qubits, adding more degrees of freedom, creating a rich multi-particle system for study.  相似文献   
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We discuss the theory of the radio-frequency single-electron transistor and the measurements that use multiwalled carbon nanotubes as active elements. Our devices made of plasma-enhanced chemical-vapor-deposition nanotubes yield charge sensitivities of 10-20 μe/ $\sqrt {Hz}$ . PACS numbers: 73.23.Hk, 73.63.Fg, 85.35.Gv, 85.35.Kt.  相似文献   
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A scheme for measuring small intrinsic critical currents I(c) in nanoscale devices is described. Changes in Josephson inductance L(J) are converted to frequency variations that are recorded via microwave reflection measurements at 700-800 MHz. The critical current is determined from the frequency shift of the reflection magnitude at zero phase bias assuming a sinusoidal current-phase relation. The method is used to study a multiwalled carbon nanotube transistor with Pd/Nb contacts inside a resistive on-chip environment. We observe gate-tunable critical currents up to I(c) ~ 8 nA corresponding to L(J) > 40 nH. The method presented is also applicable to devices shunted by closed superconducting loops.  相似文献   
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