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PEDOT:PSS‐Assisted Exfoliation and Functionalization of 2D Nanosheets for High‐Performance Organic Solar Cells 下载免费PDF全文
Wang Xing Yusheng Chen Xiaoxi Wu Xiaozhou Xu Pan Ye Ting Zhu Qingyu Guo Liqiu Yang Weiwei Li Hui Huang 《Advanced functional materials》2017,27(32)
Here, a facial and scalable method for efficient exfoliation of bulk transition metal dichalcogenides (TMD) and graphite in aqueous solution with poly(3,4‐ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) to prepare single‐ and few‐layer nanosheets is demonstrated. Importantly, these TMD nanosheets retain the single crystalline characteristic, which is essential for application in organic solar cells (OSCs). The hybrid PEDOT:PSS/WS2 ink prepared by a simple centrifugation is directly integrated as a hole extraction layer for high‐performance OSCs. Compared with PEDOT:PSS, the PEDOT:PSS/WS2‐based devices provide a remarkable power conversion efficiency due to the “island” morphology and benzoid–quinoid transition. This study not only demonstrates a novel method for preparing single‐ and few‐layer TMD and graphene nanosheets but also paves a way for their applications without further complicated processing. 相似文献
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Manipulable and Hybridized,Ultralow‐Threshold Lasing in a Plasmonic Laser Using Elliptical InGaN/GaN Nanorods 下载免费PDF全文
Tao Tao Ting Zhi Bin Liu Jiangping Dai Zhe Zhuang Zili Xie Peng Chen Fangfang Ren Dunjun Chen Youdou Zheng Rong Zhang 《Advanced functional materials》2017,27(37)
Manipulating stimulated‐emission light in nanophotonic devices on scales smaller than their emission wavelengths to meet the requirements for optoelectronic integrations is a challenging but important step. Surface plasmon polaritons (SPPs) are one of the most promising candidates for sub‐wavelength optical confinement. In this study, based on the principle of surface plasmon amplification by the stimulated emission of radiation (SPASER), III‐Nitride‐based plasmonic nanolaser with hybrid metal–oxide–semiconductor (MOS) structures is designed. Using geometrically elliptical nanostructures fabricated by nanoimprint lithography, elliptical nanolasers able to demonstrate single‐mode and multimode lasing with an optical pumping power density as low as 0.3 kW cm?2 at room temperature and a quality Q factor of up to 123 at a wavelength of ≈490 nm are achieved. The ultralow lasing threshold is attributed to the SPP‐coupling‐induced strong electric‐field‐confinement in the elliptical MOS structures. In accordance with the theoretical and experimental results, the size and shape of the nanorod are the keys for manipulating hybridization of the plasmonic and photonic lasing modes in the SPASER. This finding provides innovative insight that will contribute to realizing a new generation of optoelectronic and information devices. 相似文献
86.
一种多用户多中继MIMO通信系统迭代预编码方案 总被引:1,自引:0,他引:1
该文针对多中继MIMO通信系统多用户传输时的用户间干扰问题,提出了一种可以有效抑制多用户干扰的发射端与中继端迭代预编码的方案。该方案首先在中继端进行多中继联合的迫零预编码,然后将基站与多用户之间等效为一个点到多点的MIMO信道,采用最大化信漏噪比的预编码方法,在发射端进一步消除用户间的干扰,同时避免了噪声放大的影响,进而通过中继端预编码与发射端预编码的多次迭代,更好地保持了多中继并行传输引入空间分集所带来的性能优势,有效地抑制了用户间干扰,获得了更高的系统和容量。 相似文献
87.
改进的迭代式TOD混沌跳频序列产生算法 总被引:2,自引:0,他引:2
针对周期抽取法构造的混沌跳频序列在均衡性方面缺陷,提出了利用周期抽取与多比特抽取结合法产生迭代式TOD混沌跳频序列,理论分析及仿真结果表明,该方法构造的贝努利随机序列,具有很好的均衡性、动态特性、汉明相关性等性能,相对于多值量化与比特抽取相结合法减少了运算量,便于增加跳频序列的复杂度。 相似文献
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Li Liu Cheuk‐Lam Ho Wai‐Yeung Wong Kai‐Yin Cheung Man‐Kin Fung Wai‐Ting Lam Aleksandra B. Djurii Wai‐Kin Chan 《Advanced functional materials》2008,18(18):2824-2833
A series of solution‐processable and strongly visible‐light absorbing polyplatinynes containing oligothienyl–fluorene ring hybrids were synthesized and characterized. These rigid‐rod organometallic materials are soluble in polar organic solvents and show intense absorptions in the visible spectral region, rendering them excellent candidates for bulk heterojunction polymer solar cells. The photovoltaic behavior depends significantly on the number of thienyl rings along the polymer chain, and some of these polymer solar cells show high power conversion efficiencies (PCEs) of up to 2.9% and a peak external quantum efficiency to 83% under AM1.5 simulated solar illumination. The effect of oligothienyl chain length on improving the polymer solar cell efficiency and on their optical and charge transport properties is elucidated in detail. At the same blend ratio of 1:5, the light‐harvesting capability and PCE increase markedly with increasing number of thienyl rings. The power dependencies of the solar cell parameters (including the short‐circuit current density, open‐circuit voltage, fill‐factor, and PCE) were also examined. The present work opens up an attractive avenue to developing conjugated metallopolymers with broad and strong solar energy absorptions and tunable solar cell efficiency and supports the potential of metalated conjugated polymers for efficient power generation. 相似文献
90.
以一种进化聚类算法(ECM)为基础,提出了一种新的T-S型动态模糊推理模型的建模算法.以往许多神经模糊模型都不适用于自适应在线学习,而文章模型能够实时地调整模糊规则库及规则参数,具有较强的在线学习能力.仿真结果表明,该方法是有效的. 相似文献