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151.
Styskalik Ales Kordoghli Imene Poleunis Claude Delcorte Arnaud Dochain Denis D. Moravec Zdenek Vida Julius Homola Tomas Aprile Carmela Fusaro Luca Devred François Debecker Damien P. 《Journal of Materials Science》2021,56(25):14001-14018
Journal of Materials Science - Hybrid materials are intensely studied for potential applications in heterogeneous catalysis. Organic groups at the catalyst surface can modify not only its... 相似文献
152.
Vikrant Tiwari Michael A. Sutton S.R. McNeill Shaowen Xu Xiaomin Deng William L. Fourney Damien Bretall 《International Journal of Impact Engineering》2009
A high-speed stereo-vision system is employed to quantify dynamic material response during buried blast loading. Deformation measurements obtained using 3D image correlation of synchronized, patterned stereo-vision images obtained with an inter-frame time in the range 16 μs ≤ t ≤ 40 μs indicate that (a) buried blast loading initially induces highly localized material response directly under the buried blast location, with severity of the blast event a strong function of depth of explosive burial, (b) for relatively shallow (deep) depth of explosive burial, plate surface velocities and accelerations exceed 220 m s−1 (100 m s−1) and 6 × 106 m s−2 (1.5 × 106 m s−1) during the first 30 μs (80 μs) after detonation, respectively. 相似文献
153.
Holmstrand H Gadomski D Mandalakis M Tysklind M Irvine R Andersson P Gustafsson O 《Environmental science & technology》2006,40(12):3730-3735
Polychlorinated dibenzo-p-dioxins (PCDDs) of high concentrations in a ball clay deposit from the Mississippi Embayment were found to be consistent with a natural abiotic and non-pyrogenic origin by investigation with bulk radiocarbon analysis, compound-specific chlorine isotope analysis (CSIA-delta37Cl) of octachlorodibenzo-p-dioxin (OCDD), and black carbon (BC) analysis. The conventional radiocarbon date of total organic carbon from a depth of approximately 10 m in three parallel cores ranged from 14 700 years to >48 000 years, indicating that the strata with elevated levels of PCDDs have remained isolated from recent anthropogenic input in these >40 Ma old clay sediments. The CSIA-delta37Cl of OCDD yielded a delta37Cl of -0.2 per thousandth, which is significantly higher than the postulated range for biotic chlorination by chloroperoxidase enzymes, -11 to -10 per thousandth, and falls within the known range for abiotic organochlorines, -6 to +3 per thousandth. The absence of correlations between concentrations of PCDDs and corresponding pyrogenic black carbon (BC), together with estimations of BC sorptive loadings and the absence of polychlorinated dibenzofurans (PCDFs), suggest that vegetation fires did not form these ball-clay PCDDs. Results from this study indicate that the high levels of the toxic and carcinogenic PCDDs found in kaolinite-bearing clays may result from natural abiotic formation via in situ surface-promoted reactions on the clay mineral, including a so-far unknown organic precursor, rather than being the result of anthropogenic contamination. 相似文献
154.
Decreasing activated sludge thermal hydrolysis temperature reduces product colour, without decreasing degradability 总被引:6,自引:1,他引:6
Activated sludges are becoming more difficult to degrade in anaerobic digesters, due to the implementation of stricter nitrogen limits, longer sludge ages, and removal of primary sedimentation units. Thermal hydrolysis is a popular method to enhance degradability of long-age activated sludge, and involves pressure and heat treatment of the process fluid (150-160 degrees C saturated steam). However, as documented in this study, in a full-scale system, the use of thermal hydrolysis produces coloured, recalcitrant compounds that can have downstream impacts (e.g., failure of UV disinfection, and increased effluent nitrogen). The coloured compound formed during thermal hydrolysis was found to be melanoidins. These are coloured recalcitrant compounds produced by polymerisation of low molecular weight intermediates, such as carbohydrates and amino compounds at elevated temperature (Maillard reaction). By decreasing the THP operating temperature from 165 degrees C to 140 degrees C, THP effluent colour decreased from 12,677 mg-PtCo L(-1) to 3837 mg-PtCo L(-1). The change in THP operating temperature from 165 degrees C to 140 degrees C was shown to have no significant impact on anaerobic biodegradability of the sludge. The rate and extent of COD biodegradation remained largely unaffected by the temperature change with an average first order hydrolysis rate of 0.19 d(-1) and conversion extent of 0.43 g-COD(CH4)g-COD(-1). 相似文献
155.
Wohwe Sambo Damien Yenke Blaise Omer Förster Anna Ndong Jospeh Dayang Paul Sarr Idrissa 《Wireless Networks》2022,28(7):3275-3292
Wireless Networks - Nowadays, the exploitation of Wireless Underground Sensor Networks (WUSNs) remains challenging because of the attenuation of wireless underground communications. This issue... 相似文献
156.
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158.
This paper reviews the recent discoveries that were achieved by our group in the field of particle synthesis via ring-opening metathesis polymerization (ROMP). Both polynorbornene and polybutadiene-based particles were prepared by the respective ROMP of norbornene and cyclooctadiene initiated by (PCy3)2Cl2RuCHPh using several methods of polymerization in dispersed media, such as dispersion, suspension and miniemulsion. Depending upon the process implemented, particles size was found to range from 300 nm to 20 μm. 相似文献
159.
This paper presents an industrial problem which arises in a company specialized in drug evaluation and pharmacology research. The aim is to build employee timetables covering the demand given by a set of fixed tasks. The optimality criterion concerns the equity of the workload sharing. A solution to this problem is the assignment of all tasks whose resulting working shifts respect tasks requirements as well as legal and organizational constraints. Scheduling problems usually consider a fixed set of shifts which have to be assigned to a given number of employees whereas in our problem shifts are not fixed and are deduced from the task assignment. In the following, we refer to this problem as the shift-design personnel task scheduling problem with an equity criterion (SDPTSP-E), in reference to the shift minimization personnel task scheduling problem (SMPTSP). Even if the SDPTSP-E is related to several problems, none of them allow to grasp its full complexity. Consequently, we propose a dedicated method based on constraint programming. Several branching and exploration strategies are proposed and tested. 相似文献
160.
Laurent Denis Damien Thiry Damien Cossement Pascal Gerbaux Fabiola Brusciotti Isabel Van De Keere Veerle Goossens Herman Terryn Michel Hecq Rony Snyders 《Progress in Organic Coatings》2011,70(2-3):134-141
Plasma polymer films (PPFs) of allylamine are prepared varying the mean power injected in the plasma (Pmean). The PPF behaviour in ethanol is studied through the analysis of the PPF physico-chemistry and the composition of the resulting ethanol solutions. By Visible light Spectroscopic Ellipsometry (VISSE), it is observed that the well-known decrease of the PPF thickness (Δd) upon immersion decreases as a function of Pmean. This behaviour is attributed to an increase of the PPF cross-linking density (χ). By means of time-of-flight secondary ion mass spectrometry (ToF-SIMS) and further statistical processing of the data by principal component analysis (PCA), we propose a method to discriminate the samples according to χ. A significant increase in the PPF oxygen content is also observed after immersion which is ascribed to reaction between ethanol molecules and trapped radicals of the PPF network. On the other hand, taking into account the specificities of the gas chromatography–mass spectrometry (GC–MS) method, the resulting ethanol solutions are demonstrated to be free of chemical species containing a number of carbon atoms ranging from 7 to 40. However, Δd (accounting for PPF restructuring) might come with the dissolution of PPF materials having less than 7 carbon atoms. 相似文献