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91.
Xi Wang Xinqiang Cao Laure Bourgeois Hasigaowa Guan Shimou Chen Yeteng Zhong Dai‐Ming Tang Huiqiao Li Tianyou Zhai Liang Li Yoshio Bando Dmitri Golberg 《Advanced functional materials》2012,22(13):2682-2690
A new facile route to fabricate N‐doped graphene‐SnO2 sandwich papers is developed. The 7,7,8,8‐tetracyanoquinodimethane anion (TCNQ?) plays a key role for the formation of such structures as it acts as both the nitrogen source and complexing agent. If used in lithium‐ion batteries (LIBs), the material exhibits a large capacity, high rate capability, and excellent cycling stability. The superior electrochemical performance of this novel material is the result from its unique features: excellent electronic conductivity related to the sandwich structure, short transportation length for both lithium ions and electrons, and elastomeric space to accommodate volume changes upon Li insertion/extraction. 相似文献
92.
The synthesis of polymer-stabilized nanoparticles (PSNPs) can be successfully carried out using intermatrix synthesis (IMS) technique, which consists in sequential loading of the functional groups of a polymer with the desired metal ions followed by nanoparticles (NPs) formation stage. After each metal-loading-NPs-formation cycle, the functional groups of the polymer appear to be regenerated. This allows for repeating the cycles to increase the NPs content or to obtain NPs with different structures and compositions (e.g. core-shell or core-sandwich). This article reports the results on the further development of the IMS technique. The formation of NPs has been shown to proceed by not only the metal reduction reaction (e.g. Cu0-NPs) but also by the precipitation reaction resulting in the IMS of PSNPs of metal salts (e.g. CuS-NPs). 相似文献
93.
In Wireless Mesh Networks (WMNs), mobile clients may experience frequent handoffs due to the relatively small transmission range of the mesh routers. Each handoff may lead to packet delays and/or packet losses, which limits the performance of real-time applications over WMNs. In this work, we propose BASH—a Backhaul-Aided Seamless Handoff scheme. BASH takes advantage of the wireless backhaul feature of WMNs, and allows a mobile station to directly access the backhaul channel to probe the neighboring mesh routers. Our work shows that by utilizing the wireless backhaul, BASH (1) reduces the probing latency and, thus, the Layer-2 handoff latency; (2) allows partial overlap of the Layer-2 and Layer-3 handoffs, reducing the overall handoff latency; and (3) shortens the authentication latency by utilizing the transitivity of trust relationship. The experimental results show that BASH achieves an average Layer-2 handoff of 8.9 ms, which supports real-time applications during the handoff. 相似文献
94.
Guoqiang Xie Dmitri V. Louzguine-Luzgin Qingsheng Zhang Wei Zhang Akihisa Inoue 《Journal of Alloys and Compounds》2009,483(1-2):24
The crystallization kinetics and structure changes in a melt-spun Cu50Zr45Ti5 glassy alloy on heating were investigated by X-ray diffractometry, transmission electron microscopy, differential scanning calorimetry and differential isothermal calorimetry. The glassy phase in the Cu50Zr45Ti5 alloy was crystallized forming Cu10Zr7 and CuZr2 phases upon thermal annealing. The activation energy for crystallization obtained by the Arrhenius equation was 435 kJ/mol. The crystallization process took place by nucleation and growth mechanism, and an Avrami exponent of about 3.3 may indicate a three-dimensional interface-controlled growth of nuclei with a decreasing nucleation rate. 相似文献
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97.
Amanda Alonso Xavier Muñoz‐Berbel Núria Vigués Rosalía Rodríguez‐Rodríguez Jorge Macanás Maria Muñoz Jordi Mas Dmitri N. Muraviev 《Advanced functional materials》2013,23(19):2450-2458
Cation exchange polymeric matrices are widely used in water treatment protocols to reduce the mineral content of hard waters, even for human consumption. However, they are not antibacterial and flowing bacteria can be trapped in their structures and proliferate, thus acting as microbial contamination sources. Here, Ag@Co‐nanoparticles (Ag@Co‐NPs) with a low‐cost superparamagnetic Co0‐core and an antibacterial Ag‐shell are synthesized on granulated cation exchange polymeric matrices under soft reaction conditions. The presence of these NPs provides the final nanocomposite (NC) with additional functionalities (superparamagnetism and antibacterial activity) making it ideal for water purification applications. Ag@Co‐NPs are synthesized in situ on four cation exchange polymeric matrices containing either strong (sulfonic) or weak (carboxylic) acid functional groups homogeneously distributed (C‐type) or concentrated on an external shell (SST‐type) by the intermatrix synthesis (IMS) method. The NCs are characterized (metal content, NP size and distribution, metal oxidative state, and metal release) and evaluated for water purification applications. 相似文献
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We present an approach to similarity‐based retrieval from knowledge bases that takes into account both the structure and semantics of knowledge base fragments. Those fragments, or analogues, are represented as sparse binary vectors that allow a computationally efficient estimation of structural and semantic similarity by the vector dot product. We present the representation scheme and experimental results for the knowledge base that was previously used for testing of leading analogical retrieval models MAC/FAC and ARCS. The experiments show that the proposed single‐stage approach provides results compatible with or better than the results of two‐stage models MAC/FAC and ARCS in terms of recall and precision. We argue that the proposed representation scheme is useful for large‐scale knowledge bases and free‐structured database applications. 相似文献
100.