We demonstrate a facile and effective approach to significantly improve the photoluminescence of bulk MoS2 via laser thinning followed by gold particle decoration. Upon laser thinning of exfoliated bulk MoS2, photoluminescence emerges from the laser-thinned region. After further treatment with an AuCl3 solution, gold particles self-assemble on the laser-thinned region and thick edges, further increasing the fluorescence of bulk MoS2 28 times and the Raman response 3 times. Such fluorescence enhancement can be attributed to both surface plasmon resonance and p-type doping induced by gold particles. The combination of laser thinning and AuCl3 treatment enables the functionalization of bulk MoS2 for optoelectronic applications. It can also provide a viable strategy for mask-free and area-selective p-type doping on single MoS2 flakes.
In this study, natural materials (sodium alginate, dextran, gelatin and carboxymethyl chitosan) were modified to get aldehyde components and amino components. Upon mixing the two-component solutions together, four kinds of Schiff base hydrogels formed successfully within 5-300 s and could seal the wound tissue. The cytotoxicity tests of hydrogel extraction solution confirmed that the hydrogels are nontoxic materials. The adhesive ability was evaluated in vivo by measuring the adhesive strength after sealing the skin incisions on the back of rats. All the hydrogels showed higher adhesive strength than that of commercial fibrin glue and the blank control. The histological staining observation by hematoxylin and eosin staining (HE) and Masson’s trichrome staining (MTC) methods suggested that the hydrogels had good biocompatibility and biodegradation in vivo. They have only normal initial inflammation to skin tissue and could improve the formation of new collagen in the incision section. So, the prepared hydrogels were both safe and effective tissue adhesive, which had the great potentials to be used as skin tissue adhesive. 相似文献
Nano Research - Porous Fe3O4/carbon microspheres (PFCMs) were successfully fabricated via a facile electrospray method and subsequent heat treatment, using ferrous acetylacetonate, carbon nanotubes... 相似文献
Intrusion detection involves identifying unauthorized network activity and recognizing whether the data constitute an abnormal network transmission. Recent research has focused on using semi-supervised learning mechanisms to identify abnormal network traffic to deal with labeled and unlabeled data in the industry. However, real-time training and classifying network traffic pose challenges, as they can lead to the degradation of the overall dataset and difficulties preventing attacks. Additionally, existing semi-supervised learning research might need to analyze the experimental results comprehensively. This paper proposes XA-GANomaly, a novel technique for explainable adaptive semi-supervised learning using GANomaly, an image anomalous detection model that dynamically trains small subsets to these issues. First, this research introduces a deep neural network (DNN)-based GANomaly for semi-supervised learning. Second, this paper presents the proposed adaptive algorithm for the DNN-based GANomaly, which is validated with four subsets of the adaptive dataset. Finally, this study demonstrates a monitoring system that incorporates three explainable techniques—Shapley additive explanations, reconstruction error visualization, and t-distributed stochastic neighbor embedding—to respond effectively to attacks on traffic data at each feature engineering stage, semi-supervised learning, and adaptive learning. Compared to other single-class classification techniques, the proposed DNN-based GANomaly achieves higher scores for Network Security Laboratory-Knowledge Discovery in Databases and UNSW-NB15 datasets at 13% and 8% of F1 scores and 4.17% and 11.51% for accuracy, respectively. Furthermore, experiments of the proposed adaptive learning reveal mostly improved results over the initial values. An analysis and monitoring system based on the combination of the three explainable methodologies is also described. Thus, the proposed method has the potential advantages to be applied in practical industry, and future research will explore handling unbalanced real-time datasets in various scenarios. 相似文献