全文获取类型
收费全文 | 1225篇 |
免费 | 43篇 |
国内免费 | 9篇 |
专业分类
电工技术 | 103篇 |
综合类 | 2篇 |
化学工业 | 303篇 |
金属工艺 | 47篇 |
机械仪表 | 32篇 |
建筑科学 | 27篇 |
矿业工程 | 1篇 |
能源动力 | 96篇 |
轻工业 | 69篇 |
水利工程 | 6篇 |
石油天然气 | 6篇 |
无线电 | 104篇 |
一般工业技术 | 290篇 |
冶金工业 | 24篇 |
原子能技术 | 64篇 |
自动化技术 | 103篇 |
出版年
2023年 | 3篇 |
2022年 | 13篇 |
2021年 | 10篇 |
2020年 | 5篇 |
2019年 | 16篇 |
2018年 | 18篇 |
2017年 | 16篇 |
2016年 | 30篇 |
2015年 | 17篇 |
2014年 | 28篇 |
2013年 | 63篇 |
2012年 | 57篇 |
2011年 | 62篇 |
2010年 | 60篇 |
2009年 | 59篇 |
2008年 | 57篇 |
2007年 | 56篇 |
2006年 | 47篇 |
2005年 | 40篇 |
2004年 | 48篇 |
2003年 | 38篇 |
2002年 | 46篇 |
2001年 | 32篇 |
2000年 | 44篇 |
1999年 | 32篇 |
1998年 | 29篇 |
1997年 | 19篇 |
1996年 | 25篇 |
1995年 | 23篇 |
1994年 | 16篇 |
1993年 | 17篇 |
1992年 | 12篇 |
1991年 | 11篇 |
1990年 | 14篇 |
1989年 | 12篇 |
1988年 | 15篇 |
1987年 | 12篇 |
1986年 | 10篇 |
1985年 | 15篇 |
1984年 | 21篇 |
1983年 | 18篇 |
1982年 | 19篇 |
1981年 | 17篇 |
1980年 | 14篇 |
1979年 | 13篇 |
1978年 | 14篇 |
1977年 | 11篇 |
1975年 | 9篇 |
1974年 | 3篇 |
1973年 | 4篇 |
排序方式: 共有1277条查询结果,搜索用时 15 毫秒
51.
Effects of Atmospheric Composition on the Molecular Structure of Synthesized Silicon Oxycarbides
下载免费PDF全文
![点击此处可从《Journal of the American Ceramic Society》网站下载免费的PDF全文](/ch/ext_images/free.gif)
Masaki Narisawa Fuji Funabiki Akihiro Iwase Fumihiro Wakai Hideo Hosono 《Journal of the American Ceramic Society》2015,98(10):3373-3380
The dependence of silicon oxycarbides' chemical composition and molecular structure on their reaction conditions was tested by varying the atmosphere under which pyrolysis was performed. To obtain the silicon oxycarbides, densely cross‐linked silicone resin particles with an averaged diameter of 2 μm were pyrolyzed in various atmospheres of H2, Ar, and CO2, in the temperature range 700°C–1100°C. The residual mass of resin after pyrolysis was almost constant at 700°C, although their apparent colors varied distinctly. The sample obtained from the H2 atmosphere was white, whereas that obtained from the CO2 atmosphere was dark brown. Fourier‐transform infrared (FT‐IR) spectra of the residues suggested that the Si–O–Si network evolution was accelerated in the CO2 atmosphere. Beyond 800°C, the chemical compositions of the compounds obtained from a H2 atmosphere increasingly approached near‐stoichiometric SiO2–xSiC composition with increasing the pyrolysis temperature. Compounds from a CO2 atmosphere approached a composition of SiO2–xC with no free SiC as the pyrolysis temperature increased. In the products from an Ar atmosphere, SiO2–xSiC–yC compositions were typically obtained. The observed effects of the pyrolysis atmosphere on the resulting chemical compositions were analyzed in terms of thermodynamic calculations. Electron spin resonance (ESR) spectra revealed broad and intense signals from products obtained from either Ar or CO2. Estimating from the signal intensity, the residual spin concentrations were in the range 1018–1019 g?1. Meanwhile, the spectra from the samples obtained in H2 showed weak and sharp signals with estimated spin concentrations ranging from 1016–1017 g?1. This signal attenuation may have been due to the hydrogen capping of dangling bond formed during pyrolysis. 相似文献
52.
Ultrastructure of the digestive tract in neotropical carnivorous catfish Hemisorubim platyrhynchos (Valenciennes, 1840) (Siluriformes,Pimelodidae)
下载免费PDF全文
![点击此处可从《Scanning》网站下载免费的PDF全文](/ch/ext_images/free.gif)
53.
Efficient gas recovery and separation in a hydrate-based system was investigated for a model gaseous mixture of R22 and nitrogen. The formed hydrate settled in the recovery vessel; excess water was recycled and the hydrate was subsequently decomposed by releasing pressure from the vessel. The gas uptake rate of R22 gas from the vapor phase and the gas recovery rate from the hydrate were determined from hydrate formation and decomposition, respectively. The gas recovery rate of R22 gas gradually increased with time. On the contrary, the nitrogen gas recovery rate was a maximum in the initial stage of hydrate decomposition. A high separation factor (S.F.) was achieved by first separating the N2-rich gas generated during initial hydrate decomposition. An efficient hydrate-based gas separation and recovery process is proposed. 相似文献
54.
55.
Hideo Yamashita Tatsuya Johkoh Shinichi Takita Eihachiro Nakamae 《Computer Animation and Virtual Worlds》1991,2(1):34-40
In order to observe the physical values (magnetic flux density and eddy current) in 3D magnetic field analysis, an interactive and highly manipulative visualization system depicting stereo images is intalled in a graphics workstation with high functional graphic processors. The system has the following characteristics:
- 1 An interactive and highly manipulative menu window with many functions: it enables visualization of complex phenomena in a 3D field through observation of various combinations of physical values from various viewpoints.
- 2 Simultaneous display of both magnetic flux density and eddy current by using the appropriate use of two colour display methods for stream lines and distribution maps of density: this function facilitates observation of the mutual relations between two physical values in a 3D field.
- 3 Animations and stereo displays: since they give extremely distinct images, observers can easily understand even highly complex 3D phenomena.
56.
Koji Mori Masuo Kaji Kotohiko Sekoguchi Manabu Sakane Masao Nakazatomi Hideo Shimizu 《亚洲传热研究》1996,25(8):499-510
Time-series information on both the cross-sectional mean liquid holdup along a tube axis and the gas-liquid phase distribution along a tube diameter was obtained by means of supermultiple cross-sectional mean liquid holdup probes (S-CHOP) and semi-supermultiple point-electrode probes (SS-PEP) for vertical downward gas-liquid two-phase flow. Typical time-spatial behavior charts of interface and gas-liquid interfacial profiles are presented. Close inspection of these results reveals that a huge wave and a disturbance wave appear in downward two-phase flow as well as upward flow. It was clarified that the huge wave flow region covers a wide range of superficial gas velocities. Wave velocity, wave width and maximum liquid holdup of individual waves were examined by wave-vein analysis. Histograms of these flow parameters were also studied. It was found that there exist distinct differences in wave width between the huge wave and the disturbance wave. © 1997 Scripta Technica, Inc. Heat Trans Jpn Res, 25(8): 499–510, 1996 相似文献
57.
Kotohiko Sekoguchi Koji Mori Masuo Kaji Megumi Miwa Masao Nakazatomi Hideo Shimizu 《亚洲传热研究》1996,25(8):568-579
Gas-liquid interfacial profiles in plug flow for both upward and downward flows were obtained using semi-supermultiple point-electrode probes, comprising 67 sensing tips arranged on a tube diameter. Typical interfacial profiles are demonstrated for both flows. Close inspection of the profiles reveals that four zones exist in a pair of gas and liquid slugs for upward plug flow and a high slip velocity region in downward plug flow. The lengths of the swelling liquid front zone and the wake zone were determined. The length of the wake zone strongly depends on the relative velocity between the liquid film around the gas slug and the liquid phase in the liquid slug. Characteristic distributions of bubbles within liquid slugs were found, i.e., three types of radial distributions of void fraction, namely saddle-shaped, trapezoidal and bullet-shaped distributions, exist for upward flow. The two types for downward flow exclude the saddle-shaped distribution. © 1997 Scripta Technica, Inc. Heat Trans Jpn Res, 25 (8): 568–579, 1996 相似文献
58.
Porous glass-ceramics with a skeleton of the fast-lithium-conducting crystal Li1+ x Ti2− x Al x (PO4 )3 (where x = 0.3–0.5) were prepared by crystallization of glasses in the Li2 O─CaO─TiO2 ─Al2 O3 –P2 O5 system and subsequent acid leaching of the resulting dense glass-ceramics composed of the interlocking of Li1+ x Ti2− x Al x (PO4 )3 and β-Ca3 (PO4 )2 phases. The median pore diameter and surface area of the resulting porous Li1+ x Ti2− x Al x (PO4 )3 glass-ceramics were approximately 0.2 μm and 50 m2 /g, respectively. The electrical conductivity of the porous glass-ceramics after heating in LiNO3 aqueous solution was 8 × 10−5 S/cm at 300 K or 2 × 10−2 S/cm at 600 K. 相似文献
59.
Sang Jun Yoon Jae Goo Lee Hideo Tajima Akihiro Yamasaki Fumio Kiyono Tetsuya Nakazato Hiroaki Tao 《Journal of Industrial and Engineering Chemistry》2010,16(3):350-354
Extractions of five kinds of lanthanide metal ions by bis(2-ethylhexyl)phosphoric acid (DEHPA) with [1-Cn-3-methylimidazolium][PF6](Cn = C2, C4) or [1-butyl-4-methylpyridinium][PF6] were carried out under various DEHPA and HNO3 concentrations from 0 to 1 M and under different temperature conditions from 298 to 333 K. These results were compared with those using the conventional organic solvent, hexane, in terms of their distribution coefficient values. Under all of the conditions in this study, the ionic liquid system shows more than three times greater extractability for lanthanide compared to when hexane was used. The distribution coefficient of lanthanide ions decreased as the length of the alkyl chain increased from the ethyl to the butyl. In addition, the imidazolium cation generally shows a higher distribution coefficient compared to the pyridinium cation in an ionic liquid. The concentration ratio of lanthanides and DEHPA resulted in an extraction affinity transition for lanthanides. Also evaluated in this study were issues related to the selectivity associated with the lanthanide mixture and the dependency of the ionic radius during lanthanide extraction. 相似文献
60.
Hideo Tajima Yuta Yoshida Satoko Abiko Kazuaki Yamagiwa 《Chemical engineering journal (Lausanne, Switzerland : 1996)》2010,156(2):479-486
Temperature-sensitive hydrogel beads were prepared by Kenics static mixer technology. The temperature-sensitive monomer N,N-diethylacrylamide and photo-crosslinkable pre-polymer ENT were used as model hydrogel materials. Drop dispersion of high viscosity polymer material in low viscosity hexadecane was made using the static mixer. Drops of a solution of the mixed materials were rapidly photo-crosslinked by UV irradiation after mixing in the static mixer, and spherical hydrogel beads with narrow, normal size distribution were thus prepared. The Kenics static mixer is a useful device for the preparation of spherical beads of temperature-sensitive hydrogels. The Sauter Mean Diameter of the hydrogel beads swollen in deionized water at 293 K was measured. The experimentally determined dimensionless swollen hydrogel bead diameter was well correlated with the Weber number, degree of swelling and viscosity ratio. The effects of gelation and ENT addition on the bead size were evaluated from the degree of swelling. The correlation equation can be used for size adjustment of temperature-sensitive spherical hydrogel beads. 相似文献