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91.
Hirofumi Matsuda Makoto Kuwabara Kohichi Hamamoto 《Journal of the American Ceramic Society》1998,81(1):229-232
Thin, semiconducting BaTiO3 ceramic wires prepared in the present study exhibited reversible stress-induced, nonlinear current—;voltage characteristics across several grain boundaries. A remarkable change in resistance with the application (by the three-point bending method) of only ∼1% tensile deformation indicated that the BaTiO3 wires may have potential as stress-sensing devices. Resistance in the BaTiO3 wires bot increased and decreased with increasing tensile stress parallel to the electric fields, far below the ferroelectric transition temperature, T c ; in Sr-substituted wires near T c , on the other hand, resistance only increased. Detailed studies of the patterns and fluctuation of polarization at grain boundaries could be meaningful, because stress-sensing characteristics may be induced by changes in the relative angle between polarization vectors of adjacent grains. 相似文献
92.
Hirofumi Kakemoto Tohru Higuchi Hajime Shibata Satoshi Wada Takaaki Tsurumi 《Journal of Materials Science: Materials in Electronics》2008,19(4):311-314
The modification of thermoelectric figure of merit was estimated from enhanced mobility of [100] oriented beta-FeSi2 film. beta-FeSi2 on Si(001) substrate was prepared by molecular beam epitaxy method using an Fe source. The crystallographic orientation of
beta-FeSi2 film on Si(001) substrate was characterized by using X-ray diffraction. Using scanning electron microscopy, surface morphology
and film thickness of samples were observed and estimated, respectively. The mobility of beta-FeS2 film on Si(001) substrate were also characterized by Hall measurement at room temperature. A part of the enhancement of figure
of merit was evaluated as the functions of mobility and crystallographic orientation of samples. 相似文献
93.
Aichi Inouye Shunya Yamamoto Masahito Yoshikawa 《Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms》2008,266(2):301-307
Changes in the composition and crystalline structure of gasochromic tungsten oxide films resulting from the incorporation of hydrogen were investigated; the oxide films were prepared by reactive RF magnetron sputtering on SiO2 and glassy carbon substrates simultaneously. X-ray diffraction analysis of the deposited films at 600 °C showed a uniaxial oriented structure in the (0 1 0) plane of monoclinic WO3 for both substrates. The elastic recoil detection analysis (ERDA) and Rutherford backscattering spectroscopy (RBS) for the films on glassy carbon revealed that the hydrogen impurity was uniformly distributed up to a concentration of 0.24 H/W. The Pd-coated films on SiO2 turned blue when they were exposed to a mixture of Ar and 5% H2 gases. When the sample became colored, the hydrogen concentration in the film increased to 0.47 H/W and the crystalline structure of the film changed from monoclinic to tetragonal. These results indicated that the gasochromic coloration of the tungsten oxide films coincided with incorporation of hydrogen atoms into the crystalline lattice, corresponding to the formation of hydrogen tungsten bronze (HxWO3). 相似文献
94.
This paper describes a bidirectional isolated DC/DC converter considered as a core circuit for next‐generation 3.3‐kV/6.6‐kV high‐power‐density power conversion systems. The DC/DC converter is intended to use power switching devices based on SiC and/or GaN, which will be available on the market in the near future. A 350‐V, 10‐kW, and 20‐kHz DC/DC converter is designed, constructed, and tested in this paper. It consists of two single‐phase full‐bridge converters with the latest trench‐gate Si‐IGBTs and a 20‐kHz transformer with a nano‐crystalline soft‐magnetic material core and litz wires. The transformer plays an essential role in achieving galvanic isolation between the two full‐bridge converters. The overall efficiency from the DC‐input to DC‐output terminals is accurately measured to be as high as 97%, excluding gate drive circuit and control circuit losses from the whole loss. Moreover, loss analysis is carried out to estimate effectiveness in using SiC‐based power switching devices. The loss analysis clarifies that the use of SiC‐based power devices may bring a significant reduction in conducting and switching losses to the DC/DC converter. As a result, the overall efficiency may reach 99% or higher. © 2008 Wiley Periodicals, Inc. Electr Eng Jpn, 163(2): 75–83, 2008; Published online in Wiley InterScience ( www.interscience.wiley.com ). DOI 10.1002/eej.20505 相似文献
95.
In our previous study, the effects of the interval between the cylinder and the airfoil on the aerodynamic sound were investigated and compared with the cases of single circular and single airfoil. In this study, the effects of the attack angle of the airfoil located downstream on the characteristics of aerodynamic sound and the wake structure are investigated at a given interval between the cylinder and the airfoil. It is found that the sound pressure level of DFN and the peak frequency decrease with increasing attack angle of airfoil because of the diffusive wake structure due to the increased back pressure of circular cylinder, which is caused by the blocking effect of airfoil. It is shown that the sound sources are corresponded to the attack points of shedding vortex form the upstream circular cylinder to the downstream airfoil. We conclude that the pressure fluctuation at the airfoil surface effects on the sound pressure level, from the flow visualizations and the exploration test of sound source. 相似文献
96.
97.
Dr. Naoki Umezawa Yuhei Horai Dr. Yuki Imamura Makoto Kawakubo Mariko Nakahira Dr. Nobuki Kato Akira Muramatsu Prof. Dr. Yuko Yoshikawa Prof. Dr. Kenichi Yoshikawa Prof. Dr. Tsunehiko Higuchi 《Chembiochem : a European journal of chemical biology》2015,16(12):1811-1819
A versatile solid‐phase approach based on peptide chemistry was used to construct four classes of structurally diverse polyamines with modified backbones: linear, partially constrained, branched, and cyclic. Their effects on DNA duplex stability and structure were examined. The polyamines showed distinct activities, thus highlighting the importance of polyamine backbone structure. Interestingly, the rank order of polyamine ability for DNA compaction was different to that for their effects on circular dichroism and melting temperature, thus indicating that these polyamines have distinct effects on secondary and higher‐order structures of DNA. 相似文献
98.
Sarah Katharina Gaßmeyer Hiroyuki Yoshikawa Junichi Enoki Nadine Hülsemann Prof. Raphael Stoll Prof. Dr. Kenji Miyamoto Prof. Dr. Robert Kourist 《Chembiochem : a European journal of chemical biology》2015,16(13):1943-1949
Structure‐guided protein engineering achieved a variant of the unique racemase AMDase G74C, with 40‐fold increased activity in the racemisation of several arylaliphatic carboxylic acids. Substrate binding during catalysis was investigated by saturation‐transfer‐difference NMR (STD‐NMR) spectroscopy. All atoms of the substrate showed interactions with the enzyme. STD‐NMR measurements revealed distinct nuclear Overhauser effects in experiments with and without molecular conversion. The spectroscopic analysis led to the identification of several amino acid residues whose substitutions increased the activity of G74C. Single amino acid exchanges increased the activity moderately; structure‐guided saturation mutagenesis yielded a quadruple mutant with a 40 times higher reaction rate. This study presents STD‐NMR as versatile tool for the analysis of enzyme–substrate interactions in catalytically competent systems and for the guidance of protein engineering. 相似文献
99.
Change in liquid temperature behind the impeller blades with impeller speed in boiling stirred tanks
In our previous study (Fukuda, R., Tokumura, M., Znad, H.T. and Kawase, Y., 2009, Vapour generation from the impellers in boiling stirred tank reactors. Chem Eng Res Des, 87: 452–459), it was found that in boiling stirred tanks with multiple impeller systems vapour was generated from the heater at lower impeller speeds and with an increase in impeller speed most vapour was generated from the top impeller rather than the lower impellers and the heater. The change of nucleation sites with the impeller speed might be controlled by the local liquid temperature. Therefore we measured the liquid temperature behind the impellers blades and found the decrease in liquid temperature with increasing impeller speed. In this paper, a simple model was developed to predict the change in liquid temperature behind the impeller blades in which nucleation takes place. In the proposed model based on the results for pressure distribution on the impeller blade in the literature, the liquid temperature behind the impeller blades is estimated from the measured power consumption. The validation of the proposed model was conducted using the experimental results in our previous study and reasonable agreement was obtained. 相似文献
100.
V. Matolín M. Cabala I. Matolínov M. koda M. Vclav K.C. Prince T. Skla T. Mori H. Yoshikawa Y. Yamashita S. Ueda K. Kobayashi 《Fuel Cells》2010,10(1):139-144
The interaction of Pt with CeO2 layers was investigated by using photoelectron spectroscopy. Thirty‐nanometre‐thick Pt and Sn doped CeO2 layers were deposited simultaneously by rf‐magnetron sputtering on a Si(001) substrate and a carbon diffusion layer of a polymer membrane fuel cell by using a composite CeO2–Pt–Sn target. The laboratory XPS and synchrotron radiation soft X‐ray and hard X‐ray photoemission spectra showed the formation of cerium oxide with completely ionised Pt2+,4+ species, and with Pt4+ embedded in the film bulk. Hydrogen/air fuel cell activity measurements normalised to the amount of Pt used revealed high specific power of up to 5.4 × 104 mW mg–1 (Pt). The activity of these materials is explained by the strong activity of embedded Ptn+ cations. 相似文献