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71.
72.
This note describes the results of research into the anthropometric measurements of women in Taiwan, for use in pantihose design. 相似文献
73.
轨道角动量(orbital angular momentum, OAM)的引入丰富了光通信领域内的调制维度,为寻找更高效快捷的通信方式提供了新思路,相较于传统携带涡旋相位的涡旋光束,部分相干扭曲光束携带的OAM性质更为复杂。本文针对椭圆多高斯关联扭曲光束在梯度折射率(gradient-index, GRIN)光纤中的OAM传输,基于GRIN光纤的ABCD光学传输矩阵,着重分析了多高斯关联扭曲光束在GRIN光纤传输的OAM的传输演化特性。研究结果表明,光束的光强、OAM通量密度以及归一化OAM通量密度在光纤传输过程中均呈现周期性变化,通过对关联结构以及扭曲因子的调控不仅可以改变光束OAM通量密度的分布,还可以调控单光子携带OAM的大小。本文的研究有助于丰富扭曲部分相干光束在GRIN光纤中传输的理论结果,在光纤通信中具有潜在的应用前景。 相似文献
74.
Dovletgeldi Seyitliyev Xixi Qin Manoj K. Jana Svenja M. Janke Xiaowei Zhong Wei You David B. Mitzi Volker Blum Kenan Gundogdu 《Advanced functional materials》2023,33(21):2213021
Electron–phonon interactions play an essential role in charge transport and transfer processes in semiconductors. For most structures, tailoring electron–phonon interactions for specific functionality remains elusive. Here, it is shown that, in hybrid perovskites, coherent phonon modes can be used to manipulate charge transfer. In the 2D double perovskite, (AE2T)2AgBiI8 (AE2T: 5,5“-diylbis(amino-ethyl)-(2,2”-(2)thiophene)), the valence band maximum derived from the [Ag0.5Bi0.5I4]2– framework lies in close proximity to the AE2T-derived HOMO level, thereby forming a type-II heterostructure. During transient absorption spectroscopy, pulsed excitation creates sustained coherent phonon modes, which periodically modulate the associated electronic levels. Thus, the energy offset at the organic–inorganic interface also oscillates periodically, providing a unique opportunity for modulation of interfacial charge transfer. Density-functional theory corroborates the mechanism and identifies specific phonon modes as likely drivers of the coherent charge transfer. These observations are a striking example of how electron–phonon interactions can be used to manipulate fundamentally important charge and energy transfer processes in hybrid perovskites. 相似文献
75.
Yiqian Du Zhikai Yan Wenbin You Qiaoqiao Men Guanyu Chen Xiaowei Lv Yuyang Wu Kaicheng Luo Biao Zhao Jincang Zhang Renchao Che 《Advanced functional materials》2023,33(34):2301449
Surface chemistry and interlayer engineering determines the electrical properties of 2D MXene. However, it remains challenging to regulate the surface and interfacial chemistry of MXene simultaneously. Herein, simultaneous modulation of Ti3C2Tx MXene surface termination and layer spacing by alkali treatment are achieved. The electrical and electromagnetic properties of Ti3C2Tx are investigated in detail with respect to KOH and ammonia concentration dependence. A high concentration of KOH caused the Ti3C2Tx layer spacing to expand to 13.7 Å and the surface O/F ratio to increase to 33.84. Because of its weaker ionization effect, ammonia provides finer tuning compared to the drastic intercalation of KOH with a thorough sweeping of the F-containing groups. Ti3C2Tx is enriched with conductive -OH termination after ammonia treatment, which achieves an effective balance with the increased interlayer resistance. Therefore, NH3H2O-Ti3C2Tx achieves broad-band impedance matching and exhibits an efficient microwave loss of −49.1 dB at a low thickness of 1.7 mm, with an effective frequency bandwidth of 3.9 GHz. The results herein optimize the electrical properties of Ti3C2Tx using surface and interfacial chemistry to achieve broad microwave absorption, providing a framework for enhancing the electromagnetic wave loss of intrinsic MXene. 相似文献
76.
Shihai You Tingting Zhu Yumin Wang Zeng-Kui Zhu Zhongyuan Li Jianbo Wu Panpan Yu Lina Li Chengmin Ji Yaxing Wang Shuao Wang Junhua Luo 《Advanced functional materials》2023,33(9):2210481
The exceptional photophysical properties of 3D organic–inorganic lead halide hybrids (OILHs) endow their significant potential for usage in optoelectronics, which has sparked intense research on novel 3D OILHs and associated applications. However, constructing new 3D OILHs based on large organic cations suffers from tough challenges due to the limitation of the Goldschmidt tolerance factor rule, let alone further explorations of their practical applications. Herein, a brand-new 3D lead chloride hybrid, (1MPZ)Pb4Cl10·H2O ( 1 , 1MPZ = 1-methylpiperazine) is reported, featuring a dense 3D lead chloride framework made of the corner-, edge-, and face-shared lead chloride polyhedra. 1 presents a broadband white light emission with a large Stokes shift and a nanosecond photoluminescence lifetime, which originates from radiative recombination of self-trapped excitons (STEs) induced by the highly distorted structure. Such a reabsorption-free and fast-decayed STEs emission coupling with the dense 3D architecture further enables 1 with effective X-ray scintillation with good sensitivity. Impressively, 1 also shows superior environmental and radiation stability. This study provides a new 3D OILH with appealing luminescence, not only expanding the 3D OILH family but also inspiring the exploitation of their optoelectronic applications. 相似文献
77.
Yi Wei Wei Wang Zhennan Wang Hang Yang Xinyu You Yunna Zhao Peipei Dang Hongzhou Lian Jianhua Hao Guogang Li Jun Lin 《Advanced functional materials》2023,33(2):2205829
Bismuth (Bi3+)-included lead-free metal halide (LFMH) materials attract much attention in lighting, display, photodetectors, X-ray detectors, and photovoltaic fields, due to the tunable luminescence and optoelectronic performance in response to crystal and electronic structure, morphology, and particle sizes. This review summarizes Bi3+-included LFMH materials about their preparation approach, crystal and electronic structure properties, luminescence performance, and emerging applications. Notably, Bi3+ ions not only can act as framework cation to construct stable LFMH structure, but can also incorporate into LFMH materials as activators or sensitizers to generate remarkable luminescence tuning and band engineering. The Bi3+ effect on the luminescence and optoelectronic properties of LFMH materials, including, promotion of exciton localization, enhancement of light absorption in near-ultraviolet region, action as sensitizer ions to transfer energy to rare earth or transition metal ions and emission of highly-efficient light is systematically summarized. The proposed structure-luminescence relationship offers guidance for the optimization of current Bi3+-included LFMH materials and the exploitation of new LFMH derivatives. 相似文献
78.
79.
Can Zhang Shijie Zhan Jian Wang Zhongjian Liu Hong You Yuhong Jia 《Clean Technologies and Environmental Policy》2017,19(4):991-1001
Recently, interspecies quorum quenching (QQ) by bacteria has been reported as a novel approach in biofouling control in membrane bioreactor (MBR) for wastewater treatment. In this study, seven QQ bacteria, named RO1 to RO7, were isolated from fouling reverse osmosis (RO) membrane and were encapsulated in the microbial filters for biofouling control in MBR. Results showed that all isolates have extracellular QQ activity, and RO1 to RO6 were characterized as heat-stable enzymatic degradation of N-acyl homoserine lactones (AHLs), while RO7 was mainly pH-dependent. Analysis of the 16S rRNA gene indicated that RO7 was a species of Pseudomonas sp., others belonged to the species of Bacillus, Stenotrophomonas maltophilia and Delftia tsuruhatensis, respectively. Then, the microbial filters encapsulated each isolate were applied in a laboratory-scaled MBR and proved the substantial inhibition effect on membrane biofouling except for RO7, indicating that QQ bacteria employing enzymes to degrade AHLs have great potential in biofouling control in MBR. 相似文献
80.
Carbon Nanodot‐Sensitized Modulation of Alzheimer's β‐Amyloid Self‐Assembly,Disassembly, and Toxicity 下载免费PDF全文
You Jung Chung Kayoung Kim Byung Il Lee Chan Beum Park 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(34)
The self‐assembly of amyloidogenic peptides into β‐sheet‐rich aggregates is a general feature of many neurodegenerative diseases, including Alzheimer's disease, which signifies the need for the effective attenuation of amyloid aggregation toward alleviating amyloid‐associated neurotoxicity. This study reports that photoluminescent carbon nanodots (CDs) can effectively suppress Alzheimer's β‐amyloid (Aβ) self‐assembly and function as a β‐sheet breaker disintegrating preformed Aβ aggregates. This study synthesizes CDs using ammonium citrate through one‐pot hydrothermal treatment and passivates their surface with branched polyethylenimine (bPEI). The bPEI‐coated CDs (bPEI@CDs) exhibit hydrophilic and cationic surface characteristics, which interact with the negatively charged residues of Aβ peptides, suppressing the aggregation of Aβ peptides. Under light illumination, bPEI@CDs display a more pronounced effect on Aβ aggregation and on the dissociation of β‐sheet‐rich assemblies through the generation of reactive oxygen species from photoactivated bPEI@CDs. The light‐triggered attenuation effect of Aβ aggregation using a series of experiments, including photochemical and microscopic analysis, is verified. Furthermore, the cell viability test confirms the ability of photoactivated bPEI@CDs for the suppression of Aβ‐mediated cytotoxicity, indicating bPEI@CDs' potency as an effective anti‐Aβ neurotoxin agent. 相似文献