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81.
Hidenori Hiramatsu Takayoshi Katase Yoshihiro Ishimaru Akira Tsukamoto Toshio Kamiya Keiichi Tanabe Hideo Hosono 《Materials Science and Engineering: B》2012,177(7):515-519
Relationships between microstructure and transport properties of bicrystal grain boundary (BGB) junctions were studied in cobalt-doped BaFe2As2 (BaFe2As2:Co) epitaxial films grown on [0 0 1]-tilt bicrystal substrates of MgO and (La, Sr)(Al, Ta)O3 with misorientation angles θGB = 3–45°. The θGB of BaFe2As2:Co BGBs were exactly transferred from those of the bicrystal substrates. No segregation of impurities was detected at the BGB junction interfaces, and the chemical compositions of the BGBs were uniform and the same as those in the bulk film regions. A transition from a strongly-coupled GB behavior to a weak-link behavior was observed in current density–voltage characteristics under self-field around θGB ~ 9°. The critical current density decreased from (1.2–1.6) × 106 A/cm2 of the intragrain transport to (0.7–1.1) × 105 A/cm2 of θGB = 45° because supercurrent becomes more governed by Josephson current with increasing θGB. 相似文献
82.
Robles R Lorente N Isshiki H Liu J Katoh K Breedlove BK Yamashita M Komeda T 《Nano letters》2012,12(7):3609-3612
Being able to control the spin of magnetic molecules at the single-molecule level will make it possible to develop new spin-based nanotechnologies. Gate-field effects and electron and photon excitations have been used to achieve spin switching in molecules. Here, we show that atomic doping of molecules can be used to change the molecular spin. Furthermore, a scanning tunneling microscope was used to place or remove the atomic dopant on the molecule, allowing us to change the molecular spin in a controlled way. Bis(phthalocyaninato)yttrium (YPc(2)) molecules deposited on an Au (111) surface keep their spin-1/2 magnetic moment due to the small molecule-substrate interaction. However, when Cs atoms were carefully placed onto YPc(2) molecules, the spin of the molecule vanished as shown by our conductance measurements and corroborated by the results of density functional theory calculations. 相似文献
83.
Tetsuhiko Maeda Keiichi NishidaManabu Tange Toru TakahashiAkihiro Nakano Hiroshi ItoYasuo Hasegawa Masao MasudaYoshiaki Kawakami 《International Journal of Hydrogen Energy》2011,36(17):10845-10854
Numerical simulation of a hydrogen storage tank of a Totalized Hydrogen Energy Utilization System (THEUS) for application to commercial buildings was done to verify the practicality of THEUS. THEUS consists of a fuel cell, water electrolyzer, hydrogen storage tank and their auxiliary machinery. The hydrogen storage tanks with metal hydrides for load leveling have been previously experimentally investigated as an important element of THEUS. A hydrogen storage tank with 50 kg AB5 type metal hydride was assembled to investigate the hydrogen-absorbing/desorbing process, which is exothermic/endothermic process. The goal of this tank is to recover the cold heat of the endothermic process for air conditioning, and thus improve the efficiency of THEUS. To verify the practical effectiveness of this improved system, we developed a numerical simulation code of hydrogen storage tank with metal hydride. The code was validated by comparing its results with experimental results. In this code the specific heat value of the upper and lower flanges of the hydrogen storage tank was adjusted to be equal to the thermal capacity of the entire tank. The simulation results reproduce well the experimental results. 相似文献
84.
Keiichi Shibata 《Journal of Nuclear Science and Technology》2017,54(2):147-157
Neutron nuclear data on 10 isotopes of platinum have been evaluated for the next version of Japanese Evaluated Nuclear Data Library general-purpose file in the energy region from 10?5 eV to 20 MeV. Resolved resonance parameters of naturally occurring isotopes were taken from a compilation work, while unresolved resonance parameters were obtained by fitting to the total and capture cross sections calculated from nuclear models. A statistical model code was applied to evaluate cross sections above the resolved resonance region. Compound, pre-equilibrium and direct-reaction processes were considered for cross-section calculation. Coupled-channel optical model parameters were employed for the interaction between neutrons and nuclei. Giant-dipole and pygmy resonance parameters for E1 γ-ray transition from platinum isotopes were determined so as to reproduce measured γ-ray spectrum. The present results reproduce experimental data very well. The evaluated data are compiled into Evaluated Nuclear Data File formatted data files. 相似文献
85.
Hirohisa Narita Keiichi Shirase Eiji Arai Keiichi Nakamoto Lian-Yi Chen Hideo Fujimoto 《国际生产研究杂志》2013,51(17):3657-3673
In order to satisfy the recent various consumers’?needs, an advanced manufacturing system will be required. So, the innovative concept of Future Oriented Machine Tools (FOMT), which consists of four function blocks to realize the advanced manufacturing system, is proposed. The four function blocks are Management, Prediction, Observation and Strategy, and intelligent manufacturing processes are realized by utilizing these function blocks. FOMT can make a significant contribution in four stages: design stage, production scheduling stage, machining stage and post-machining stage. In the design stage, the product information such as accuracy can be evaluated in CAD, considering the manufacturing ability concurrently. In the production scheduling stage, the product schedules can be generated automatically and flexibly for the various products. In the machining stage, cutting conditions adjusted autonomously according to the machining status and machining problems. In the post-machining stage, the machining know-how data are accumulated and stored for future production and human engineers. The feasibility of it, especially the machining stage, is discussed using the developed cutting process simulator called VMSim (virtual machining simulator) from the view points of cutting force, machining error and environmental burden (CO2 emission). 相似文献
86.
Jin Nishikawa Kazuya Nakamura Mohammad Asadullah Tomohisa Miyazawa Kimio Kunimori Keiichi Tomishige 《Catalysis Today》2008,131(1-4):146-155
In the steam gasification of biomass, the additive effect of noble metals such as Pt, Pd, Rh and Ru to the Ni/CeO2/Al2O3 catalyst was investigated. Among these noble metals, the addition of Pt was most effective even when the loading amount of added Pt was as small as 0.01 wt.%. In addition, the catalyst characterization suggests the formation of the Pt–Ni alloy over the Pt/Ni/CeO2/Al2O3. 相似文献
87.
Rheological properties in a molten state are studied extensively for poly(3‐hydroxybutyrate‐co‐3‐hydroxyvalerate), PHB‐HV, with a small amount of crosslinked poly(epichlorohydrin), PECH, having low density of crosslink points. It is found that adding 2 wt % of xPECH greatly enhances the melt elasticity of PHB‐HV, one of the serious defects of microbial PHB, whereas it has no effect on the shear viscosity. As a result, viscoelastic nature, and thus processability, of PHB‐HV can be controlled by blending the crosslinked PECH. © 2007 Wiley Periodicals, Inc. J Appl Polym Sci, 2008 相似文献
88.
We investigated the surface potential built across the electrode/fullerene (C60) or copper phthalocyanine (CuPc) interface and C60/CuPc interface as a function of the thickness of the semiconductor film in the dark condition and under illumination. The surface potential of C60 on Au, Al and Mg changes negatively with the increment of film thickness and it saturates at − 0.25, − 1.0 and − 1.5 V within 20 nm. The Fermi level alignment at C60/electrode interface is established within ∼ 20 nm from electrode, and very high electric field exists due to the displacement of negative electronic charges from electrode into C60. On the other hand, the surface potential of CuPc on ITO changes to + 0.1 V, and the work functions of C60 and CuPc were estimated as 5.0 eV and 4.7 eV. C60 film also accepts electrons from CuPc at hetero-junction interface, and the Fermi-level alignment was again obtained at C60/CuPc interface under illumination. The built-in potential of ca. 0.3 V formed at C60/CuPc interface was considered as the origin of the reduction of open-circuit voltage in ITO/CuPc/C60/Au device compared with the optimum value of 0.6 V. On the other hand, the very high electric field formed at C60/Mg contact improved the photovoltaic properties. 相似文献
89.
To investigate the effect of molecular structure on macroscopic flow behavior of polymeric liquid, attempts have been made to embed the microscopic information into the flow simulation. Constitutive equation based on the theory of polymer dynamics is ideal but the theory is still under development. The CONNFFESSIT approach (where microscopic simulation is embedded into calculation grid in macroscopic simulation) is another promising direction but the computational cost is not practical yet. In this study, we propose another simple method using parameter-based bridging where the parameters for phenomenological constitutive equations in macroscopic flow simulation are obtained from coarse-grained molecular simulation. As an example, we performed a simulation of injection molding and examined the effect of molecular weight on warpage of the molded product. We used the primitive chain network simulation to calculate linear viscoelasticity of linear monodispersed polystyrenes from molecular weight. The obtained linear viscoelasticity was converted into the relaxation spectrum and into the flow curve to be used in the macroscopic simulations. From the flow curve, the parameters of an inelastic non-Newtonian constitutive equation were obtained and used for the simulation of filling process. The relaxation spectrum was used to calculate residual stress from the flow profile in the filling process. From the residual stress and thermal shrinkage, warpage of the product was obtained. For the examined thin plate product, significant change in the warpage direction was demonstrated according to the molecular weight of the material. © 2012 Wiley Periodicals, Inc. J Appl Polym Sci, 2012 相似文献
90.
Kawamura A Ooyama K Kojima K Kachi H Abe T Amano K Aoyama T 《Journal of oleo science》2011,60(12):597-607
Disruption of the skin barrier function caused by epidermal hyper-proliferation, results in the skin becoming dry and showing high transepidermal water loss (TEWL). Gamma linolenic acid (GLA) is reportedly efficacious for treating TEWL and epidermal hyper-proliferation. In this study, to elucidate the effect of GLA-rich oil on skin function, GLA-containing food was given to adults with dry skin or mild atopic dermatitis and skin parameters were evaluated. In the results, we recognized beneficial effects on the TEWL index. The efficacy of GLA was also demonstrated to be statistically significant especially in subjects with pro-inflammatory features. The results suggest that the mechanism of improvement of skin barrier has been associated with possible generation of anti-inflammatory metabolites from GLA. The clinical physician also confirmed that none of the subjects showed any noteworthy side effects. GLA-enriched food appears to be safe and to improve skin barrier function in subjects with dry skin conditions and mild atopic dermatitis. 相似文献