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131.
Yang Li Defu Che Chenglong Yang Mingyu Yao Tingwen Zhao Kangli Fu Hanchen Zhao 《中国化学工程学报》2021,29(1):401-408
SO2 and NO emitted from coal-fired power plants have caused serious air pollution in China. In this study, a test system for NO oxidation using O3 is established. The basic characteristics of NO oxidation and products forms are studied. A separate test system for the combined removal of SO2 and NOx is also established, and the absorption characteristics of NOx are studied. The characteristics of NO oxidation and NOx absorption were verified in a 35 t·h-1 industrial boiler wet combined desulfurization and denitrification project. The operating economy of ozone oxidation wet denitrification technology is analyzed. The results show that O3 has a high rate and strong selectivity for NO oxidation. When O3 is insufficient, the primary oxidation product is NO2. When O3 is present in excess, NO2 continues to get oxidized to N2O5 or NO3. The removal efficiency of NO2 in alkaline absorption system is low (only about 15%). NOx removal efficiency can be improved by oxidizing NOx to N2O5 or NO3 by increasing ozone ratio. When the molar ratio of O3/NO is 1.77, the NOx removal efficiency reaches 90.3%, while the operating cost of removing NOx per kilogram is 6.06 USD (NO2). 相似文献
132.
The nucleation efficiency (NE) of stereocomplex crystallites (SCs) formed in asymmetric poly(L-lactide)/poly(D-lactide) (PLLA/PDLA) blends is generally unsatisfactory because the competition between stereocomplexation and chain mixing involved in the melt-mixing process can cause low formation efficiency and even severe aggregation of SCs. Herein, it is attempted to achieve high-efficient formation of finely dispersed SCs particles by designing a unique melt-mixing procedure, where the mixing of PLLA with 0.75 wt% PDLA is first performed at elevated temperatures (far above the melting temperature of SCs) to allow the homogeneous mixing of PLLA/PDLA chains and then at a low temperature (slightly above that of homocrystallites) to permit the full stereocomplexation of the premixed chains. It is found that the SCs formed in the blends exhibit unexpectedly low NEs (e.g., 54.5%), much inferior to that (73.6%) in the counterpart without undergoing premixing. This is because the introduction of premixing leads to a remarkable deterioration in the amount of SCs particles formed, despite decreased particle size, highlighting that the direct mixing at low temperatures of 170–180 °C (about 20–30 °C lower than that used in common melt-processing of PLA) is more effective for the construction of SCs with superior NE. The mechanisms for these striking findings are discussed. 相似文献
133.
Tanyalak Parimon Miriam S. Hohmann Changfu Yao 《International journal of molecular sciences》2021,22(12)
Pulmonary fibrosis is a chronic and fatal lung disease that significantly impacts the aging population globally. To date, anti-fibrotic, immunosuppressive, and other adjunct therapy demonstrate limited efficacies. Advancing our understanding of the pathogenic mechanisms of lung fibrosis will provide a future path for the cure. Cellular senescence has gained substantial interest in recent decades due to the increased incidence of fibroproliferative lung diseases in the older age group. Furthermore, the pathologic state of cellular senescence that includes maladaptive tissue repair, decreased regeneration, and chronic inflammation resembles key features of progressive lung fibrosis. This review describes regulatory pathways of cellular senescence and discusses the current knowledge on the senescence of critical cellular players of lung fibrosis, including epithelial cells (alveolar type 2 cells, basal cells, etc.), fibroblasts, and immune cells, their phenotypic changes, and the cellular and molecular mechanisms by which these cells contribute to the pathogenesis of pulmonary fibrosis. A few challenges in the field include establishing appropriate in vivo experimental models and identifying senescence-targeted signaling molecules and specific therapies to target senescent cells, known collectively as “senolytic” or “senotherapeutic” agents. 相似文献
134.
Caroline K. Brennan Marya Y. Ornelas Zi W. Yao Prof. Dr. Jennifer A. Prescher 《Chembiochem : a European journal of chemical biology》2021,22(16):2650-2654
Bioluminescent tools have been used for decades to image processes in complex tissues and preclinical models. However, few distinct probes are available to probe multicellular interactions. We and others are addressing this limitation by engineering new luciferases that can selectively process synthetic luciferin analogues. In this work, we explored naphthylamino luciferins as orthogonal bioluminescent probes. Three analogues were prepared using an optimized synthetic route. The luciferins were found to be robust emitters with native luciferase in vitro and in cellulo. We further screened the analogues against libraries of luciferase mutants to identify unique enzyme-substrate pairs. The new probes can be used in conjunction with existing bioluminescent tools for multi-component imaging. 相似文献
135.
Yang Zhu Xiangli Meng Qiang Zhang Liansheng Yan Hong Cui 《International Journal of Applied Ceramic Technology》2021,18(4):1330-1341
A 3D architecture carbon fiber preform, specifically fine-woven cloth and punctured felt preform, is used to manufacture a novel advanced Cf/C-SiC-ZrC composite. The composite matrix is produced by chemical vapor infiltration (CVI) plus precursor infiltration and pyrolysis (PIP) process and finalized by using a chemical vapor deposition (CVD) of SiC coating to make the final density of the material reach 1.95 g/cm3. The organic precursors of SiC and ZrC have a weight ratio of 4:1 in a xylene solute. The composite mechanical properties, such as tensile, compression, bending, shear, and Z-direction load bearing, are introduced under analysis to find possible applications for the composite. What is more, scanning electron microscope (SEM) images are employed to illustrate the failure behavior of the ceramic composite. The results showed that the punctured filament tows will be beneficial, not only for the composite to withstand compression force up to 308.6 MPa and shear strength to 18.14 MPa but also for the alternatively stacked weave piles and short fiber layers to support the punctured bundles, as well as to hold the composite structure under mechanical forces from different orientations, which is believed to reinforce the ceramic matrix for some high pressure and severe ablation applications. 相似文献
136.
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138.
Chai Linjiang Xia Jiying Murty Korukonda L. Gu Xinfu Fan Jiangkun Yao Zhongwen 《Metallurgical and Materials Transactions A》2022,53(8):3179-3193
Metallurgical and Materials Transactions A - A hot-rolled Ti–6Al–4V sheet was annealed at 960 °C (sub β-transus temperature) and then subjected to different coolings [in water... 相似文献
139.
Zhang Hongtao Cai Minghui Zhu Wanjun Sun Shenghui Yan Haile Yao Shengjie Luan Yikun Tang Shuai Hodgson P. D. 《Metallurgical and Materials Transactions A》2022,53(11):3869-3880
Metallurgical and Materials Transactions A - A cold-rolled low Al-added medium Mn steel was employed to investigate the low-temperature superplastic deformation at a relatively high initial strain... 相似文献
140.