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Ordered mesoporous SnO2 and mesoporous Pd/SnO2 have been successfully synthesized via nanocasting method using the hexagonal mesoporous SBA-15 as template. Two different procedures, impregnation technique and direct synthesis, were utilized for the doping of Pd in the mesoporous SnO2. The results of small angle X-ray diffraction (SAXD), nitrogen adsorption–desorption and transmission electron microscopy (TEM) demonstrate that the SnO2 and Pd/SnO2 display ordered mesoporous structures and high surface areas. Wide angle X-ray diffraction (WAXD) and X-ray photoelectron spectroscopy (XPS) reveal tetragonal structure of SnO2 and the existence of Pd element. The sensing properties of mesoporous SnO2 and mesoporous Pd/SnO2 for H2 were detected. The sensor utilizing mesoporous Pd/SnO2 via direct synthesis method exhibits excellent response and recovery behavior and much higher sensitivity to H2, compared to those using mesoporous SnO2 and mesoporous Pd/SnO2 via impregnation technique. It is believed that its high gas sensing performance is derived from the large surface area, high activity and well dispersion of Pd additive, as well as high porosity, which lead to highly effective surface interaction between the target gas molecules and the surface active sites.  相似文献   
84.
In this work, we aim to discover real-world events from Flickr data by devising a three-stage event detection framework. In the first stage, a multimodal fusion (MF) model is designed to deal with the heterogeneous feature modalities possessed by the user-shared data, which is advantageous in computation complexity. In the second stage, a dual graph regularized non-negative matrix factorization (DGNMF) model is proposed to learn compact feature representations. DGNMF incorporates Laplacian regularization terms for the data graph and base graph into the objective, keeping the geometry structures underlying the data samples and dictionary bases simultaneously. In the third stage, hybrid clustering algorithms are applied seamlessly to discover event clusters. Extensive experiments conducted on the real-world dataset reveal the MF-DGNMF-based approaches outperform the baselines.  相似文献   
85.
The aim of this paper is to present a microstructural topology optimization methodology for the structural-acoustic coupled system. In the structural-acoustic system, the structure is considered to be a thin composite plate composed of periodic uniform microstructures. The discrete design variables are used in the microstructural topology optimization, and the constitutive matrix is interpolated by the power-law scheme at the micro scale. The equivalent macro material properties of the microstructure are computed through the homogenization method. The design objective is to minimize the sound pressure level (SPL) in an interior acoustic medium. The sensitivities of the SPL with respect to design variables are derived. The bi-directional evolutionary structural optimization (BESO) method is extended to solve the structural-acoustic coupled optimization problem to find the optimal material distribution of the microstructure. Numerical examples of a hexahedral box and an automobile passenger compartment are given to demonstrate the efficiency of the presented microstructural topology optimization method.  相似文献   
86.
在802.11 WLAN(Wireless Local Network)中,当一些无线节点的传输速率明显低于其他节点与AP(Access Point)间的传输速率时,将会使区域内所有节点的传输性能降低,这种现象称为效果异常(Performance Anomaly),Hyogon K等人在文献[6-7]中提出用改变封包容量和竞争窗口大小的方式来解决这个问题.文章通过在NS2网络仿真环境下,设计实验拓扑,编写性能分析脚本,对效果异常现象进行仿真并验证了上述两种方案能够有效缓解该现象并保持系统传输性能稳定.  相似文献   
87.
In the partition of unity (PU)-based methods, the global approximation is built by multiplying a partition of unity by local approximations. Within this framework, high-order approximations are achieved by directly adopting high-order polynomials as local approximations, and therefore nodes along sides or inside elements, which are usually adopted in the conventional finite element methods, are no more required. However, the PU-based approximation constructed in this way may suffer from rank deficiency due to the linear dependence of the global degrees of freedom. In this paper, the origin of the rank deficiency in the PU-based approximation space is first dissected at an element level, and then an approach to predict the rank deficiency for a mesh is proposed together with the principle of the increase of rank deficiency. Finally, examples are investigated to validate the present approach. The current work indicates such a fact that the rank deficiency is an unrelated issue to the nullity of the global matrix. It can be resolved in its own manner.  相似文献   
88.
论文介绍了文本分类技术的研究进展及发展方向,给出了中英文文本分类系统构建的一般模型和过程,分析总结了中英文文本分类过程中的异同,并介绍了针对这些异同因素常用的处理方法。  相似文献   
89.
The surface tension of the Ni3S2-FeS-Cu2S ternary mattes have been calculated from those of the Ni3S2-FeS·FeS-Cu2S and Cu2S-Ni3S2 pseudo-binary boundary systems by using geometric models (Kohler and Toop model) and a general solution model (Chou model). Taking account of the experimental accuracy of ±2.5%, the respective calculated results are in agreement with the experimental data. At the same time, surface tensions of molten Ni3S2-FeS-Cu2S mattes and their pseudo-binary boundary systems are predicted based on Butler's original treatment with great attention to the model parameter β. The predicted results also agree with the experimental data. Therefore, the resulting iso-surface tension curves in molten Ni3S2-FeS-Cu2S mattes at 1473K, especially calculated by using Kohler, Toop and Chou models, are generally acceptable.  相似文献   
90.
作为辐射生物学发展的前沿,微束已经成为当今世界上用来研究低剂量辐射生物效应的一个强有力手段.单离子微束装置是一种将离子束斑的直径限制在微米量级范围内,并能将预定数目的离子精确注入到细胞中某一指定位置的辐射装置.结合一套自行开发的控制程序,CAS-LIBB微束装置的计算机控制系统可以实施对生物样品的精确定量和定点辐射.本文首先给出了装置定量和定点辐射的精度测定结果,该精度完全能够胜任细胞-亚细胞尺度的精确辐射.接下来详细探讨了控制系统的改进工作,最后对控制系统进行了展望.  相似文献   
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