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81.
Eigler DM Lutz CP Crommie MF Manoharan HC Heinrich AJ Gupta JA 《Philosophical transactions. Series A, Mathematical, physical, and engineering sciences》2004,362(1819):1135-1147
We discuss two examples of novel information-transport and processing mechanisms in nanometre-scale structures. The local modulation and detection of a quantum state can be used for information transport at the nanometre length-scale, an effect we call a 'quantum mirage'. We demonstrate that, unlike conventional electronic information transport using wires, the quantum mirage can be used to pass multiple channels of information through the same volume of a solid. We discuss a new class of nanometre-scale structures called 'molecule cascades', and show how they may be used to implement a general-purpose binary-logic computer in which all of the circuitry is at the nanometre length-scale. 相似文献
82.
This work addresses the problem of improving the generalization capabilities of continuous recurrent neural networks. The learning task is transformed into an optimal control framework in which the weights and the initial network state are treated as unknown controls. A new learning algorithm based on a variational formulation of Pontrayagin's maximum principle is proposed. Under reasonable assumptions, its convergence is discussed. Numerical examples are given that demonstrate an essential improvement of generalization capabilities after the learning process of a dynamic network. 相似文献
83.
Object-oriented (OO) modeling languages, tools, and methods more and more attract the interest of embedded (real-time) system developers. This is especially true if embedded (real-time) system software has to cooperate with interactive multimedia software, as it is more and more the case in automotive systems. It is still an open question whether and how the standard OO modeling language UML and its accompanying tools have to be adapted to the regarded application domain. This paper evaluates the development of a rapid prototype for an air condition controller with the popular CASE tool Rational Rose/RT®. We point out some weaknesses of the presented solution and propose an extension to Rose/RT®, which overcomes the weaknesses by combining Rose/RTs UML dialect with data flow equations. 相似文献
84.
Establishment of a knee-joint coordinate system from helical axes analysis--a kinematic approach without anatomical referencing 总被引:1,自引:0,他引:1
Mannel H Marin F Claes L Dürselen L 《IEEE transactions on bio-medical engineering》2004,51(8):1341-1347
This study establishes a functional knee-joint coordinate system (FCS) derived from active motion. The scale invariant properties of helical axes were used in order to avoid inter-observer errors associated with the traditional anatomical referencing techniques. The algorithm was tested with six cadaveric specimens in a knee-joint motion and loading apparatus. To determine the FCS sensitivity to variable loading, rotational moments were applied to the tibia while extending and flexing the knee. Each derived FCS was compared with the clinically derived anatomical coordinate system (ACS). The FCS was reproducible when the loading condition was the same. Changing the rotational moments from internal to external affected the orientations and the positions of the FCS. The largest displacement of 20.8 mm in average occurred in the medio/lateral direction. The FCS corresponded with the ACS for all specimens and loading conditions. The origin was always located within the femur along the transepicondylar line. The orientations differed less than 16.6 degrees in average, thus allowing the use of clinical terminology. These findings suggest that the FCS might improve the ability to clinically assess kinematic alterations provided that the reference motion is reproducible. 相似文献
85.
Prager L Mark G Mätzing H Paur HR Schubert J Frimmel FH Hesse S Schuchmann HP Schuchmann MN von Sonntag C 《Environmental science & technology》2003,37(2):379-385
The electron-beam (EB) degradation of volatile aromatics (benzene, toluene, ethylbenzene, xylenes: BTEX) in groundwater strip gas, which in the present work has been modeled by the introduction of the desired aromatic(s) to a stream of air or another gas, such as oxygen, is initiated essentially by the addition of *OH radicals to the aromatic ring, giving rise to hydroxycyclohexadienyl radicals, which form the corresponding peroxyl radicals upon addition of oxygen. As studied in some detail with benzene as a BTEX representative, various reactions of these lead to numerous oxidation products in a cascade of reactions, including the decomposition of products under the prevailing conditions of high turnover of the initial aromatic. Importantly, hydroxycyclohexadienylperoxyl radical formation is partly reversible, and the reactions of the hydroxycyclohexadienyl radicals, which thus have a significant presence in these systems, must therefore also be taken into consideration. In the gas phase, in contrast to the aqueous phase (see Part 1), the reactions of the hydroxycyclohexadienyl radicals lead to oligomeric products that appear to contribute, in addition to ionic clusters, to nucleation for the aerosols observed. Various nitrated products, among them nitrophenols, are observed when air is used for the stripping. However, these studies did not clear the pilot plant stage, since BTEX degradation using a bioreactor carried out in parallel was so successful that the EB technology was judged to be noncompetitive. As for the latter, expensive equipment consisting of a stripper, the EB machine, and an aerosol precipitator would be required. The condensed aerosols are biorefractory and would require further treatment for detoxification. 相似文献
86.
Using both Rayleigh scattering and time-resolved emission spectroscopy, we have recorded the spatial and temporal evolution of laser-generated sparks in argon from changes during the first ten of nano-seconds to complete dissipation, which occurs in a time span of approximately 5 ms. Maps of either emission intensity or argon density spanning the entire region affected by the energy deposited by the laser show the dissipation of the spark in detail. Immediately after ignition, the argon plasma occupies an ellipsoidal volume of roughly 3-mm vertical (axial) length. After approximately 20-40 micros, the spark region has transformed into a toroidal shape in a plane perpendicular to the vertical axis, with a radius of approximately 1.5 mm. The torus rises slowly up and expands noticeably in the radial direction. A record of peak temperatures of the spark ranging from approximately 10,000 K at 60-micros delay time to approximately 450 K at 4-ms delay time indicate cooling rates from approximately 100 to 1 K/micros at these times. 相似文献
87.
Diffuse reflection infrared Fourier transform (DRIFT) spectra of the hydroxides Mg(OH)2 and Zn(OH)F and the iodate hydrates beta-Ni(IO3)2.4H2O and Ni(IO3)2.2H2O have been recorded at ambient and high temperature. Spectra without shifts of the band maxima compared to those of conventional infrared transmission spectra and without inversion of the bands were obtained by dilution of the compounds to about 2-10% with an appropriate embedding material. alpha-Al2O3, TiO2, ZrO2, PbF2, MgO, BaO, ZnO, Na2SiO3, SiO2 (aerosil), and powdered copper, aluminum, and magnesium were tested as diluents for hydrates and hydroxides, especially at elevated temperatures, as alternatives for the commonly used KBr. Thus, alpha-Al2O3, PbF2, and powdered copper were established as the most favorable diluents. Using these novel embedding materials, high-temperature DRIFT spectra are obtainable at temperatures not accessible with KBr discs. Dehydration and decomposition of the iodate hydrates under study were shown by change or disappearance of the respective water bands. 相似文献
88.
A homology model of penicillin acylase from Alcaligenes faecalis and in silico evaluation of its selectivity 总被引:1,自引:0,他引:1
Braiuca P Ebert C Fischer L Gardossi L Linda P 《Chembiochem : a European journal of chemical biology》2003,4(7):615-622
A three-dimensional model of the relatively unknown penicillin acylase from Alcaligenes faecalis (PA-AF) was built up by means of homology modeling based on three different crystal structures of penicillin acylase from various sources. An in silico selectivity study was performed to compare this homology model to the structure of the Escherichia coli enzyme (PA-EC) in order to find any selectivity differences between the two enzymes. The program GRID was applied in combination with the principal component analysis technique to identify the regions of the active sites where the PAs potentially engage different interactions with ligands. These differences were further analyzed and confirmed by molecular docking simulations. The PA-AF homology model provided the structural basis for the explanation of the different enantioselectivities of the enzymes previously demonstrated experimentally and reported in the literature. Different substrate selectivities were also predicted for PA-AF compared to PA-EC. Since no crystallographic data are available for PA-AF to date, the three-dimensional homology model represents a useful and efficient tool for fully exploiting this attractive and efficient biocatalyst, particularly in enantioselective acylations of amines. 相似文献
89.
Complying with the obligation in the current ozone directive, the European Commission came forward in 1999 with a strategy to combat tropospheric ozone together with a proposed revision of the air quality legislation for this pollutant. As a daughter legislation under the 1996 Framework Directive on Air Quality, the proposed ozone daughter directive defines for the first time (interim) air quality targets for ozone to be attained by 2010, complemented by long-term objectives for ozone based on the guideline values of the World Health Organisation. It also sets out enhanced requirements for monitoring and assessment of ozone concentrations, as well as minimum criteria for appropriate information of the public about the measured air pollution.In the past, abatement strategies against air pollution consisted of concrete obligations for controlling emissions derived solely on the basis of technical and economic aspects, covering specific types of installations or activities, thus with no direct quantitative relationship to the level of air pollution let alone to its effects.In compensating this deficit, the Commission presented, as a complement to the existing sectoral legislation, a proposal for a directive on national emission ceilings (NEC) which quantifies emission targets for every Member State to bring its total precursor emissions by 2010 down to levels being considered as necessary to achieve everywhere on a regional scale the air quality targets set in the ozone daughter directive.As the core element of the ozone abatement strategy, the national ceilings for emissions of sulfur dioxide (SO(2)), nitrogen oxides (NO(x)), ammonia (NH(3)) and volatile organic compounds (VOC) were derived from a cost-effectiveness analysis integrating information on economic, technical, physical and biological aspects of ozone pollution and abatement. This integrated assessment considers the potential and costs for further emission control in the various economic sectors in the Member States and combines this with information on ozone formation and transport processes in the atmosphere and with indicators for the impact of ozone on human health and environmental. Reflecting the discussions with Member States and stakeholders, a number of decisive steps in the process of deriving the national emission ceilings are presented here: the way of framing interim objectives, how to choose an appropriate ambition level, aspects of how to cope with uncertainties in the model and the input data and how to treat extreme meteorological situations and resolve problems in the spatial distribution of the interim objectives given the different size of countries. Finally, the paper explains the scenario underpinning the proposed national emission ceilings, its environmental gains and the distribution of cost incurring for emission control measures in Member States. 相似文献
90.
Lutz Volkmann 《Information Processing Letters》2007,103(6):234-239
Since interconnection networks are often modeled by graphs or digraphs, the edge-connectivity of a graph or arc-connectivity of a digraph are important measurements for fault tolerance of networks.The restricted edge-connectivity λ′(G) of a graph G is the minimum cardinality over all edge-cuts S in a graph G such that there are no isolated vertices in G−S. A connected graph G is called λ′-connected, if λ′(G) exists.In 1988, Esfahanian and Hakimi [A.H. Esfahanian, S.L. Hakimi, On computing a conditional edge-connectivity of a graph, Inform. Process. Lett. 27 (1988), 195-199] have shown that each connected graph G of order n?4, except a star, is λ′-connected and satisfies λ′(G)?ξ(G), where ξ(G) is the minimum edge-degree of G.If D is a strongly connected digraph, then we call in this paper an arc set S a restricted arc-cut of D if D−S has a non-trivial strong component D1 such that D−V(D1) contains an arc. The restricted arc-connectivity λ′(D) is the minimum cardinality over all restricted arc-cuts S.We observe that the recognition problem, whether λ′(D) exists for a strongly connected digraph D is solvable in polynomial time. Furthermore, we present some analogous results to the above mentioned theorem of Esfahanian and Hakimi for digraphs, and we show that this theorem follows easily from one of our results. 相似文献