全文获取类型
收费全文 | 983篇 |
免费 | 34篇 |
专业分类
电工技术 | 50篇 |
化学工业 | 345篇 |
金属工艺 | 16篇 |
机械仪表 | 23篇 |
建筑科学 | 13篇 |
能源动力 | 44篇 |
轻工业 | 93篇 |
水利工程 | 2篇 |
石油天然气 | 1篇 |
无线电 | 69篇 |
一般工业技术 | 214篇 |
冶金工业 | 22篇 |
原子能技术 | 25篇 |
自动化技术 | 100篇 |
出版年
2023年 | 9篇 |
2022年 | 20篇 |
2021年 | 27篇 |
2020年 | 18篇 |
2019年 | 19篇 |
2018年 | 20篇 |
2017年 | 15篇 |
2016年 | 25篇 |
2015年 | 23篇 |
2014年 | 48篇 |
2013年 | 79篇 |
2012年 | 40篇 |
2011年 | 90篇 |
2010年 | 73篇 |
2009年 | 41篇 |
2008年 | 56篇 |
2007年 | 58篇 |
2006年 | 34篇 |
2005年 | 40篇 |
2004年 | 50篇 |
2003年 | 32篇 |
2002年 | 24篇 |
2001年 | 14篇 |
2000年 | 19篇 |
1999年 | 7篇 |
1998年 | 13篇 |
1997年 | 9篇 |
1996年 | 19篇 |
1995年 | 14篇 |
1994年 | 9篇 |
1993年 | 8篇 |
1992年 | 6篇 |
1991年 | 4篇 |
1990年 | 9篇 |
1989年 | 11篇 |
1988年 | 4篇 |
1987年 | 3篇 |
1986年 | 6篇 |
1985年 | 3篇 |
1984年 | 3篇 |
1983年 | 3篇 |
1982年 | 3篇 |
1981年 | 3篇 |
1980年 | 1篇 |
1979年 | 2篇 |
1978年 | 1篇 |
1977年 | 2篇 |
排序方式: 共有1017条查询结果,搜索用时 15 毫秒
11.
Masaru Takahashi Tetsu Nakatani Shinji Iwamoto Tsunenori Watanabe Masashi Inoue 《Applied catalysis. B, Environmental》2007,70(1-4):73-79
The solvothermal reaction of mixtures of aluminum isopropoxide (AIP) and gallium acetylacetonate (Ga(acac)3) directly yielded the mixed oxides of γ-Ga2O3-Al2O3. In the solvothermal synthesis, the crystal structure of mixed oxides was controlled by the initial formation of γ-Ga2O3 nuclei. The mixed oxides prepared in diethylenetriamine have extremely high activities for selective catalytic reduction (SCR) of NO with methane as a reducing agent. With increasing crystallite size of the spinel structure, the catalytic activity increased. The ratio of the amount of methane consumed by combustion to total methane conversion was proportional to the density of acid sites on the surface of the mixed oxides. The mixed oxide catalysts prepared in diethylenetriamine had lower densities of acid sites and showed a higher methane-efficiency for CH4-SCR than those prepared in other solvents. These catalysts maintained their high activity even when the reaction was carried out under the severe conditions (i.e., high space velocity and low NO concentration). 相似文献
12.
Masaru Takahashi Noriyuki Inoue Tatsuya Takeguchi Shinji Iwamoto Masashi Inoue Tsunenori Watanabe 《Journal of the American Ceramic Society》2006,89(7):2158-2166
The reaction of mixtures of aluminum isopropoxide and gallium acetylacetonate in 1,4-butanediol or 1,5-pentanediol at high temperatures (glycothermal reaction) directly gave the γ-Ga2 O3 –Al2 O3 solid solutions, which had high catalytic activities for selective reduction of NO using methane as the reducing agent. However, the reaction with a higher Al/(Ga+Al) charged ratio yielded the glycol derivative of boehmite as a by-product and the catalytic activity of the solid solution decreased. Therefore, synthesis of the solid solution using various glycols was examined and it was found that solid solutions with high Al contents without contamination of the glycol derivative of boehmite were obtained by using 1,6-hexanediol as a reaction medium. The solid solution exhibited a higher NO conversion than that synthesized in other glycols. 相似文献
13.
Residues important for the function of a multihelical DNA binding domain in the new transcription factor family of Cam and Tet repressors 总被引:5,自引:0,他引:5
Aramaki Hironori; Yagi Naoto; Suzuki Masashi 《Protein engineering, design & selection : PEDS》1995,8(12):1259-1266
We report that some prokaryotic repressors including CamR andTetR belong to the same family. CamR and TetR bind to DNA usinga multihelical DNA binding domain (DBD) at the N-termini ofthe proteins, while the C-termini are important for regulatingthe DNA binding in a manner dependent on their co-factors (camphorfor CamR, tetracycline for TetR). In all, 11 important aminoacid positions have been identified in the CamR DBD by the systematicsubstitution of residues by Ala. Of the 11 positions, 10 areeither buried in the core, and thus important for creating thehydrophobic environment, or exposed on the surface, and thusimportant for binding to DNA. The eleventh residue, Gly, seemsto be important for a loop structure. The DNA binding mode ofthis type of DBD and a general mechanism of regulating theirDNA binding are discussed in reference to the crystal structureof TetR [Hinrichs et al., (1994) Science, 264, 418420]. 相似文献
14.
Takako Takasu Noritaka Ishihara Masashi Oota Yoshimi Ishiguro Yoichi Kurosawa Koji Dairiki Shunpei Yamazaki 《Journal of the Society for Information Display》2015,23(12):593-599
We have reported that the transistors having the c‐axis‐aligned crystalline (CAAC) In‐Ga‐Zn oxide (IGZO) show good performance. Recently, In‐Sn‐Zn Oxide (ITZO) has attracted much attention because of its high electron mobility, as well as IGZO. However, it has been reported that ITZO field effect transistors (FET) tend to have positive Vth (normally‐on characteristics) and poor reliability compared with IGZO‐FETs. We have reported that high‐performance and high‐reliability OS‐FETs can be fabricated by using CAAC‐IGZO, which has high crystallinity and has no clear grain boundaries, as an active layer. Therefore, we have fabricated CAAC‐ITZO thin films to improve performance of ITZO‐FETs by using CAAC‐ITZO as an active layer. In addition, FETs employing CAAC‐ITZO have better characteristics and reliability than FETs using nano‐crystal ITZO. Furthermore, constant photocurrent method (CPM) measurement was carried out in order to estimate density of deep‐level defect states caused by oxygen vacancies in oxide semiconductors. The results show that CAAC‐ITZO has lower density of deep‐level defect states than nano‐crystal ITZO. We attribute the improvement in reliability of ITZO‐FETs to a decrease in deep‐level defect states of an ITZO active layer, as is the case with IGZO. 相似文献
15.
16.
A DC (data center) demands air-conditioning power as large as the 1/3-1/2 of total electricity consumption. Thus, energy saving of cooling power of DC yields considerable effect on both economic and environmental views. PV (Photovoltaic) and absorption refrigerator with CGS (cogeneration systems) or gas boiler are possible power saving options. The waste warm air from DC would be utilized for greenhouse heating when DC and greenhouse locate near in the suburbs. In this study, the authors develop an energy network model to assess the potential contribution of DC as a major electric power and chilled air consumer as well as the warm air supplier in a district to the energy efficiency improvement. The evaporation heat of LNG (liquefied natural gas) utilization is also considered as well as PV, CGS. This model is applied to the cases of the urban area in Tokyo which involves athletic center, shops and hospital and the suburbs including greenhouse and then compared. 相似文献
17.
在全球的CDMA运营商中,日本KDDI是非常突出的一家。KDDI于2002年4月推出了自己的3G业务,采用的是cdma20001x技术。与NTTDoCoMo的3G业务一开始缓慢发展相比,KDDI虽晚半年推出3G业务,但其3G业务一起步就进入了快速发展阶段,业务开展才84天,用户数就突破百万大关。到2004年10月,用户数突破1600万的KDDI。那么,到底是什么使KDDI后来居上的呢?本文试图从分析KDDI的业务人手,破解KDDI的成功密码. 相似文献
18.
A technique for preparation of a pillar-shaped specimen and its multidirectional observation using a combination of a scanning transmission electron microscope (STEM) and a focused ion beam (FIB) instrument has been developed. The system employs an FIB/STEM compatible holder with a specially designed tilt mechanism, which allows the specimen to be tilted through 360 degrees [T. Yaguchi, M. Konno, T. Kamino, T. Hashimoto, T. Ohnishi, K. Umemura, K. Asayama, Microsc. Microanal. 9 (Suppl. 2) (2003) 118; T. Yaguchi, M. Konno, T. Kamino, T. Hashimoto, T. Ohnishi, M. Watanabe, Microsc. Microanal. 10 (Suppl. 2) (2004) 1030]. This technique was applied to obtain the three-dimensional (3D) elemental distributions around a contact plug of a Si device used in a 90-nm technology. A specimen containing only one contact plug was prepared in the shape of a pillar with a diameter of 200nm and a length of 5mum. Elemental maps were obtained from the pillar specimen using a 200-kV cold-field emission gun (FEG) STEM model HD-2300C equipped with the EDAX genesis X-ray energy-dispersive spectrometry (XEDS) system through a spectrum imaging technique. In this study, elemental distributions of minor elements with weak signals were enhanced by applying principal component analysis (PCA), which is a superior technique to extract weak signals from a large dataset. The distributions of elements, especially the metallization component Ti and minor dopant As in this particular device, were successfully extracted by PCA. Finally, the 3D elemental distributions around the contact plug could be visualized by reconstruction from the tilt series of maps. 相似文献
19.
In order to facilitate the implementations ofTMN interface protocols/services studied inITU-T, it is very important to define profiles for supportingTMN management service. This paper proposes a concrete method for achieving this based on osi management standards as a promisingTMN implementation method. It proposes an idea of structuring theTMN ISP’S based on the structure of the osi managementISP’S. The paper discusses aTMN based on the osi managementISP’S. Finally the implementation as software is discussed and a software architecture for efficient application development is proposed. 相似文献
20.
Zihan Ma Xiaofei Lu Sunghyun Park Tatsuya Shinagawa Masashi Okubo Kazuhiro Takanabe Atsuo Yamada 《Advanced functional materials》2023,33(25):2214466
Hydrogen is a promising alternative to fossil fuels that can reduce greenhouse gas emissions. Decoupled water electrolysis system using a reversible proton storage redox mediator, where the oxygen evolution reaction and hydrogen evolution reaction are separated in time and space, is an effective approach to producing hydrogen gas with high purity, high flexibility, and low cost. To realize fast hydrogen production in such a system, a redox mediator capable of releasing protons rapidly is required. Herein, α-MoO3, with an ultrafast proton transfer property that can be explained by a dense hydrogen bond network in the lattice oxygen arrays of HxMoO3, is examined as a high-rate redox mediator for fast hydrogen production in acidic electrolytes. The α-MoO3 redox mediator shows both a large capacity of 204 mAh g−1 and fast hydrogen production at a current rate of 10 A cm−2(≈153 A g−1), outperforming most of the previously reported solid-state redox mediators. 相似文献