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排序方式: 共有1340条查询结果,搜索用时 31 毫秒
91.
JosA. Castillo Christine Gurard‐Hlaine Mariana Gutirrez Xavier Garrabou Martine Sancelme Melanie Schürmann Tomoyuki Inoue Virgil Hlaine Franck Charmantray Thierry Gefflaut Laurence Hecquet Jesús Joglar Pere Claps GeorgA. Sprenger Marielle Lemaire 《Advanced Synthesis \u0026amp; Catalysis》2010,352(6):1039-1046
A mutant of D ‐fructose‐6‐phosphate aldolase (FSA) of Escherichia coli, FSA A129S, with improved catalytic efficiency towards dihydroxyacetone (DHA), the donor substrate in aldol addition reactions, was explored for synthetic applications. The kcat/KM value for DHA was 17‐fold higher with FSA A129S than that with FSA wild type (FSA wt). On the other hand, for hydroxyacetone as donor substrate FSA A129S was found to be 3.5‐fold less efficient than FSA wt. Furthermore, FSA A129S also accepted glycolaldehyde (GA) as donor substrate with 3.3‐fold lower affinity than FSA wt. This differential selectivity of both FSA wt and FSA A129S for GA makes them complementary biocatalysts allowing a control over donor and acceptor roles, which is particularly useful in carboligation multi‐step cascade synthesis of polyhydroxylated complex compounds. Production of the mutant protein was also improved for its convenient use in synthesis. Several carbohydrates and nitrocyclitols were efficiently prepared, demonstrating the versatile potential of FSA A129S as biocatalyst in organic synthesis. 相似文献
92.
Direct steam generation in parabolic trough or linear Fresnel collectors represents one interesting technological option for concentrating solar electricity production. Today's state of the art characterized by the first commercial plants in operation is a result of more than 20 years of intensive research on this topic. This article provides a review on the key results from research that includes physical effects like heat transfer and pressure drop in horizontal boiler tubes, plant layout considerations, and thermal storage options. An overview on test and demonstration facilities as well as on commercial plants is given, leading to an outlook on the next generation of direct steam generation systems. 相似文献
93.
A composite material was prepared from graphene and palladium nanoparticles (PdNP) by layer-by-layer deposition on gold electrodes. The material was characterized by absorption spectroscopy, scanning electron microscopy, Raman spectroscopy and surface plasmon resonance. Cyclic voltammetry demonstrated the presence of electrocatalytic centers in the palladium decorated graphene. This material can serve as a sensor material for hydrogen at levels from 0.5 to 1% in synthetic air. Pure graphene is poorly sensitive to hydrogen, but incorporation of PdNPs increases its sensitivity by more than an order of magnitude. The effects of hydrogen, nitrogen dioxide and humidity were studied. Sensor regeneration is accelerated in humid air. The sensitivity of the nanocomposite depends on the number of bilayers of graphene–PdNPs. 相似文献
94.
Neutral iodobromide emulsions made by the addition of silver nitrate to alkali halides in gelatin may, under certain conditions, contain a proportion of grains with cores of iodobromide phases. The maximum iodide contents (i) of these cores are related to the precipitation temperature (T) by the empirical equation i= 34.5+0.165(T–25). Grains containing such cores show very regular print-out distribution. 相似文献
95.
Norman MUIRHEAD Paul A. KEOWN David N. CHURCHILL Melanie POULIN‐COSTELLO Sandeep GANTOTTI Lei LEI Matthew GITLIN Tracy J. MAYNE 《Hemodialysis international. International Symposium on Home Hemodialysis》2011,15(1):87-94
The risks/benefits of anemia treatment in dialysis patients have been redefined in the US Epoetin α label. This analysis was carried out to determine if increasing hemoglobin (Hb) levels improve exercise tolerance and physical function in anemic dialysis patients. This is a new analysis of the Canadian Erythropoietin Study Group trial, a double‐blind, randomized, placebo‐controlled trial in dialysis patients. Subjects were 18 to 75 years old, on hemodialysis for >3 months, and had a baseline Hb <9.0 g/dL. Patients with a history of diabetes mellitus, ischemic heart disease, or severe/uncontrolled hypertension were excluded. Patients were randomized to receive Epoetin α to a target Hb of 9.5 to 11.0 g/dL (n=40) or a target of 11.5 to 13.0 g/dL (n=38), or receive placebo (n=40). Results from patients in the Epoetin‐α–treated arms were combined for this analysis. Hb level, exercise tolerance (Treadmill Stress Test and 6‐Minute Walk Test) and patient‐reported physical function measures (Physical Summary domain from the Kidney Disease Questionnaire, and 4 domains from the Sickness Impact Profile) were reported at baseline and months 2, 4, and 6. Differences in measures were statistically significant for exercise tolerance (Treadmill Stress, P=0.0001) and patient‐reported physical function (Kidney Disease Questionnaire Physical, P=0.0001; Sickness Impact Profile Physical, P=0.0015) across all time points for Epoetin‐α–treated patients compared with placebo. Improvements were seen at 2 months and were maintained through months 4 and 6. Dialysis patients receiving Epoetin α showed improved exercise tolerance and physical function. These findings should be considered as physicians weigh the risks and benefits of treatment. 相似文献
96.
Price W.W. Hargrave A.W. Hurysz B.J. Chow J.H. Hirsch P.M. 《Power Systems, IEEE Transactions on》1998,13(3):768-774
This paper presents the results of applying the EPRI Dynamic Equivalencing Program to a large-scale system test case of the New York Power Pool. The effects of coherent generator selection, network reduction, generator aggregation, and generator modeling on the accuracy of the reduced models are investigated 相似文献
97.
Melanie Po-Leen Ooi Hong Kuan Sok Ye Chow Kuang Serge Demidenko Chris Chan 《Engineering Applications of Artificial Intelligence》2013,26(3):1029-1043
The International Technology Roadmap for Semiconductors (ITRS) identifies production test data as an essential element in improving design and technology in the manufacturing process feedback loop. One of the observations made from the high-volume production test data is that dies that fail due to a systematic failure have a tendency to form certain unique patterns that manifest as defect clusters at the wafer level. Identifying and categorising such clusters is a crucial step towards manufacturing yield improvement and implementation of real-time statistical process control. Addressing the semiconductor industry’s needs, this research proposes an automatic defect cluster recognition system for semiconductor wafers that achieves up to 95% accuracy (depending on the product type). 相似文献
98.
Sonja Berg Melanie J. Leng Christopher P. Kendrick Holger Cremer Bernd Wagner 《SILICON》2013,5(1):19-34
Organic carbon occluded in diatom silica is assumed to be protected from degradation in the sediment. δ13C from diatom carbon (δ13C(diatom)) therefore potentially provides a signal of conditions during diatom growth. However, there have been few studies based on δ13C(diatom). Numerous variables can influence δ13C of organic matter in the marine environment (e.g., salinity, light, nutrient and CO2 availability). Here we compare δ13C(diatom) and δ13C(TOC) from three sediment records from individual marine inlets (Rauer Group, East Antarctica) to (i) investigate deviations between δ13C(diatom) and δ13C(TOC), to (ii) identify biological and environmental controls on δ13C(diatom) and δ13C(TOC), and to (iii) discuss δ13C(diatom) as a proxy for environmental and climate reconstructions. The records show individual δ13C(diatom) and δ13C(TOC) characteristics, which indicates that δ13C is not primarily controlled by regional climate or atmospheric CO2 concentration. Since the inlets vary in water depths offsets in δ13C are probably related to differences in water column stratification and mixing, which influences redistribution of nutrients and carbon within each inlet. In our dataset changes in δ13C(diatom) and δ13C(TOC) could not unequivocally be ascribed to changes in diatom species composition, either because the variation in δ13C(diatom) between the observed species is too small or because other environmental controls are more dominant. Records from the Southern Ocean show depleted δ13C(diatom) values (1–4 ‰) during glacial times compared to the Holocene. Although climate variability throughout the Holocene is low compared to glacial/interglacial variability, we find variability in δ13C(diatom), which is in the same order of magnitude. δ13C of organic matter produced in the costal marine environment seems to be much more sensitive to environmental changes than open ocean sites and δ13C is of strongly local nature. 相似文献
99.
We tested the hypothesis that poor performance on the Piagetian invisible displacement task is related to increased memory requirements. Rhesus monkeys and orangutans received 3 types of problems (invisible, visible, and no transfer problems) each containing a number of steps equivalent to that of standard invisible displacements. If failure to solve invisible displacements was due to increased memory requirements, then the primates should perform at chance level on all 3 problems. However, rhesus monkeys solved visible and no transfer problems, but not invisible transfer problems. Half of the orangutans solved all 3 transfer problems, although their performance on invisible transfer problems was lower than that on the other problems. A subsequent cuing phase led to improved performance, and a few monkeys solved invisible transfer problems. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
100.
C. Collado G. GoglioG. Demazeau A.S. BarrièreL. Hirsch M. Leroux 《Materials Research Bulletin》2002,37(5):841-848
GaN microcrystallites have been prepared by a solvothermal process. The influence of the synthesis temperature on the crystallinity of the resulting GaN has been studied on three samples, prepared at 400, 600 and 800°C in the same pressure conditions (150 MPa) and duration (6 h). The resulting powders were characterized by several techniques: X-ray diffraction to evaluate the reaction rate, scanning electron microscopy (SEM) to determine the morphology and size of the microcrystallites and photoluminescence to evaluate the quality of the powders. 相似文献