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排序方式: 共有6838条查询结果,搜索用时 15 毫秒
951.
952.
Xiaoen Wang Robert Kerr Fangfang Chen Nicolas Goujon Jennifer M. Pringle David Mecerreyes Maria Forsyth Patrick C. Howlett 《Advanced materials (Deerfield Beach, Fla.)》2020,32(18):1905219
With increasing demands for safe, high capacity energy storage to support personal electronics, newer devices such as unmanned aerial vehicles, as well as the commercialization of electric vehicles, current energy storage technologies are facing increased challenges. Although alternative batteries have been intensively investigated, lithium (Li) batteries are still recognized as the preferred energy storage solution for the consumer electronics markets and next generation automobiles. However, the commercialized Li batteries still have disadvantages, such as low capacities, potential safety issues, and unfavorable cycling life. Therefore, the design and development of electromaterials toward high-energy-density, long-life-span Li batteries with improved safety is a focus for researchers in the field of energy materials. Herein, recent advances in the development of novel organic electrolytes are summarized toward solid-state Li batteries with higher energy density and improved safety. On the basis of new insights into ionic conduction and design principles of organic-based solid-state electrolytes, specific strategies toward developing these electrolytes for Li metal anodes, high-energy-density cathode materials (e.g., high voltage materials), as well as the optimization of cathode formulations are outlined. Finally, prospects for next generation solid-state electrolytes are also proposed. 相似文献
953.
Charles Guillemard Wei Zhang Gregory Malinowski Claudia de Melo Jon Gorchon Sebastien Petit-Watelot Jaafar Ghanbaja Stéphane Mangin Patrick Le Fèvre Francois Bertran Stéphane Andrieu 《Advanced materials (Deerfield Beach, Fla.)》2020,32(26):1908357
Engineering of magnetic materials for developing better spintronic applications relies on the control of two key parameters: the spin polarization and the Gilbert damping, responsible for the spin angular momentum dissipation. Both of them are expected to affect the ultrafast magnetization dynamics occurring on the femtosecond timescale. Here, engineered Co2MnAlxSi1-x Heusler compounds are used to adjust the degree of spin polarization at the Fermi energy, P, from 60% to 100% and to investigate how they correlate with the damping. It is experimentally demonstrated that the damping decreases when increasing the spin polarization from 1.1 × 10−3 for Co2MnAl with 63% spin polarization to an ultralow value of 4.6 × 10−4 for the half-metallic ferromagnet Co2MnSi. This allows the investigation of the relation between these two parameters and the ultrafast demagnetization time characterizing the loss of magnetization occurring after femtosecond laser pulse excitation. The demagnetization time is observed to be inversely proportional to 1 – P and, as a consequence, to the magnetic damping, which can be attributed to the similarity of the spin angular momentum dissipation processes responsible for these two effects. Altogether, the high-quality Heusler compounds allow control over the band structure and therefore the channel for spin angular momentum dissipation. 相似文献
954.
Martin D. Hager Birgit Esser Xinliang Feng Wolfgang Schuhmann Patrick Theato Ulrich S. Schubert 《Advanced materials (Deerfield Beach, Fla.)》2020,32(39):2000587
Batteries have become an integral part of everyday life—from small coin cells to batteries for mobile phones, as well as batteries for electric vehicles and an increasing number of stationary energy storage applications. There is a large variety of standardized battery sizes (e.g., the familiar AA-battery or AAA-battery). Interestingly, all these battery systems are based on a huge number of different cell chemistries depending on the application and the corresponding requirements. There is not one single battery type fulfilling all demands for all imaginable applications. One battery class that has been gaining significant interest in recent years is polymer-based batteries. These batteries utilize organic materials as the active parts within the electrodes without utilizing metals (and their compounds) as the redox-active materials. Such polymer-based batteries feature a number of interesting properties, like high power densities and flexible batteries fabrication, among many more. 相似文献
955.
Thanh Tran-Phu Manjunath Chatti Joshua Leverett Thi Kim Anh Nguyen Darcy Simondson Dijon A Hoogeveen Alexander Kiy The Duong Bernt Johannessen Jaydon Meilak Patrick Kluth Rose Amal Alexandr N. Simonov Rosalie K. Hocking Rahman Daiyan Antonio Tricoli 《Small (Weinheim an der Bergstrasse, Germany)》2023,19(25):2208074
Unlocking the potential of the hydrogen economy is dependent on achieving green hydrogen (H2) production at competitive costs. Engineering highly active and durable catalysts for both oxygen and hydrogen evolution reactions (OER and HER) from earth-abundant elements is key to decreasing costs of electrolysis, a carbon-free route for H2 production. Here, a scalable strategy to prepare doped cobalt oxide (Co3O4) electrocatalysts with ultralow loading, disclosing the role of tungsten (W), molybdenum (Mo), and antimony (Sb) dopants in enhancing OER/HER activity in alkaline conditions, is reported. In situ Raman and X-ray absorption spectroscopies, and electrochemical measurements demonstrate that the dopants do not alter the reaction mechanisms but increase the bulk conductivity and density of redox active sites. As a result, the W-doped Co3O4 electrode requires ≈390 and ≈560 mV overpotentials to reach ±10 and ±100 mA cm−2 for OER and HER, respectively, over long-term electrolysis. Furthermore, optimal Mo-doping leads to the highest OER and HER activities of 8524 and 634 A g−1 at overpotentials of 0.67 and 0.45 V, respectively. These novel insights provide directions for the effective engineering of Co3O4 as a low-cost material for green hydrogen electrocatalysis at large scales. 相似文献
956.
Stella Gries Manuel Brinker Berit Zeller-Plumhoff Dagmar Rings Tobias Krekeler Elena Longo Imke Greving Patrick Huber 《Small (Weinheim an der Bergstrasse, Germany)》2023,19(22):2370157
Many biological materials exhibit a multiscale porosity with small, mostly nanoscale pores as well as large, macroscopic capillaries to simultaneously achieve optimized mass transport capabilities and lightweight structures with large inner surfaces. Realizing such a hierarchical porosity in artificial materials necessitates often sophisticated and expensive top-down processing that limits scalability. Here, an approach that combines self-organized porosity based on metal-assisted chemical etching (MACE) with photolithographically induced macroporosity for the synthesis of single-crystalline silicon with a bimodal pore-size distribution is presented, i.e., hexagonally arranged cylindrical macropores with 1 µm diameter separated by walls that are traversed by pores 60 nm across. The MACE process is mainly guided by a metal-catalyzed reduction–oxidation reaction, where silver nanoparticles (AgNPs) serve as the catalyst. In this process, the AgNPs act as self-propelled particles that are constantly removing silicon along their trajectories. High-resolution X-ray imaging and electron tomography reveal a resulting large open porosity and inner surface for potential applications in high-performance energy storage, harvesting and conversion or for on-chip sensorics and actuorics. Finally, the hierarchically porous silicon membranes can be transformed structure-conserving by thermal oxidation into hierarchically porous amorphous silica, a material that could be of particular interest for opto-fluidic and (bio-)photonic applications due to its multiscale artificial vascularization. 相似文献
957.
Forschung im Ingenieurwesen - Anschmierungen innerhalb von Wälzlagern zählen zu den Verschleißarten, die bis heute nicht vollständig verstanden wurden. Bekannt ist, dass... 相似文献
958.
Scientometrics - This paper applies clustering techniques and multi-dimensional scaling (MDS) analysis to a 500?×?500 composers’ similarity/distance matrix. The objective is... 相似文献
959.
Neural Computing and Applications - The state-of-the-art performance of deep learning models comes at a high cost for companies and institutions, due to the tedious data collection and the heavy... 相似文献
960.