Air-Stable Li2S Cathode for Quasi-Solid-State Anode-Free Batteries with High Volumetric Energy

Anode-free batteries can maximize the energy density but their development is hindered by a lack of Li-rich cathodes for compensating the irreversible Li loss. Li₂S cathode is particularly appealing to this desire due to 2.6–4.7 folds more Li content and 4.2–6.8 times higher capacity than conventional intercalation cathodes. But its practical application is hindered by poor stability against moisture attacking in the air. Herein, a facile expendable polymer sheathing strategy toward air-stable Li₂S cathodes with high capacities for developing high-performance quasi-solid-state anode-free batteries without risk of cell leakage is reported. Tight protection by dense polymer barrier dramatically prolongs the lifetime of Li₂S cathode by 2,000 times at least in the air. Such air-stable Li₂S cathode allows for high compatibility of anode-free battery production with commercial schemes. More attractively, the polymer protective layer can in situ transform to multifunctional gel polymer electrolyte for releasing ionic pathways and enhancing cell performance by inhibiting LiPS loss and smoothing Li plating. With air-stable Li₂S cathode, the quasi-solid-state anode-free cells are assembled in ambient environment to deliver superb volumetric energy density of 1093 Wh L⁻¹. This study may shed new light to push the commercialization of high-energy and reliable anode-free batteries forward.     

Wavelet CMAC for MIMO uncertain nonlinear systems using a modified social ski-driver algorithm

This study uses a Mexican hat wavelet membership function for a cerebellar model articulation controller (CMAC) to develop a more efficient adaptive controller for multiple input multiple output (MIMO) uncertain nonlinear systems. The main controller is called the adaptive Mexican hat wavelet CMAC (MWCMAC), and an auxiliary controller is used to remove the residual error. For the MWCMAC, the online learning laws are derived from the gradient descent method. In addition, the learning rate values are very important and have a great impact on the performance of the control system; however, they are difficult to choose accurately. Therefore, a modified social ski driver (SSD) algorithm is proposed to find optimal learning rates for the control parameters. Finally, a magnetic ball levitation system and a nine-link biped robot are used to illustrate the effectiveness of the proposed SSD-based MWCMAC control system. The comparisons with other existing control algorithms have shown the superiority of the proposed control system.     

Complex Attributed Network Embedding for medical complication prediction

Knowledge and Information Systems - To assure the development of effective treatment plans, it is crucial for understanding the complication relationships among diseases. In practice, traditional...     

A model of checkpoint behavior for applications that have I/O

Due to the increase and complexity of computer systems, reducing the overhead of fault tolerance techniques has become important in recent years. One technique in fault tolerance is checkpointing, which saves a snapshot with the information that has been computed up to a specific moment, suspending the execution of the application, consuming I/O resources and network bandwidth. Characterizing the files that are generated when performing the checkpoint of a parallel application is useful to determine the resources consumed and their impact on the I/O system. It is also important to characterize the application that performs checkpoints, and one of these characteristics is whether the application does I/O. In this paper, we present a model of checkpoint behavior for parallel applications that performs I/O; this depends on the application and on other factors such as the number of processes, the mapping of processes and the type of I/O used. These characteristics will also influence scalability, the resources consumed and their impact on the IO system. Our model describes the behavior of the checkpoint size based on the characteristics of the system and the type (or model) of I/O used, such as the number I/O aggregator processes, the buffering size utilized by the two-phase I/O optimization technique and components of collective file I/O operations. The BT benchmark and FLASH I/O are analyzed under different configurations of aggregator processes and buffer size to explain our approach. The model can be useful when selecting what type of checkpoint configuration is more appropriate according to the applications’ characteristics and resources available. Thus, the user will be able to know how much storage space the checkpoint consumes and how much the application consumes, in order to establish policies that help improve the distribution of resources.

     

High Q 2D-length extension mode resonators for potential time–frequency applications

Microsystem Technologies - This paper presents recent advances on two dimensional length-extension mode (2D-LEM) quartz resonators providing high quality (Q) factor on resonances at a few MHz. The...     

Intelligent wavelet fuzzy brain emotional controller using dual function-link network for uncertain nonlinear control systems

This study aims to propose a more efficient hybrid algorithm to achieve favorable control performance for uncertain nonlinear systems. The proposed algorithm comprises a dual function-link network-based multilayer wavelet fuzzy brain emotional controller and a sign(.) functional compensator. The proposed algorithm estimates the judgment and emotion of a brain that includes two fuzzy inference systems for the amygdala network and the prefrontal cortex network via using a dual-function-link network and three sub-structures. Three sub-structures are a dual-function-link network, an amygdala network, and a prefrontal cortex network. Particularly, the dual-function-link network is used to adjust the amygdala and orbitofrontal weights separately so that the proposed algorithm can efficiently reduce the tracking error, follow the reference signal well, and achieve good performance. A Lyapunov stability function is used to determine the adaptive laws, which are used to efficiently tune the system parameters online. Simulation and experimental studies for an antilock braking system and a magnetic levitation system are presented to verify the effectiveness and advantage of the proposed algorithm.

     

基于神威·太湖之光的非结构网格计算加速算法

在国产异构众核平台神威·太湖之光上的非结构网格计算具有稀疏存储、离散访存、数据依赖等特点,严重制约了众核处理器的性能发挥。为解决稀疏存储和离散访存问题,提出一种N阶对角染色算法,以有效平衡主从核计算并利用从核将全局访存转化为LDM访问。针对数据依赖造成的计算竞争问题,采用自适应和无依赖的任务划分方法,避免并行计算时的数据冲突。为对处理器架构和非结构网格计算进行优化,采用主核与从核异步并行的方式,差异化使用主从核以充分利用硬件资源,同时,取消处理器提供的寄存器通信机制,降低从核阵列的同步开销同时便于扩展到新一代神威平台。此外,使用计算访存异步重叠技术来充分隐藏访存延迟。利用SpMV、Integration、calcLudsFcc算子进行实验,结果表明,相比主核实现,组合加速算法在不同算例规模下平均取得了10倍的加速效果,加速比最高可达24倍,N阶对角染色算法相比非染色分块算法取得了超过5.8倍的性能加速,有效提升了数据局部性和计算并行度。该算法对有依赖关系的计算冲突算子同样具有良好的加速性能,验证了自适应和无依赖任务划分方法的有效性。     

Bandwidth selection in kernel density estimation for interval-grouped data

When interval-grouped data are available, the classical Parzen–Rosenblatt kernel density estimator has to be modified to get a computable and useful approach in this context. The new nonparametric grouped data estimator needs of the choice of a smoothing parameter. In this paper, two different bandwidth selectors for this estimator are analyzed. A plug-in bandwidth selector is proposed and its relative rate of convergence obtained. Additionally, a bootstrap algorithm to select the bandwidth in this framework is designed. This method is easy to implement and does not require Monte Carlo. Both proposals are compared through simulations in different scenarios. It is observed that when the sample size is medium or large and grouping is not heavy, both bandwidth selection methods have a similar and good performance. However, when the sample size is large and under heavy grouping scenarios, the bootstrap bandwidth selector leads to better results.