A series of hydrophilic alkanethiols, HS(CH2)nOH with n = 3, 4, 6, 8, 9 and 11, have been self-assembled on gold electrodes of pentacene-based thin-film transistors. The multi-parametric and ultra-sensitive response of these devices allows us to characterize both charge–injection and electrical stability moving from vacuum to air. The decay exponent β of charge injection is found to be 0.7–1.1 Å?1 in agreement with earlier measurements of charge tunneling done by electrochemistry and large-area molecular junctions. We find that the intermediate chain lengths (n = 4 and 6) yield an optimum response as they represent the best compromise in terms of decrease of the contact-resistance and bias stress. 相似文献
An effective method to generate a large number of parallel sentences for training improved neural machine translation (NMT) systems is the use of the back-translations of the target-side monolingual data. The standard back-translation method has been shown to be unable to efficiently utilize huge amounts of existing monolingual data because of the inability of translation models to differentiate between authentic and synthetic parallel data during training. Tagging, or using gates, has been used to enable translation models to distinguish between synthetic and authentic data, improving standard back-translation and also enabling the use of iterative back-translation on language pairs that underperformed using standard back-translation. In this work, we approach back-translation as a domain adaptation problem, eliminating the need for explicit tagging. In our approach—tag-less back-translation—the synthetic and authentic parallel data are treated as out-of-domain and in-domain data, respectively, and through pre-training and fine-tuning, the translation model is shown to be able to learn more efficiently from them during training. Experimental results have shown that the approach outperforms the standard and tagged back-translation approaches on low resource English-Vietnamese and English-German NMT.
This study presents the effect of combined membrane separation and heterogeneous catalysts for the production of ethyl lactate solvent. The enhanced process is a flat sheet cellulose acetate membrane and cation-exchange resin catalysts. A methodology based on catalyst and acetate membrane impregnation in the presence of a sweep gas at low pressure with the aim of obtaining a higher yield of the ester product have been developed. The esterification reaction was carried out at the temperature of 60 °C. The ester product gave a percentage yield of up to 75%. The ion chromatogram of the ester product obtained in the catalyst and membrane impregnation was compared with the esterification product of the batch esterification reaction. The gas chromatograph NIST library spectra of the ester product indicated the structure of ethyl lactate (45) on the mass spectra which was in accordance with the commercial ethyl lactate. Products obtained on dowex 50W8x and amberlyst 36 resin catalysts were found to elute faster at 1.503 and 1.527 min respectively in contrast to those using amberlyst 15 and amberlyst 16. In all, the percentage yield of the ethyl lactate can be improved using cellulose acetate membrane. Amberlyst 36 and dowex 50W8x cation-exchange resins were revealed as the most effective catalysts for the esterification process involving lactic and ethanol to produce ethyl lactate in contrast to other cation-exchange resins that were used in the study. The results further confirms effectiveness of cellulose acetate membrane in the selective removal of the water from the esterification product. 相似文献
In this work, we study the split common null point problem in the framework of Banach spaces. We propose an iterative scheme for solving the problem and then prove strong convergence theorem of the sequences generated by our iterative scheme under suitable conditions. We finally provide some numerical examples to support the main theorem. 相似文献
Networks and Spatial Economics - Using the Bregman distance technique, we study the approximation of solution of pseudomonotone equilibrium problem using modified extragradient method in a real... 相似文献
The purpose of this paper is to introduce and study an iterative algorithm for solving a general split equality problem. The problem consists of finding a common element of the set of common zero points for a finite family of maximal monotone operators, the set of common fixed points for a finite family of demimetric mappings and the set of common solutions of variational inequality problems for a finite family of inverse strongly monotone mappings in the setting of infinite-dimensional Hilbert spaces. Using our iterative algorithm, we state and prove a strong convergence theorem for approximating a solution of the split equality problem. As special cases, we shall utilize our results to study the split equality equilibrium problems and the split equality optimization problems. Our result complements and extends some related results in literature. 相似文献