全文获取类型
收费全文 | 563篇 |
免费 | 28篇 |
国内免费 | 4篇 |
专业分类
电工技术 | 35篇 |
综合类 | 8篇 |
化学工业 | 222篇 |
金属工艺 | 20篇 |
机械仪表 | 11篇 |
建筑科学 | 21篇 |
矿业工程 | 1篇 |
能源动力 | 37篇 |
轻工业 | 43篇 |
水利工程 | 1篇 |
无线电 | 31篇 |
一般工业技术 | 103篇 |
冶金工业 | 18篇 |
原子能技术 | 14篇 |
自动化技术 | 30篇 |
出版年
2023年 | 2篇 |
2022年 | 9篇 |
2021年 | 11篇 |
2020年 | 3篇 |
2019年 | 15篇 |
2018年 | 8篇 |
2017年 | 15篇 |
2016年 | 14篇 |
2015年 | 9篇 |
2014年 | 19篇 |
2013年 | 40篇 |
2012年 | 24篇 |
2011年 | 33篇 |
2010年 | 28篇 |
2009年 | 26篇 |
2008年 | 43篇 |
2007年 | 26篇 |
2006年 | 24篇 |
2005年 | 17篇 |
2004年 | 12篇 |
2003年 | 22篇 |
2002年 | 17篇 |
2001年 | 16篇 |
2000年 | 17篇 |
1999年 | 9篇 |
1998年 | 20篇 |
1997年 | 13篇 |
1996年 | 14篇 |
1995年 | 7篇 |
1994年 | 5篇 |
1993年 | 10篇 |
1992年 | 7篇 |
1991年 | 8篇 |
1990年 | 4篇 |
1989年 | 5篇 |
1988年 | 4篇 |
1986年 | 3篇 |
1984年 | 2篇 |
1983年 | 6篇 |
1981年 | 2篇 |
1980年 | 2篇 |
1979年 | 3篇 |
1978年 | 4篇 |
1977年 | 1篇 |
1976年 | 5篇 |
1975年 | 1篇 |
1974年 | 2篇 |
1973年 | 2篇 |
1972年 | 2篇 |
1969年 | 1篇 |
排序方式: 共有595条查询结果,搜索用时 15 毫秒
61.
Hitomi Murakami Gunkichi Sato Shuichi Matsumoto Tatsuhiko Hirabayashi Hideo Yamamoto Wallance W. Donald Erik Bachmann 《International Journal of Satellite Communications and Networking》1986,4(3):127-137
This paper describes field test results of multi-channel digital TV transmission using a PSK/FDMA system and the related subjective test results of received TV pictures. The picture quality of the multi-channel 15 or 30 Mb/s transmission for both NTSC and PAL systems through the INTELSAT POR satellite are subjectively evaluated for various bit-error rates. In addition, subjective evaluations were made at various values of earth-station e.i.r.p. to compare the picture quality of digital transmissions with that of current half-transponder FM transmission. 相似文献
62.
Jian-Yu Zheng Shuichi Noguchi Kenjo Miyauchi Masahiro Hamada Kazushi Kinbara Kazuhiko Saigo 《Fullerenes, Nanotubes and Carbon Nanostructures》2001,9(4):467-475
A series of [60]fullerene bis-adducts having a π-electron-rich aromatic ring as a donor in a face-to-face arrangement were synthesized by the bis-cyclopropanation of [60]fullerene with tether-linked bis-malonates. One of the bis-adducts showed a photoinduced intramolecular electron transfer which caused the dramatic quenching of its fluorescence in a polar solvent. 相似文献
63.
To functionalize the surface of nanoparticles with phenyl groups for subsequent cross-linking with aromatic molecules by mutual interactions, we prepared functional nanoparticles (d = 3 nm) by silanization with phenyl-triethoxysilane. The nanoparticles had Fe(2)O(3) cores conjugated to phenyl groups; this was confirmed by Fourier transform infrared (FT-IR) spectroscopy and absorption spectrophotometry. The typical C-H and C-C peaks and the absorption at 240 nm, which corresponds to aromatic rings, were detected in the spectroscopic results for the phenyl group-modified nanoparticles. The nanoparticles could ionize aromatic (colchicine, reserpine, and bradykinin peptide) and nonaromatic (L-α-phosphatidylethanolamine,dioleoyl, and polyethylene glycol) molecules by nanoparticle-assisted laser desorption/ionization mass spectrometry. The nanoparticles worked as a selective trap and an ionization-assisting reagent in mass spectrometry for the aromatic molecular targets. 相似文献
64.
A Mokashi A Roy C Rozanov S Osanai BT Storey S Lahiri 《Canadian Metallurgical Quarterly》1998,803(1-2):194-197
We measured the effect of high PCO (500-550 Torr) on the pHi and [Ca2+]i in cultured glomus cells of adult rat carotid body (CB) as a test of the two models currently proposed for the mechanism of CB chemoreception. The metabolic model postulates that the rise in glomus cell [Ca2+]i, the initiating reaction in the signalling pathway leading to chemosensory neural discharge, is due to [Ca2+] release from intracellular Ca2+ stores. The membrane potential model postulates that the rise in [Ca2+]i comes from influx of extracellular Ca2+ through voltage-dependent Ca2+ channels (VDCC) of the L-type. High PCO did not change pHi at PO2 of 120-135 Torr, showing that CO-induced changes in [Ca2+]i are not due to changes in pHi. High PCO caused a highly significant rise in [Ca2+]i from 90+/-12 nM to 675+/-65 nM, both in the absence and in the presence of 200 microM CdCl2, a potent blocker of L-type VDCCs. This result is fully consistent with release of Ca2+ from glomus cell intracellular stores according to metabolic model, but inconsistent with influx of extracellular Ca2+ through VDCCs according to the membrane potential model. 相似文献
65.
Variation of Fructooligosaccharides and their Metabolizing Enzymes in Onion Bulb (Allium cepa L. cv. Tenshin) During Long-term Storage 总被引:1,自引:0,他引:1
Noureddine Benkeblia Keiji Ueno Shuichi Onodera Norio Shiomi 《Journal of food science》2005,70(3):S208-S214
ABSTRACT: The objective of this study was to assess the status of fructooligosaccharides (FOS) in onion bulbs ( Allium cepa L. cv. Tenshin) and their metabolizing-enzymes—1-fructoexohydrolase (1-FEH), 1-kestose hydrolyzing enzyme (1-KH), fructan:fructan 1F -fructosyltransferase (1-FFT) and fructan:fructan 6G -fructosyltransferase (6G-FFT)—during storage at 15°C. Fructose varies slightly, whereas 1-kestose peaked after 6 wk and then decreased progressively during the last 18 wk of storage. Lower degree of polymerization (DP) 3 to 6) FOS, higher (DP 7 to 12) FOS, total FOS, and total carbohydrates showed similar and close patterns during 24 wk. They varied slightly at the beginning of the storage period; afterward they decreased progressively and regularly during the last 20 wk of storage. 1-FEH and 1-KH activities were low but peaked abruptly after 12 and 16 wk, respectively, after which they decreased to levels higher (1-FEH) or similar (1-KH) to those observed at the beginning of the storage. Surprisingly, 1-FFT activity showed similar pattern to the variation of 1-KH hydrolyzing activity; on the other hand, 6G-FFT, although higher, was stable during 16 wk but decreased after that. The results allowed us to associate FOS to the dormancy and sprouting states, and the peaks of the degrading enzymes were shown to signal the release of dormancy of onion bulb. 相似文献
66.
We examined the synthesis, transport, and localization of surfactant protein A (SP-A) in primary cultures of alveolar type II cells. In type II cells maintained in culture for 6 h, 39% of the SP-A pool detected with an enzyme-linked immunosorbent assay (ELISA) was found in lamellar bodies (LBs). After 24 h in culture, 53% of the cellular SP-A pool was found in LBs. The absolute amount of SP-A in the LB compartment was almost identical at 6 and 24 h of culture. In contrast to the results obtained with ELISA, 35S labeling of newly synthesized SP-A revealed that less than 7% of the cellular SP-A pool was in LBs at either 6 or 24 h of culture. In the 6-h cultures, 17% of the total (i.e., cells and media) [35S]SP-A pool was extracellular. In the 24-h cultures, 70% of the [35S]SP-A pool was extracellular. The secretion of [35S]SP-A was blocked by brefeldin A at all times. When medium containing newly secreted [35S]SP-A was incubated with alveolar type II cells maintained in culture for 24 h, the protein was taken up and incorporated into the LB fraction. More than 80% of the internalized SP-A was associated with the LB compartment after a 6 h incubation. The uptake of [35S]SP-A was blocked at 4 degrees C and was promoted by addition of unlabeled SP-A at 37 degrees C. These findings support a pathway of extracellular routing of SP-A prior to its accumulation in LBs in cultured type II cells. 相似文献
67.
Takayuki Tomaru Shinji Miyoki Masatake Ohashi Kazuaki Kuroda Takashi Uchiyama Toshikazu Suzuki Akira Yamamoto Takakazu Shintomi Akitoshi Ueda Daisuke Tatsumi Shuichi Sato Koji Arai Masaki Ando Koji Watanabe Kenji Nakamura Masahiko Watanabe Kazuhiko Ito Izumi Kataoka Hiroaki Yamamoto Brett Bochner Yaron Hefetz 《Applied optics》2003,42(7):1306-1307
68.
Takashi Hirano Yuiko Kazahaya Akio Nakamura Toshihiro Miyao Shuichi Naito 《Catalysis Letters》2007,117(1-2):73-78
The effect of addition of In and Pb on the reduction of N2O by CO was studied over SiO2 supported Pd catalysts, using a closed gas circulation system as well as in-situ infrared spectroscopy. Formation of intermetallic
compounds such as Pd0.48In0.52, Pd3Pb and Pd3Pb2 was observed which caused a drastic enhancement of the rate of N2 formation. The infrared spectroscopic analyses revealed a weakening of the adsorption strength of CO on Pd metal by the formation
of intermetallic compounds, which is likely the main reason for the enhancement of the reaction rate. From a kinetic investigation
as well as in situ FT-IR observation during the N2O-CO reaction, a redox mechanism was proposed involving the oxidation of the surface by N2O followed by its reduction by CO. Over Pd/SiO2, the former process seems to be the rate limiting step because of the inhibition of N2O activation by strongly adsorbed CO. By adding In or Pb, the rate limiting step shifted to the latter process, which resulted
in a large enhancement in the rate of N2 formation. 相似文献
69.
Takao Yamamoto Shuichi Okuda Masatoshi Fujishiro 《Journal of Nuclear Materials》1988,160(2-3):247-252
A thin titanium layer with uniformly absorbed tritium (T/Ti ˜1.0) was bombarded by 390 keV D3+ ions (130 keV per deuteron). Bombardment was performed at low (111 K) and room temperatures up to fluences of 5.9 × 1018 D/cm2 and 3.0 × 1018 D/cm2, respectively. Depth profiles of tritium up to a depth of 0.8 mg/cm2 (˜1.8 μm) were measured and the change of the profile with fluence was investigated by means of the T(d, )n nuclear reaction. At both of the temperatures, a dip was formed on the depth profile of tritium at the depth around the projected range, indicating that the deuteron bombardment induced the migration of tritium against the concentration gradient. At the low temperature, the dip showed a gradual growth with fluence and saturation of the growth at the higher fluences, which could not be described by the existing model for isotope mixing. The spectrum of protons from the D(d, p)T reaction obtained in the same measurement suggested that the release of deuterium suddenly started at the final stage of the present bombardment. The dip formed at room temperature was larger than that at the low temperature. The migration of tritium induced by the bombardment is discussed on the basis of the experimental results obtained. 相似文献
70.
Shunichi Hasegawa Takahiro Nishiwaki Hitoe Habuchi Shoji Nitta Shuichi Nonomura 《Fullerenes, Nanotubes and Carbon Nanostructures》1995,3(2):163-178
CPM spectra of the fullerene film was measured to obtain the below gap absorption. The optical energy gap Eo was obtained by using the Tauc's plots. Eo did not change so much with the intercalated impurities. The absorption due to intercalated impurities was found below 1.6eV. 相似文献