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Xiaofan Wang Keisuke Shinokita Hong En Lim Nur Baizura Mohamed Yuhei Miyauchi Nguyen Thanh Cuong Susumu Okada Kazunari Matsuda 《Advanced functional materials》2019,29(6)
Atomically thin‐layered ReS2 with a distorted 1T structure has attracted attention because of its intriguing optical and electronic properties. Here, the direct and indirect exciton dynamics of a three‐layered ReS2 is investigated by polarization‐resolved transient photoluminescence (PL) and ultrafast pump‐probe spectroscopy. The various time scales of the decay signals of the time‐resolved PL (<10 ps), with monitoring of the populations of electron–hole pairs (exciton), and the transient differential reflectance (≈1 and 100 ps), with monitoring of the populations of electrons and/or holes in the excited states, are observed. These results reveal the characteristic exciton dynamics: rapid relaxation of direct excitons (electron–hole pairs) and slow relaxation of the momentum‐mismatched indirect excitons accompanied by a one‐phonon emission process. These findings provide important information regarding the indirect bandgap nature of few‐layered ReS2 and its characteristic exciton dynamics, boosting the understanding of the novel electronic and optical properties of atomically thin‐layered ReS2. 相似文献
53.
跨技术通信迅猛发展推动着单一网络向异构无线网络的转变,该转变极大地提高异构无线设备(如Wi-Fi和ZigBee)的高效共存和协作,但也给异构无线网络中的数据分发问题带来了挑战.由于异构网络节点通信范围差异和低占空比节点周期性睡眠的特点,传统数据分发方法不能高效地利用信道资源而导致较低的分发效率.为了解决这些问题,该文提出一种适用于异构网络的并行数据分发方法.通过数据分发时延和能耗定义新的系统损失函数,并证明了损失函数的合理性,利用信标控制的延迟接收数据包的分发策略,从而实现对周期性睡眠的ZigBee网络进行高效数据分发.进一步地,该文根据动态规划的思想,推导出系统的整体能量损耗和时延的最优值.通过仿真实验证明,在考虑时延和能量损耗的前提下,该文的数据分发方法的性能优于传统的数据分发方法. 相似文献
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An optical interference method was used to display the distorted film shape in nominally parallel surface thrust washers. The bearings were made of aluminium to accentuate thermal expansion and were carefully lapped flat before use. Both the experimental results and an analysis of the coupled elasticity, Reynolds and energy equations confirm that these bearings operate by the formation of a slightly converging film over the leading 80 percent (or less) of the pad. Fair agreement was obtained between the analysis and previously developed multiple regression equations. Thrust washers for industrial use with random waviness are likely lo perform better than lapped bearings. 相似文献
57.
The authors propose a new design concept for controlling the deflection of a micro-membrane with the aid of its thickness distribution for realizing a prescribed design in the MEMS. As an example, the authors treat a micro air pump that comprises a micro-membrane. The membrane is actuated by an electrostatic force. The membrane deflects and thus the deflection is influenced by the air pressure and the electrostatic field. This is a highly complicated system. To find out a proper thickness distribution, the authors use the genetic algorithm that is appropriate to reduce the searching space of solution. 相似文献
58.
Nora MartinezKenji Hisada Isao TabataKazumasa Hirogaki Susumu YonezawaTeruo Hori 《The Journal of Supercritical Fluids》2011,56(3):322-329
The effect of thermal treatment to improve the metal adhesion into poly-(p-phenylene terephthalamide) (PPTA), e.g. aramid fiber, has been investigated. After palladium(II)-hexafluoroacetylacetonate metal complex, Pd(hfac)2, seeding into the fiber using supercritical fluid carbon dioxide, scCO2, a post-thermal treatment was conducted. As a result, after carrying out electroless copper plating, the adhesive strength between polymer substrate and copper layer greatly increased. Also, in order to have a better comprehension on decomposition reactions of Pd(hfac)2 under supercritical conditions, remains of metal complex were analyzed using electron ionization mass spectrometry technique (EI-MS). EI-MS mass spectra derived from Pd(hfac)2 gave us useful information about its dissociation reactions and reaction temperature under supercritical conditions. Additionally, to verify the Pd particles seeding in the fiber surface, X-ray photoelectron spectrometry (XPS) analyses were performed. The results confirmed that post-thermal treatment induced Pd particles diffusion and deeper penetration of Pd complex and its fragments into the fiber. 相似文献
59.
Zhi-xue Tian Akifumi Uozumi Ikutaro Hamada Susumu Yanagisawa Hidetoshi Kizaki Kouji Inagaki Yoshitada Morikawa 《Nanoscale research letters》2013,8(1):203
First-principles calculations were performed to investigate the effect of Pd concentration and oxygen vacancies on the stability of Pd at LaFeO3 surfaces. We found a much stronger tendency of Pd to segregate by taking the aggregation of Pd at LaFe1-xPdxO3-y surfaces into consideration, resulting in a pair of Pd-Pd around a vacancy. Moreover, we predicted that one oxygen-vacancy-containing FeO2-terminated surfaces would be stable at high temperatures by comparing the stability of LaFe1-xPdxO3-y surfaces, which further supports our previous conclusion that a Pd-containing perovskite catalyst should be calcined at 1,073 K or higher temperatures in air to enhance the segregation of Pd in the vicinity of surfaces to rapidly transform the Pd catalyst from oxidized to reduced states on the perovskite support. 相似文献
60.
Some approximate indexing schemes have been recently proposed in metric spaces which sort the objects in the database according to pseudo-scores. It is known that (1) some of them provide a very good trade-off between response time and accuracy, and (2) probability-based pseudo-scores can provide an optimal trade-off in range queries if the probabilities are correctly estimated. Based on these facts, we propose a probabilistic enhancement scheme which can be applied to any pseudo-score based scheme. Our scheme computes probability-based pseudo-scores using pseudo-scores obtained from a pseudo-score based scheme. In order to estimate the probability-based pseudo-scores, we use the object-specific parameters in logistic regression and learn the parameters using MAP (Maximum a Posteriori) estimation and the empirical Bayes method. We also propose a technique which speeds up learning the parameters using pseudo-scores. We applied our scheme to the two state-of-the-art schemes: the standard pivot-based scheme and the permutation-based scheme, and evaluated them using various kinds of datasets from the Metric Space Library. The results showed that our scheme outperformed the conventional schemes, with regard to both the number of distance computations and the CPU time, in all the datasets. 相似文献