全文获取类型
收费全文 | 7369篇 |
免费 | 755篇 |
国内免费 | 17篇 |
专业分类
电工技术 | 101篇 |
综合类 | 14篇 |
化学工业 | 1855篇 |
金属工艺 | 264篇 |
机械仪表 | 500篇 |
建筑科学 | 131篇 |
矿业工程 | 4篇 |
能源动力 | 347篇 |
轻工业 | 684篇 |
水利工程 | 15篇 |
石油天然气 | 1篇 |
无线电 | 1424篇 |
一般工业技术 | 1767篇 |
冶金工业 | 200篇 |
原子能技术 | 123篇 |
自动化技术 | 711篇 |
出版年
2024年 | 14篇 |
2023年 | 122篇 |
2022年 | 158篇 |
2021年 | 299篇 |
2020年 | 236篇 |
2019年 | 250篇 |
2018年 | 314篇 |
2017年 | 301篇 |
2016年 | 376篇 |
2015年 | 310篇 |
2014年 | 413篇 |
2013年 | 537篇 |
2012年 | 537篇 |
2011年 | 668篇 |
2010年 | 502篇 |
2009年 | 537篇 |
2008年 | 416篇 |
2007年 | 279篇 |
2006年 | 282篇 |
2005年 | 224篇 |
2004年 | 224篇 |
2003年 | 194篇 |
2002年 | 176篇 |
2001年 | 107篇 |
2000年 | 106篇 |
1999年 | 109篇 |
1998年 | 107篇 |
1997年 | 74篇 |
1996年 | 64篇 |
1995年 | 56篇 |
1994年 | 29篇 |
1993年 | 13篇 |
1992年 | 26篇 |
1991年 | 15篇 |
1990年 | 16篇 |
1989年 | 10篇 |
1988年 | 9篇 |
1987年 | 10篇 |
1986年 | 3篇 |
1985年 | 6篇 |
1984年 | 2篇 |
1983年 | 1篇 |
1981年 | 2篇 |
1980年 | 3篇 |
1979年 | 1篇 |
1976年 | 1篇 |
1975年 | 1篇 |
1974年 | 1篇 |
排序方式: 共有8141条查询结果,搜索用时 15 毫秒
71.
Flexible heaters were prepared by extruding platinum‐catalyzed silicone rubber composites with conductive carbon black (CB) and metallic fillers. The conductor resistivity of the extruded heaters decreased in order of conductive titanium dioxide (TiO2) > aluminum powder ≈ zinc powder > copper powder. Thermoelectric switching phenomena were investigated for the silicone rubber/CB/metallic powder systems. The positive temperature coefficient effect was dependent mainly on the CB content rather than on the content of the metallic powders. Resistivity and thermal reproducibility of the extruded heaters were also investigated by periodically applying AC voltage of 110 V. The heaters containing copper and TiO2 powders exhibited excellent electrical reproducibility. © 2005 Wiley Periodicals, Inc. J Appl Polym Sci 95: 1122–1128, 2005 相似文献
72.
The High-Performance Computing (HPC) is an infrastructure to support various research fields. The research using HPC requires big storage for large-scale of raw data and the huge computing resources to analyze. The consolidated operations of the computing center for supporting various researches using HPC are a very effective organization. The consolidated operations are able to increase the utilization. The computing center has to be re-organized continuously in order to support the various fields of research effectively and flexibly. Re-organization to reuse the limited resources enforces the update of the information for verification of the computing resources after the re-allocation of computing resources and the re-distribution of trusted connection between computing resources. Consequently, to maintain effective research support we need automated resource re-organization environment. In this paper, we build an automated update of the trusted connection for re-organized computing resource using puppet which is automated system management platform. Finally, we provide a unified verification point and efficient environment for the re-allocation and re-organization of the integrated computing center. 相似文献
73.
Fault identification for process monitoring using kernel principal component analysis 总被引:2,自引:0,他引:2
In this research, we develop a new fault identification method for kernel principal component analysis (kernel PCA). Although it has been proved that kernel PCA is superior to linear PCA for fault detection, the fault identification method theoretically derived from the kernel PCA has not been found anywhere. Using the gradient of kernel function, we define two new statistics which represent the contribution of each variable to the monitoring statistics, Hotelling's T2and squared prediction error (SPE) of kernel PCA, respectively. The proposed statistics which have similar concept to contributions in linear PCA are directly derived from the mathematical formulation of kernel PCA and thus they are straightforward to understand. The main contribution of this work is that we firstly suggest a fault identification method especially applicable to process monitoring using kernel PCA. To demonstrate the performance, the proposed method is applied to two simulated processes, one is a simple nonlinear process and the other is a non-isothermal CSTR process. The simulation results show that the proposed method effectively identifies the source of various types of faults. 相似文献
74.
Poly(trimethylene terephthalate) (PTT) nano composites were synthesized by in situ polymerization at high temperature with two thermally stable organoclays: 1,2‐dimethylhexadecylimidazolium‐montmorillonite (IMD‐MMT) and dodecyltriphenyl phosphonium‐MMT (C12PPh‐MMT). PTT hybrid fibers with various organoclay contents were melt‐spun at various draw ratios (DRs) to produce monofilaments. The thermomechanical properties and morphologies of the PTT hybrid fibers were characterized using differential scanning calorimetry, thermogravimetric analysis, wide‐angle X‐ray diffraction, electron microscopy, and mechanical tensile properties analysis. The nanostructure of the hybrid fibers was observed by both scanning and transmission electron microscopy, which showed that the clay layers were well dispersed into the matrix polymer, although some clusters or agglomerated particles were also detected. Unlike the hybrids containing IMD‐MMT, the clay layers of the C12PPh‐MMT hybrid fiber were more dispersed into the matrix polymer. The thermal stability and tensile properties of the hybrid fibers increased with increasing clay content for DR = 1. However, as DR increased from 1 to 9 the ultimate strength and initial modulus of the hybrid fibers with IMD‐MMT increased slightly whereas those of C12PPh‐MMT hybrid fibers decreased slightly. © 2006 Wiley Periodicals, Inc. J Appl Polym Sci 102: 4535–4545, 2006 相似文献
75.
The important mechanical mechanism for the electrical conduction of anisotropic conductive films (ACFs) is the joint clamping force after the curing and cooling processes of ACFs. In this study, the mechanism of shrinkage and contraction stress and the relationship between these mechanisms and the thermomechanical properties of ACFs were investigated in detail. Both thickness shrinkages and modulus changes of four kinds of ACFs with different thermomechanical properties were experimentally investigated with thermomechanical and dynamic mechanical analysis. Based on the incremental approach to linear elasticity, contraction stresses of ACFs developed along the thickness direction were estimated. Contraction stresses in ACFs were found to be significantly developed by the cooling process from the glass‐transition temperature to room temperature. Moreover, electrical characteristics of ACF contact during the cooling process indicate that the electrical conduction of ACF joint is robustly maintained by substantial contraction stress below Tg. The increasing rate of contraction stresses below Tg was strongly dependent on both thermal expansion coefficient (CTE) and elastic modulus (E) of ACFs. A linear relationship between the experimental increasing rate and E × CTE reveals that the build‐up behavior of contraction stress is closely correlated with the ACF material properties: thermal expansion coefficient, glassy modulus, and Tg. © 2004 Wiley Periodicals, Inc. J Appl Polym Sci 93: 2634–2641, 2004 相似文献
76.
Jong-Ho Ryu Jong Hyun Seo Jae-Han Jeong Sung-Kap Kim Dong Nyung Lee 《Journal of Applied Electrochemistry》2004,34(9):879-884
A study has been made of the electrochemical etching of 99.99% aluminum foils at a current density of 50 mA cm–2in AlCl3–HCl solutions (1 m Cl–) at 80 °C. The solutions were made by dissolving metallic aluminum into 1m HCl solution, to give a Cl– concentration of 1 m. The number density of etch tunnels and the homogeneity of tunnel length decreased, and the mean pit size and its standard deviation increased with increasing Al3+ concentration. The results were discussed based on potential transients at a current density of 50 mA cm–2, current–potential curves at a scan rate of 10 m Vs–1 and electrochemical impedance spectra. 相似文献
77.
Seong‐Ho Choi Min‐Seok Kim Jae Jeong Ryoo Kwang‐Pill Lee Hyun‐Dong Shin Sun‐Hwa Kim Yong‐Hyun Lee 《应用聚合物科学杂志》2002,85(11):2451-2457
Carboxylic acid groups were introduced onto polyethylene (PE) film by radiation‐induced graft copolymerization. Subsequently, the clodextrin glucanotransferase (CGTase) was immobilized on the PE film with a carboxylic acid group. The activity of the immobilized CGTase on PE film was in the range of 0.40–1.04 U/cm2 per min. The production of cyclodextrins (CDs) from corn starch was examined using the CGTase‐immobilized PE film. The production ratios of CDs using CGTase‐immobilized PE film was in the following order: α–CD > β–CD > γ–CD. © 2002 Wiley Periodicals, Inc. J Appl Polym Sci 85: 2451–2457, 2002 相似文献
78.
A D-Phenylalanine (Phe) imprinted terpolymer, Polyacrylonitrile-Poly(acrylic acid)-Poly(acryl amide) (Poly(AN-AA-AAm)) bead
was prepared by the wet-phase inversion method. Acrylamide (AAm) and acrylic acid (AA) were used as the functional monomer
and acrylonitrile (AN) was used as a physical cross linker. The characteristics of selective adsorption by the D-Phe imprinted
terpolymer beads were investigated at high concentrations of Phe racemate solution, 1 g Phe/L, and 10 g Phe/L. The adsorption
selectivity of the D-Phe imprinted terpolymer beads prepared by anin-situ implanting method reached 0.82 and 0.8 at 1.0 g and 10 g Phe/L racemate solution, respectively, and almost all of the adsorbed
D-Phe and about 43% of the adsorbed L-Phe were desorbed by 4% acetic acid. The uptake capacities of the terpolymer beads were
maintained for several repeated batches. 相似文献
79.
Neung‐Ju Lee Ja‐Chul Koo Sung‐Suk Ju Seong‐Bae Moon Won‐Jei Cho In‐Cheol Jeong Song‐Jae Lee Moo‐Youn Cho Emmanuel A Theodorakis 《Polymer International》2002,51(7):569-576
The attachment of anticancer agents to polymers is a promising approach towards reducing the toxic side‐effects and retaining the potent antitumour activity of these agents. A new tetrahydrophthalimido monomer containing 5‐fluorouracil (ETPFU) and its homopolymer and copolymers with acrylic acid (AA) and with vinyl acetate (VAc) have been synthesized and spectroscopically characterized. The ETPFU contents in poly(ETPFU‐co‐AA) and poly(ETPFU‐co‐VAc) obtained by elemental analysis were 21 mol% and 20 mol%, respectively. The average molecular weights of the polymers determined by gel permeation chromatography were as follows: Mn = 8900 g mol?1, Mw = 13 300 g mol?1, Mw/Mn = 1.5 for poly(ETPFU); Mn = 13 500 g mol?1, Mw = 16 600 g mol?1, Mw/Mn = 1.2 for poly(ETPFU‐co‐AA); Mn = 8300 g mol?1, Mw = 11 600 g mol?1, Mw/Mn = 1.4 poly(ETPFU‐co‐VAc). The in vitro cytotoxicity of the compounds against FM3A and U937 cancer cell lines increased in the following order: ETPFU > 5‐FU > poly(ETPFU) > poly(ETPFU‐co‐AA) > poly(ETPFU‐co‐VAc). The in vivo antitumour activities of all the polymers in Balb/C mice bearing the sarcoma 180 tumour cell line were greater than those of 5‐FU and monomer at the highest dose (800 mg kg?1). © 2002 Society of Chemical Industry 相似文献
80.
Multifunctional monomers, m‐xylylenedimaleimide, p‐phenylenedimaleimide, m‐phenylenedimaleimide, and p‐phenylenedinadimide, all of which have maleimide groups, were synthesized to increase thermal and radiation stabilities. The synthesized multifunctional monomers showed good compatibility with low‐density polyethylene (LDPE). Mixtures of LDPE and these multifunctional monomers were irradiated with γ‐rays from a Co‐60 source at room temperature in a nitrogen atmosphere. The absorbed dose ranged from 0 to 160 KGy. Among these multifunctional monomers, m‐xylylenedimaleimide was the best in gel fraction enhancement. Crosslinked LDPE with m‐xylylenedimaleimide displayed a higher modulus than that of crosslinked LDPE with triallyl cyanurate. For the elongation property, LDPE with m‐xylylenedimaleimide as a multifunctional monomer showed better results than that with commercial multifunctional monomers such as triallyl cyanurate (TAC) and trimethylol propane triacrylate (TMPTA). © 2003 Wiley Periodicals, Inc. J Appl Polym Sci 88: 2339–2345, 2003 相似文献