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111.
Eric R. MacamAuthor VitaeBryan M. BlackburnAuthor Vitae Eric D. WachsmanAuthor Vitae 《Sensors and actuators. B, Chemical》2011,158(1):304-312
The intent of this work is to look at the effects of varying the La2CuO4 electrode area and the asymmetry between the sensing and counter electrode in a solid state potentiometric sensor with respect to NOx sensitivity. NO2 sensitivity was observed at 500-600 °C with a maximum sensitivity of ∼22 mV/decade [NO2] observed at 500 °C for the sensor with a La2CuO4 electrode area of ∼30 mm2. The relationship between NO2 sensitivity and area is nearly parabolic at 500 °C, decreases linearly with increasing electrode area at 600 °C, and was a mixture of parabolic and linear behavior 550 °C. NO sensitivity varied non-linearly with electrode area with a minima (maximum sensitivity) of ∼−22 mV/decade [NO] at 450 °C for the sensor with a La2CuO4 electrode area of 16 mm2. The behavior at 400 °C was similar to that of 450 °C, but with smaller sensitivities due to a saturation effect. At 500 °C, NO sensitivity decreases linearly with area.We also used electrochemical impedance spectroscopy (EIS) to investigate the electrochemical processes that are affected when the sensing electrode area is changed. Changes in impedance with exposure to NOx were attributed to either changes in La2CuO4 conductivity due to gas adsorption (high frequency impedance) or electrocatalysis occurring at the electrode/electrolyte interface (total electrode impedance). NO2 caused a decrease in high frequency impedance while NO caused an increase. In contrast, NO2 and NO both caused a decrease in the total electrode impedance. The effect of area on both the potentiometric and impedance responses show relationships that can be explained through the mechanistic contributions included in differential electrode equilibria. 相似文献
112.
Valérie Duplan Eric Frost Jan J. DubowskiAuthor vitae 《Sensors and actuators. B, Chemical》2011,160(1):46
This work describes a novel method of detecting Escherichia coli using photoluminescence (PL) emission from III–V quantum semiconductor (QS) devices functionalized with two different antibody-based architectures. The first approach employed self-assembled monolayers of biotinylated polyethylene glycol thiols to immobilize biotinylated antibody via neutravidin. In the second approach, we used QS microstructures coated with a thin layer of Si3N4 allowing direct functionalization with E. coli antibodies through hydrofluoric acid etching and glutaraldehyde-based reticulation. Atomic force, optical and fluorescence microscopy measurements were used to assess the immobilization process. Depending on the biosensing architecture, density of the immobilized bacteria was observed in the range of 0.5–0.7 bacteria/100 μm2. The detection of E. coli at 104 CFU/ml was achieved within less than 120 min of the bacteria exposure. It is expected that an even better sensitivity threshold could be achieved following further optimization of the method. 相似文献
113.
We present an integral feedback controller that regulates the average copy number of an assembly in a system of stochastically
interacting robots. The mathematical model for these robots is a tunable reaction network, which makes this approach applicable to a large class of other systems, including ones that exhibit stochastic self-assembly
at various length scales. We prove that this controller works for a range of setpoints and how to compute this range both
analytically and experimentally. Finally, we demonstrate these ideas on a physical testbed. 相似文献
114.
Most studies on the role of IT for economic exchange predicted that under a given set of exchange attributes buyers would choose a certain mode of relationship with suppliers. Our study of an online IT services marketplace revealed that buyers do not have a single, uniformly preferred type of relationship, but rather maintain a portfolio of relationships. Furthermore, different buyers arrange their portfolios of exchange relationships in different ways. We found four clusters of buyers' portfolios of relationships labeled Transactional buyers, Recurrent buyers, Small diversifiers and Large diversifiers, that differ in their usage of auction or negotiation mechanism, their supplier relations as well as their usage of preferred suppliers. Our results thus paint a richer picture of how buyers organize their supplier networks online. 相似文献
115.
116.
In this work, we describe an autonomous mobile robotic system for finding, investigating, and modeling ambient noise sources
in the environment. The system has been fully implemented in two different environments, using two different robotic platforms
and a variety of sound source types. Making use of a two-step approach to autonomous exploration of the auditory scene, the
robot first quickly moves through the environment to find and roughly localize unknown sound sources using the auditory evidence
grid algorithm. Then, using the knowledge gained from the initial exploration, the robot investigates each source in more
depth, improving upon the initial localization accuracy, identifying volume and directivity, and, finally, building a classification
vector useful for detecting the sound source in the future. 相似文献
117.
118.
Ahmed Samet Eric Lefèvre Sadok Ben Yahia 《Journal of Intelligent Information Systems》2016,47(1):135-163
Associative classification has been shown to provide interesting results whenever of use to classify data. With the increasing complexity of new databases, retrieving valuable information and classifying incoming data is becoming a thriving and compelling issue. The evidential database is a new type of database that represents imprecision and uncertainty. In this respect, extracting pertinent information such as frequent patterns and association rules is of paramount importance task. In this work, we tackle the problem of pertinent information extraction from an evidential database. A new data mining approach, denoted EDMA, is introduced that extracts frequent patterns overcoming the limits of pioneering works of the literature. A new classifier based on evidential association rules is thus introduced. The obtained association rules, as well as their respective confidence values, are studied and weighted with respect to their relevance. The proposed methods are thoroughly experimented on several synthetic evidential databases and showed performance improvement. 相似文献
119.
120.
Eric Pedrol Javier Martínez Magdalena Aguiló Manuel Garcia-Algar Moritz Nazarenus Luca Guerrini Eduardo Garcia-Rico Francesc Díaz Jaume Massons 《Microfluidics and nanofluidics》2017,21(12):181
This paper presents an optofluidic device for cell discrimination with two independent interrogation regions. Pumping light is coupled to the device, and cell fluorescence is extracted from the two interrogation zones by using optical fibers embedded in the optofluidic chip. To test the reliability of this device, AU-565 cells—expressing EpCAM and HER2 receptors—and RAMOS cells were mixed in a controlled manner, confined inside a hydrodynamic focused flow in the microfluidic chip and detected individually so that they could be discriminated as positive (signal reception from fluorescently labeled antibodies from the AU-565 cells) or negative events (RAMOS cells). A correlation analysis of the two signals reduces the influence of noise on the overall data. 相似文献