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Silvia Gazzin Matteo Dal Ben Michele Montrone Sri Jayanti Andrea Lorenzon Alessandra Bramante Cristina Bottin Rita Moretti Claudio Tiribelli 《International journal of molecular sciences》2021,22(1)
Bilirubin toxicity to the central nervous system (CNS) is responsible for severe and permanent neurologic damage, resulting in hearing loss, cognitive, and movement impairment. Timely and effective management of severe neonatal hyperbilirubinemia by phototherapy or exchange transfusion is crucial for avoiding permanent neurological consequences, but these therapies are not always possible, particularly in low-income countries. To explore alternative options, we investigated a pharmaceutical approach focused on protecting the CNS from pigment toxicity, independently from serum bilirubin level. To this goal, we tested the ability of curcumin, a nutraceutical already used with relevant results in animal models as well as in clinics in other diseases, in the Gunn rat, the spontaneous model of neonatal hyperbilirubinemia. Curcumin treatment fully abolished the landmark cerebellar hypoplasia of Gunn rat, restoring the histological features, and reverting the behavioral abnormalities present in the hyperbilirubinemic rat. The protection was mediated by a multi-target action on the main bilirubin-induced pathological mechanism ongoing CNS damage (inflammation, redox imbalance, and glutamate neurotoxicity). If confirmed by independent studies, the result suggests the potential of curcumin as an alternative/complementary approach to bilirubin-induced brain damage in the clinical scenario. 相似文献
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Silicon - This paper presents recent progress in computational modeling on blend morphology of silicon nanowires (SiNWs) dispersed in a conjugated polymer poly(3-hexylthiophene) P3HT hybrid solar... 相似文献
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Faraz Montazersadgh Hao Zhang Anas Alkayal Benjamin Buckley Ben W.Kolosz Bing Xu Jin Xuan 《Frontiers of Chemical Science and Engineering》2021,15(1):208-219
Utilizing CO2 in an electro-chemical process and synthesizing value-added chemicals are amongst the few viable and scalable pathways in carbon capture and utilization technologies.CO2 electro-reduction is also counted as one of the main options entailing less fossil fuel consumption and as a future electrical energy storage strategy.The current study aims at developing a new electrochemical platform to produce low-carbon e-biofuel through multifunctional electrosynthesis and integrated co-valorisation of biomass feedstocks with captured CO2.In this approach,CO2 is reduced at the cathode to produce drop-in fuels(e.g.,methanol)while value-added chemicals(e.g.,selective oxidation of alcohols,aldehydes,carboxylic acids and amines/amides)are produced at the anode.In this work,a numerical model of a continuous-flow design considering various anodic and cathodic reactions was built to determine the most techno-economically feasible configurations from the aspects of energy efficiency,environment impact and economical values.The reactor design was then optimized via parametric analysis. 相似文献
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Mansour N. Ben Djeridi W. Mir L. El 《Journal of Inorganic and Organometallic Polymers and Materials》2021,31(11):4360-4371
Journal of Inorganic and Organometallic Polymers and Materials - Nanoporous carbon matrix was prepared by the sol–gel process from pyrogallol-formaldehyde (PF) mixtures in water using picric... 相似文献
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The molecular orientation at the outer surface of injection–stretch–blow‐molded bottles made from poly(ethylene terephthalate) was characterized and quantified by means of front‐surface reflection infrared spectroscopy based on a method developed previously. Results were obtained for two different bottle shapes (cylindrical and rectangular) molded at different injection mold temperatures (16, 38, and 60°C). For the cylindrical bottles, the preferred molecular chain orientation was found to be in the axial direction, with the Hermans orientation function near 0.3 for all three mold temperatures. For the less symmetrical rectangular bottles, a significant difference was observed between the large and small faces. For the large face, the orientation was mainly in the hoop direction; the Hermans orientation function was in the range of 0.3–0.5 and was essentially the same at all mold temperatures and positions along the bottle height. For the small face, on the other hand, the preferred orientation changed from the hoop direction near the bottom to the axial direction near the top, and the variation was more pronounced at lower mold temperatures. The utility of the front‐surface reflection technique was clearly demonstrated. It was also applied, with the use of an infrared microscope, to examine the orientation gradient across the wall thickness. © 2007 Wiley Periodicals, Inc. J Appl Polym Sci 104: 1319–1327, 2007 相似文献
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对反应器网络综合问题进行了研究,分析了瞬时选择性对关键组份组成的偏导数与最佳反应器类型之间的关系,给出了确定最优反应器的三条规则。对δS/δC符号不变的反应体系,用这些规则可获得最优反应器网络。对一般的反应体系,假设了五种典型S-CA曲线所对应的反应过程,分别对不同曲线类型给出了确定最优反应器网络的方法。此外,按本文方法所得的最优反应器网络结构是一个CSTR或PFR或由CSTR、PFR组成的串联结构。由dS/dCA的符号及其变化情况决定。给出了两个说明本文方法的例子,结果表明本文方法简单并可获得与文献相同或相似的结果。 相似文献
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High molecular weight polyacetylenes bearing nonlinear chromophoric pendants poly[4-ethynyl-4′-(N,N-diethylamino)azobenzene-co-phenylacetylene]s [poly(EAAB-co-PA)s] were synthesized in moderate yields by [Rh(nbd)Cl]2-Et3N. The azo unit in the copolymers can be effectively controlled by the monomer feed ratio. Whereas the homopolymer of EAAB possessed low solubility, all the copolymers, however, dissolved readily in common organic solvents when the poly(EAAB) molar content was less than 41.7%. The structures and properties of the polymers were characterized and evaluated by UV, NMR, optical limiting, and nonlinear optical analyses. All the copolymers possessed high stereoregularity and thermal stability (≥300 °C). They can attenuate intense laser pulses, with solutions of high concentrations showing better performances. The third-order nonlinear susceptibility of the copolymers was as high as 4.62×10−11 esu, which are two orders of magnitude larger than those of poly(PA), and larger than that of poly(N-carbazoylacetylene), and poly(1-naphthylacetylene). 相似文献