全文获取类型
收费全文 | 805篇 |
免费 | 26篇 |
国内免费 | 2篇 |
专业分类
电工技术 | 33篇 |
综合类 | 1篇 |
化学工业 | 328篇 |
金属工艺 | 20篇 |
机械仪表 | 10篇 |
建筑科学 | 29篇 |
能源动力 | 42篇 |
轻工业 | 66篇 |
水利工程 | 1篇 |
无线电 | 25篇 |
一般工业技术 | 158篇 |
冶金工业 | 27篇 |
原子能技术 | 19篇 |
自动化技术 | 74篇 |
出版年
2023年 | 8篇 |
2022年 | 11篇 |
2021年 | 16篇 |
2020年 | 14篇 |
2019年 | 18篇 |
2018年 | 11篇 |
2017年 | 15篇 |
2016年 | 28篇 |
2015年 | 7篇 |
2014年 | 17篇 |
2013年 | 43篇 |
2012年 | 31篇 |
2011年 | 54篇 |
2010年 | 32篇 |
2009年 | 44篇 |
2008年 | 42篇 |
2007年 | 38篇 |
2006年 | 40篇 |
2005年 | 27篇 |
2004年 | 25篇 |
2003年 | 34篇 |
2002年 | 26篇 |
2001年 | 12篇 |
2000年 | 21篇 |
1999年 | 19篇 |
1998年 | 13篇 |
1997年 | 14篇 |
1996年 | 14篇 |
1995年 | 20篇 |
1994年 | 14篇 |
1993年 | 7篇 |
1992年 | 9篇 |
1991年 | 7篇 |
1990年 | 9篇 |
1989年 | 8篇 |
1988年 | 11篇 |
1987年 | 11篇 |
1986年 | 10篇 |
1985年 | 5篇 |
1984年 | 3篇 |
1983年 | 5篇 |
1981年 | 5篇 |
1980年 | 6篇 |
1979年 | 3篇 |
1978年 | 2篇 |
1977年 | 10篇 |
1976年 | 3篇 |
1975年 | 4篇 |
1974年 | 3篇 |
1973年 | 2篇 |
排序方式: 共有833条查询结果,搜索用时 406 毫秒
121.
Sayaka Yanagida Akira Nakajima Takayoshi Sasaki Toshihiro Isobe Yoshikazu Kameshima Kiyoshi Okada 《Applied Catalysis A: General》2009,366(1):130
Keggin ions (PW12O403− (PW12), SiW12O404− (SiW12), H2W12O406− (H2W12)) and TiO2 hybrid thin films were prepared using the layer-by-layer method. Their photocatalytic activities were investigated using gaseous 2-propanol decomposition. All films were transparent in the visible wavelength range. For 2-propanol decomposition, H2W12 was the most effective for the combination with TiO2 despite having the smallest TiO2 deposition amount. The photocatalytic activity of the PW12–TiO2 hybrid film was increased 2.3 times by visible light with UV illumination. This increase was less remarkable for hybrid films of other Keggin ions, suggesting that the visible light excitation of reduced PW12 plays an important role in the enhancement of 2-propanol decomposition. 相似文献
122.
Ming L. Tang Anna D. Reichardt Toshihiro Okamoto Nobuyuki Miyaki Zhenan Bao 《Advanced functional materials》2008,18(10):1579-1585
A series of compounds from the tetraceno[2,3‐b]thiophene and the anthra[2,3‐b]thiophene family of semiconducting molecules has been made. Specifically, synthetic routes to functionalize the parent molecules with bromo and then hexyl groups are shown. The bromo‐ and hexyl‐functionalized tetraceno[2,3‐b]thiophene and anthra[2,3‐b]thiophene were characterized in the top‐contact thin‐film transistor (TFT) geometry. They give high mobilities, ranging from 0.12 cm2 V?1 s?1 for α‐n‐hexylanthra[2,3‐ b]thiophene to as high as 0.85 cm2 V?1 s?1 for α‐bromotetraceno[2,3‐b]thiophene. Notably, grain size increases, going from the shorter anthra[2,3‐b]thiophene core to the longer tetraceno[2,3‐b]thiophene core, with a corresponding increase in mobility. The transition from undesirable 3D to desirable 2D thin‐film growth is explained by the increase in length of the molecule, in this case by one benzene ring, which results in an increase in intralayer interactions relative to interlayer interactions. 相似文献
123.
Shigeru Katayama Rio Yamazaki Hikaru Umise Hsu Pei Han Toshihiro Mihara Kimiko Uchiyama Hajime Takahashi Soichiro Nakamura 《Molecular nutrition & food research》2023,67(16):2200212
Scope
Ultraviolet B (UVB) radiation causes skin barrier dysfunction, leading to decreased water-holding capacity, impaired epidermal barrier function, and increased skin thickness. This study investigates the protective effects of oral administration of Lacticaseibacillus paracasei K71 against skin barrier dysfunction in UVB-irradiated mice.Methods and results
Mice are fed diets with or without K71 and irradiated with UVB three times a week for 12 weeks. Oral administration of K71 suppresses UVB-induced decrease in stratum corneum water content, mitigates the increase of transepidermal water loss, and decreases epidermal thickness of the dorsal skin. Treatment with K71 reverses the upregulation of inflammatory cytokines and the activation of nuclear factor-κB induced by UVB irradiation and upregulates the expression of anti-inflammatory IL-10 in the dorsal skin. Notable upregulation of IL-10 is observed in the spleens of K71-treated mice. K71 treatment enhances IL-10 production in J774.1 macrophages; however, this enhancement is diminished by inhibiting K71 phagocytosis and TLR3. Furthermore, transfection using K71 RNAs significantly increases IL-10 production.Conclusion
These results indicate that K71 may alleviate UVB-induced skin barrier dysfunction by attenuating inflammation via increasing IL-10 production and that K71 RNAs may induce IL-10 production in macrophages. Therefore, K71 may be beneficial for preventing skin barrier dysfunction. 相似文献124.
Maki Toshihiro Horimoto Hiroumi Ishihara Takashi Kofuji Kazuya 《International Journal of Control, Automation and Systems》2020,18(3):597-604
International Journal of Control, Automation and Systems - This paper proposes a method for autonomous underwater vehicles to chase sea turtles without attaching any tag to them, toward efficient... 相似文献
125.
Ryutaro Usukawa Toshihiro Ishikawa 《International Journal of Applied Ceramic Technology》2019,16(6):2111-2120
Most of the present production processes of SiC sintered bodies require some powder mixing using a mechanical milling process (ball milling, and so on). In this case, relatively long hours are required, and there is the problem of contamination during the preparation process. To avoid these problems, we developed a new process for obtaining a self-sinterable, stoichiometric SiC powder, whose precursor material is water-soluble; the precursor material was synthesized from aqueous silica and citric acid containing a small amount of aluminum compound. In order to obtain the stoichiometric SiC composition, the above aqueous precursor material was adequately cured in air (200°C-400°C); subsequently carbonization reaction (~800°C) in nitrogen atmosphere, carbothermal reduction (~1600°C) in argon atmosphere, and pressureless sintering (~1900°C) were performed. Among these processes, the curing process (cross-linking process) is very important for obtaining the equivalent composition (silica and carbon) for the subsequent carbothermal reduction. In this study, the adequate curing temperature and suitable preparation condition for the carbothermal reduction were investigated for the production of stoichiometric self-sinterable SiC powder. The pressureless sintered body achieved using the obtained SiC powder demonstrated a desirable trans-crystalline fracture behavior. 相似文献
126.
127.
128.
Zhang Lan Lu Jian Nogami Hirofumi Okada Hironao Itoh Toshihiro Arai Shozo 《Microsystem Technologies》2018,24(1):457-463
Microsystem Technologies - During the growth of Japanese cows, the ruminal pH value is an important physiological parameter, which remarkably affects their nutritional status. To monitor the health... 相似文献
129.
Kiyotaka Shibata Toshihiro Okabe Kouji Saito Takayuki Okayama Masahiro Shimada Akira Yamamura Ryoichi Yamamoto 《Journal of Porous Materials》1997,4(4):269-275
Woodceramics are new porous carbon materials, which are made by impregnating woody materials with phenol resin and then thermoformed in a vacuum furnace and these have been shown to have electromagnetic shielding properties. In the recycling of wastepaper, ways of using the wastepaper other than for paper pulp are needed to be developed. In this study, we made Woodceramics from handbill advertisement paper and telephone directory paper, and measured their electromagnetic shielding properties in order to find new uses for wastepaper. The results showed that the Woodceramics made from wastepaper had an electric shielding effectiveness of 30 dB for 100 MHz and 40 to 43 dB for 300 MHz or higher, and had a magnetic shielding effectiveness of 30 dB for 100 MHz and 37 dB for about 400 MHz. An electric equivalent circuit of the pore model in the Woodceramics is introduced. In addition, it is proposed that the excellent electromagnetic shielding effectiveness of the Woodceramics is caused by dielectric loss. 相似文献
130.
Akihiko Sugai Rie Sakuma Ikuko Fukuda Norio Kurosawa Yuko H. Itoh Kazuo Kon Susumu Ando Toshihiro Itoh 《Lipids》1995,30(4):339-344
The major ether-type lipid structures ofSulfolobus acidocaldarius (ATCC33909) were composed of caldarchaeol and calditoglycerocaldarchaeol. However, the characterization by nuclear magnetic
resonance spectroscopy and mass spectrometry showed that the structure of calditol in calditoglycerocaldarchaeol is not nonitol,
2-(1′,2′,3′-trihydroxypropyl)1,2,3,4,5,6-hexahydroxyhexane, but 2-hydroxymethyl-1-(2,3-dihydroxypropoxy),2,3,4,5-cyclopentanetetraol
with an ether linkage in the molecule. Such an intermolecular ether linkage was resistant, to BCl3 treatment, but nonresistant to 57% HI degradation treatment conducted at 100°C for 60 h, producting 2-hydroxymethyl-1,2,3,4,5-cyclopentanepentaol
from calditol as reaction product. Further, it was confirmed that the structure of calditol is essentially a derivative of
glycerol, and hydrocarbon chains were conjugated to the glycerol-like site in the structure. The calditol with an ether linkage
in the molecule suggested an important role regarding the properties of heat-resistance and acid-resistance observed inSulfolobales.
Presented at the international workshop on “Molecular Biology and Biotechnology of Extremophiles and Archaebacteria,” Wako,
Japan, August 1993. 相似文献