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991.
992.
993.
Robust dynamic surface control (RDSC) is effective in alleviating the implementation difficulty of backstepping‐based multiple‐surface sliding control (MSSC) for a class of strict‐feedback nonlinear systems with mismatched uncertainties. However, the synthesis and analysis of the classical RDSC are conservative, which not only may lead to an impractical control law but also cannot fully reveal the technical nature of RDSC. This article provides a comprehensive study of a preferred RDSC law with an approximation of the signum function based on the singular perturbation theory. By formulating the control problem into a singular perturbation form, it is proven that the preferred RDSC recovers the performance of MSSC as the decrease of a filter parameter. The attractive features of the preferred RDSC revealed during the proposed synthesis and analysis include: (a) the control gain can be significantly reduced resulting in a sharp decrease of control energy and (b) the closed‐loop stability can be guaranteed by only decreasing the filter parameter. Simulation results have been shown to be consistent with the theoretical findings. 相似文献
994.
Chee Keong Ng Sutharshan Rajasegarar Lei Pan Frank Jiang Leo Yu Zhang 《Concurrency and Computation》2020,32(14)
This research presents a novel framework comprising the IPS gateway, analysis system, and honeypot for identifying and detecting ransomware based on the client honeypot concept, and active interception of downloads using Suricata inline intruder prevention system. Unlike previous frameworks that report on the accuracy rate of detecting ransomware, the proposed framework features a multiple voting platform for the validation of confidence levels in the accuracy detection rates. The proposed framework achieves high accuracy levels than other machine learning models for the detection of ransomware. 相似文献
995.
996.
Xiaofei Pan Cheng-Tang Wu Wei Hu 《International journal for numerical methods in engineering》2020,121(17):3979-4002
A new particle Galerkin method is introduced to solve the Naiver-Stokes equations in a Lagrangian fashion. The present method aims to suppress key numerical instabilities observed in the strong form Lagrangian particle methods such as smoothed particle hydrodynamics (SPH), incompressible SPH, and moving particle semi-implicit for incompressible free surface flow simulations. It is well-known that strong form Lagrangian particle methods usually rely on ad hoc particle stabilization techniques based on particle shifting, artificial viscosity, or density-invariant condition due to some formulation inconsistency issues. In the present method, we introduce a momentum-consistent velocity smoothing algorithm which is used to combine with the second-order rotational incremental pressure-correction scheme to stabilize the pressure field as well as to enforce the consistency of Neumann boundary condition. To further impose slip-free or nonslip boundary conditions for the fluid flow, a penalty method which is free of ghost or dummy particles is developed. Finally, a particle insertion-deletion adaptive scheme is proposed when the violent fluid flow is considered. Four numerical examples are studied to validate the accuracy and stability of the present method. 相似文献
997.
Pan Xiong Bing Sun Nobuyuki Sakai Renzhi Ma Takayoshi Sasaki Shijian Wang Jinqiang Zhang Guoxiu Wang 《Advanced materials (Deerfield Beach, Fla.)》2020,32(18):1902654
2D genuine unilamellar nanosheets, that are, the elementary building blocks of their layered parent crystals, have gained increasing attention, owing to their unique physical and chemical properties, and 2D features. In parallel with the great efforts to isolate these atomic-thin crystals, a unique strategy to integrate them into 2D vertically stacked heterostuctures has enabled many functional applications. In particular, such 2D heterostructures have recently exhibited numerous exciting electrochemical performances for energy storage and conversion, especially the molecular-scale heteroassembled superlattices using diverse 2D unilamellar nanosheets as building blocks. Herein, the research progress in scalable synthesis of 2D superlattices with an emphasis on a facile solution-phase flocculation method is summarized. A particular focus is brought to the advantages of these 2D superlattices in applications of supercapacitors, rechargeable batteries, and water-splitting catalysis. The challenges and perspectives on this promising field are also outlined. 相似文献
998.
Qi Wen Pan Jia Liuxuan Cao Jipeng Li Di Quan Lili Wang Yanbing Zhang Diannan Lu Lei Jiang Wei Guo 《Advanced materials (Deerfield Beach, Fla.)》2020,32(16):1903954
Layered graphene oxide membranes (GOMs) offer a unique platform for precise sieving of small ions and molecules due to controlled sub-nanometer-wide interlayer distance and versatile surface chemistry. Pristine and chemically modified GOMs effectively block organic dyes and nanoparticles, but fail to exclude smaller ions with hydrated diameters less than 9 Å. Toward sieving of small inorganic salt ions, a number of strategies are proposed by reducing the interlayer spacing down to merely several angstroms. However, one critical challenge for such compressed GOMs is the extremely low water flux (<0.1 Lm−2 h−1 bar−1) that prevents these innovative nanomaterials from being used in real-world applications. Here, a planar heterogeneous graphene oxide membrane (PHGOM) with both nearly perfect salt rejection and high water flux is reported. Horizontal ion transport through oppositely charged GO multilayer lateral heterojunction exhibits bi-unipolar transport behavior, blocking the conduction of both cations and anions. Assisted by a forward electric field, salt concentration is depleted in the near-neutral transition area of the PHGOM. In this situation, deionized water can be extracted from the depletion zone. Following this mechanism, a high rejection rate of 97.0% for NaCl and water flux of 1529 Lm−2 h−1 bar−1 at the outlet via an inverted T-shaped water extraction mode are achieved. 相似文献
999.
Durga Prasad Karothu Jad Mahmoud Halabi Liang Li Abraham Colin-Molina Braulio Rodríguez-Molina Panče Naumov 《Advanced materials (Deerfield Beach, Fla.)》2020,32(20):1906216
Crystal adaptronics is an emergent materials science discipline at the intersection of solid-state chemistry and mechanical engineering that explores the dynamic nature of mechanically reconfigurable, motile, and explosive crystals. Adaptive molecular crystals bring to materials science a qualitatively new set of properties that associate long-range structural order with softness and mechanical compliance. However, the full potential of this class of materials remains underexplored and they have not been considered as materials of choice in an engineer's toolbox. A set of general performance metrics that can be used for quantification of the performance of these prospective dynamic materials as micro- and macroactuators is presented. The indices are calculated on two selected representatives of thermosalient solids—materials that undergo rapid martensitic transitions accompanied with macroscopic locomotion. Benchmarking of their performance against extensive set of data for the existing actuator classes and visualization using materials property charts uncover the hidden potential and advantages of dynamic crystals, while they also reveal their drawbacks for actual application as actuators. Altogether the results indicate that, if the challenges with fabrication and implementation in devices are overcome, adaptive molecular crystals can have far-reaching implications for emerging fields such as smart microelectronics and soft microrobotics. 相似文献
1000.
Jiacheng Sun Yuyan Wang Shaoqiang Guo Bensong Wan Lianqing Dong Youdi Gu Cheng Song Caofeng Pan Qinghua Zhang Lin Gu Feng Pan Junying Zhang 《Advanced materials (Deerfield Beach, Fla.)》2020,32(9):1906499
As unique building blocks for next-generation optoelectronics, high-quality 2D p–n junctions based on semiconducting transition metal dichalcogenides (TMDs) have attracted wide interest, which are urgent to be exploited. Herein, a novel and facile electron doping of WSe2 by cetyltrimethyl ammonium bromide (CTAB) is achieved for the first time to form a high-quality intramolecular p–n junction with superior optoelectronic properties. Efficient manipulation of charge carrier type and density in TMDs via electron transfer between Br− in CTAB and TMDs is proposed theoretically by density functional theory (DFT) calculations. Compared with the intrinsic WSe2 photodetector, the switching light ratio (Ilight/Idark) of the p–n junction device can be enhanced by 103, and the temporal response is also dramatically improved. The device possesses a responsivity of 30 A W−1, with a specific detectivity of over 1011 Jones. In addition, the mechanism of charge transfer in CTAB-doped 2D WSe2 and WS2 are investigated by designing high-performance field effect transistors. Besides the scientific insight into the effective manipulation of 2D materials by chemical doping, this work presents a promising applicable approach toward next-generation photoelectronic devices with high efficiency. 相似文献