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101.
Yong‐Ning Zhou Mahsa Sina Nathalie Pereira Xiqian Yu Glenn G. Amatucci Xiao‐Qing Yang Frederic Cosandey Kyung‐Wan Nam 《Advanced functional materials》2015,25(5):696-703
Searching high capacity cathode materials is one of the most important fields of the research and development of sodium‐ion batteries (SIBs). Here, we report a FeO0.7F1.3/C nanocomposite synthesized via a solution process as a new cathode material for SIBs. This material exhibits a high initial discharge capacity of 496 mAh g?1 in a sodium cell at 50 °C. From the 3rd to 50th cycle, the capacity fading is only 0.14% per cycle (from 388 mAh g?1 at 3rd the cycle to 360 mAh g?1 at the 50th cycle), demonstrating superior cyclability. A high energy density of 650 Wh kg?1 is obtained at the material level. The reaction mechanism studies of FeO0.7F1.3/C with sodium show a hybridized mechanism of both intercalation and conversion reaction. 相似文献
102.
A compact-size microstrip spiral resonator and its application to microwave oscillator 总被引:1,自引:0,他引:1
Young-Taek Lee Jong-Sik Lim Chul-Soo Kim Dal Ahn Sangwook Nam 《Microwave and Wireless Components Letters, IEEE》2002,12(10):375-377
This letter presents a compact size microstrip spiral resonator and its application to a low phase noise oscillator. This resonator has stopband characteristics to be used in the series feedback oscillator topology. The whole circuit area of the proposed resonator is within 1/10 wavelength, which results in the reduction of the circuit area and cost. A 10-GHz oscillator incorporated with this resonator was designed, fabricated and measured. It shows low phase noise performance of -95.4-dBc/Hz at 100 kHz offset. 相似文献
103.
Chan-Soo Hwang Seung Hoon Nam Jaehak Chung Tarokh V. 《Signal Processing, IEEE Transactions on》2003,51(11):2955-2964
We propose differential space time block codes (STBC) using nonconstant modulus constellations, e.g., quadrature amplitude modulation (QAM), which cannot be utilized in the conventional differential STBC. Since QAM constellations have a larger minimum distance compared with the phase shift keying (PSK), the proposed method has the advantage of signal-to-noise ratio (SNR) gain compared with conventional differential STBC. The QAM signals are encoded in a manner similar to that of the conventional differential STBC. To decode nonconstant modulus signals, the received signals are normalized by the channel power estimated forgoing training symbols and then decoded with a conventional QAM decoder. Assuming the knowledge of the channel power at the receiver, the symbol error rate (SER) bound of the proposed method under independent Rayleigh fading assumption is derived, which shows better SER performance than the conventional differential STBC. When the transmission rate is more than 3 bits/channel use in time-varying channels, the simulation results demonstrate that the proposed method with the channel power estimation outperforms the conventional differential STBC. Specifically, the posed method using the channel power estimation obtains a 7.3 dB SNR gain at a transmission rate of 6 bits/channel use in slow fading channels. Although the performance gap between the proposed method and the conventional one decreases as the Doppler frequency increases, the proposed method still exhibits lower SER than the conventional one, provided the estimation interval L is chosen carefully. 相似文献
104.
Kim H. Nam B.-G. Sohn J.-H. Woo J.-H. Yoo H.-J. 《Solid-State Circuits, IEEE Journal of》2006,41(11):2373-2381
A 32-bit fixed-point logarithmic arithmetic unit is proposed for the possible application to mobile three-dimensional (3-D) graphics system. The proposed logarithmic arithmetic unit performs division, reciprocal, square-root, reciprocal-square-root and square operations in two clock cycles and powering operation in four clock cycles. It can program its number range for accurate computation flexibility of 3-D graphics pipeline and eight -region piecewise linear approximation model for logarithmic and antilogarithmic conversion to reduce the operation error under 0.2%. Its test chip is implemented by 1-poly 6-metal 0.18-mum CMOS technology with 9-k gates. It operates at the maximum frequency of 231 MHz and consumes 2.18 mW at 1.8-V supply 相似文献
105.
Dohyung Kim Hyeonsu Bang Hyoung Won Baac Jongmin Lee Phuoc Loc Truong Bum Ho Jeong Tamilselvan Appadurai Kyu Kwan Park Donghyeok Heo Vu Binh Nam Hocheon Yoo Kyeounghak Kim Daeho Lee Jong Hwan Ko Hui Joon Park 《Advanced functional materials》2023,33(14):2213064
Reversible metal-filamentary mechanism has been widely investigated to design an analog resistive switching memory (RSM) for neuromorphic hardware-implementation. However, uncontrollable filament-formation, inducing its reliability issues, has been a fundamental challenge. Here, an analog RSM with 3D ion transport channels that can provide unprecedentedly high reliability and robustness is demonstrated. This architecture is realized by a laser-assisted photo-thermochemical process, compatible with the back-end-of-line process and even applicable to a flexible format. These superior characteristics also lead to the proposal of a practical adaptive learning rule for hardware neural networks that can significantly simplify the voltage pulse application methodology even with high computing accuracy. A neural network, which can perform the biological tissue classification task using the ultrasound signals, is designed, and the simulation results confirm that this practical adaptive learning rule is efficient enough to classify these weak and complicated signals with high accuracy (97%). Furthermore, the proposed RSM can work as a diffusive-memristor at the opposite voltage polarity, exhibiting extremely stable threshold switching characteristics. In this mode, several crucial operations in biological nervous systems, such as Ca2+ dynamics and nonlinear integrate-and-fire functions of neurons, are successfully emulated. This reconfigurability is also exceedingly beneficial for decreasing the complexity of systems—requiring both drift- and diffusive-memristors. 相似文献
106.
Hye-Seon Jeong Eunseo Kim Changwoo Nam Yoon Choi You-Jeong Lee David A. Weitz Hyomin Lee Chang-Hyung Choi 《Advanced functional materials》2021,31(18):2009553
A hydrogel microcapsule with an intermediate thin oil layer is presented to achieve smart release of a broad range of cargoes triggered via diverse stimuli. A microfluidic technique is used to produce triple emulsion droplets with a thin oil layer that separates the innermost aqueous phase from the hydrogel prepolymer phase, which transforms into a hydrogel shell via photopolymerization. The intermediate oil layer within the hydrogel microcapsule acts as an effective diffusion barrier, allowing encapsulation of various small cargoes within a porous hydrogel shell until a stimulus is applied to destabilize the oil layer. It is demonstrated that diverse stimuli including chemical dissolution, mechanical stress, and osmotic pressure can be utilized to release the encapsulated cargo on-demand. In addition, osmotic pressure and the hydrogel shell thickness can be independently tuned to control the onset time of release as well as the release behavior of multi-cargo encapsulated hydrogel microcapsule. The release can be either simultaneous or selective. 相似文献
107.
Light‐Induced Surface Modification of Natural Plant Microparticles: Toward Colloidal Science and Cellular Adhesion Applications 下载免费PDF全文
Ee‐Lin Tan Michael G. Potroz Gaia Ferracci Joshua A. Jackman Haram Jung Lili Wang Nam‐Joon Cho 《Advanced functional materials》2018,28(18)
Playing an instrumental role in the life of plants, pollen microparticles are one of the most fascinating biological materials in existence, with abundant and renewable supply, ultrahigh durability, and unique, species‐specific architectural features. Aside from their biological role, pollen microparticles also demonstrate broad utility as functional materials for drug delivery and microencapsulation, and increasingly for emulsion‐type applications. As natural pollen microparticles are predominantly hydrophobic, developing robust surface functionalization strategies to increase surface hydrophilicity would increase the range of colloidal science applications, including opening the door to interfacing microparticles with biological cells. This research investigates the extraction and light‐induced surface modification of discrete pollen microparticles from bee‐collected pollen granules toward achieving functional control over the responses elicited from discrete particles in colloidal science and cellular applications. Ultraviolet–ozone treatment is shown to increase the proportion of surface elemental oxygen and ketones, leading to increased surface hydrophilicity, enhanced particle dispersibility, tunable control over Pickering emulsion characteristics, and enhanced cellular adhesion. In summary, the findings demonstrate that light‐induced surface modification improves the functional properties of pollen microparticles, and such insights also have broad implications across materials science and environmental science applications. 相似文献
108.
Hierarchical NiMoS and NiFeS Nanosheets with Ultrahigh Energy Density for Flexible All Solid‐State Supercapacitors 下载免费PDF全文
Jayaraman Balamurugan Chao Li Vanchiappan Aravindan Nam Hoon Kim Joong Hee Lee 《Advanced functional materials》2018,28(35)
Highly flexible supercapacitors (SCs) have great potential in modern electronics such as wearable and portable devices. However, ultralow specific capacity and low operating potential window limit their practical applications. Herein, a new strategy for the fabrication of free‐standing Ni?Mo?S and Ni?Fe?S nanosheets (NSs) for high‐performance flexible asymmetric SC (ASC) through hydrothermal and subsequent sulfurization technique is reported. The effect of Ni2+ is optimized to attain hierarchical Ni?Mo?S and Ni?Fe?S NS architectures with high electrical conductivity, large surface area, and exclusive porous networks. Electrochemical properties of Ni?Mo?S and Ni?Fe?S NS electrodes exhibit that both have ultrahigh specific capacities (≈312 and 246 mAh g?1 at 1 mA cm?2), exceptional rate capabilities (78.85% and 78.46% capacity retention even at 50 mA cm?2, respectively), and superior cycling stabilities. Most importantly, a flexible Ni?Mo?S NS//Ni?Fe?S NS ASC delivers a high volumetric capacity of ≈1.9 mAh cm?3, excellent energy density of ≈82.13 Wh kg?1 at 0.561 kW kg?1, exceptional power density (≈13.103 kW kg?1 at 61.51 Wh kg?1) and an outstanding cycling stability, retaining ≈95.86% of initial capacity after 10 000 cycles. This study emphasizes the potential importance of compositional tunability of the NS architecture as a novel strategy for enhancing the charge storage properties of active electrodes. 相似文献
109.
Thermally Controlled,Patterned Graphene Transfer Printing for Transparent and Wearable Electronic/Optoelectronic System 下载免费PDF全文
Moon Kee Choi Inhyuk Park Dong Chan Kim Eehyung Joh Ok Kyu Park Jaemin Kim Myungbin Kim Changsoon Choi Jiwoong Yang Kyoung Won Cho Jae‐Ho Hwang Jwa‐Min Nam Taeghwan Hyeon Ji Hoon Kim Dae‐Hyeong Kim 《Advanced functional materials》2015,25(46):7109-7118
Graphene has been highlighted as a platform material in transparent electronics and optoelectronics, including flexible and stretchable ones, due to its unique properties such as optical transparency, mechanical softness, ultrathin thickness, and high carrier mobility. Despite huge research efforts for graphene‐based electronic/optoelectronic devices, there are remaining challenges in terms of their seamless integration, such as the high‐quality contact formation, precise alignment of micrometer‐scale patterns, and control of interfacial‐adhesion/local‐resistance. Here, a thermally controlled transfer printing technique that allows multiple patterned‐graphene transfers at desired locations is presented. Using the thermal‐expansion mismatch between the viscoelastic sacrificial layer and the elastic stamp, a “heating and cooling” process precisely positions patterned graphene layers on various substrates, including graphene prepatterns, hydrophilic surfaces, and superhydrophobic surfaces, with high transfer yields. A detailed theoretical analysis of underlying physics/mechanics of this approach is also described. The proposed transfer printing successfully integrates graphene‐based stretchable sensors, actuators, light‐emitting diodes, and other electronics in one platform, paving the way toward transparent and wearable multifunctional electronic systems. 相似文献
110.
Yoo SK Wang G Collison F Rubinstein JT Vannier MW Kim HJ Kim NH 《IEEE transactions on bio-medical engineering》2004,51(5):838-846
Three-dimensional (3-D) localization of individual cochlear implant electrodes within the inner ear is of importance for modeling the electrical field of the cochlea, designing the electrode array, and programming the associated speech processor. A 3-D reconstruction method of cochlear implant electrodes is proposed to localize individual electrodes from two X-ray views in combination with the spiral computed tomography technique. By adapting epipolar geometry to the configuration of an X-ray imaging system, we estimate individual electrode locations in the least square sense without using a patient attachment required by an existing stereophotogrammetry technique. Furthermore, our method does not require any knowledge of the intrinsic and extrinsic parameters of the imaging system. The performance of our method is studied in numerical simulation and with patient data and is found to be sufficiently accurate for clinical use. The maximum root mean-square errors measured are 0.0445 and 0.214 mm for numerical simulation and patient data, respectively. 相似文献