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排序方式: 共有9085条查询结果,搜索用时 15 毫秒
71.
Optimized Photoinitiator for Fast Two‐Photon Absorption Polymerization of Polyester‐Macromers for Tissue Engineering 下载免费PDF全文
72.
Structure and Magnetic Property Control of Copper Hydroxide Acetate by Non‐Classical Crystallization 下载免费PDF全文
RuiQi Song Theodora Krasia‐Christoforou Christian Debus Helmut Cölfen 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(9)
Copper hydroxide acetate (CHA), one layered hydroxide compound with tunable magnetism, attracts great interest because of its potential applications in memory devices. However, ferromagnetism for CHA is only demonstrated by means of GPa pressure. Herein, a new method is reported, involving the combination of different crystallization pathways to control crystallization of amorphous CHA toward the formation of CHA/polymer composites with tunable magnetic properties and even a tunability that can be tested at room temperature. By using poly[(ethylene glycol)6 methyl ether methacrylate]‐block‐poly[2‐(acetoacetoxy) ethyl methacrylate] (PEGMA‐b‐PAEMA) diblock copolymers as additives in combination with a post‐treatment process by ultracentrifugation, it is demonstrated that CHA and PEGMA‐b‐PAEMA form composites exhibiting different magnetic properties, depending on CHA in‐plane nanostructures. Analytical characterization reveals that crystallization of CHA is induced by ultracentrifugation, during which CHA nanostructures can be well controlled by changing the degrees of polymerization of the PEGMA and PAEMA blocks and their block length ratios. These findings not only present the first example of using crystallization from polymer stabilized amorphous precursors toward the generation of magnetic nanomaterials with tunable magnetism but also pave the way for the future design of functional composite materials. 相似文献
73.
Mariano J. Savelski C. Stewart Slater Paul V. Tozzi Christian M. Wisniewski 《Clean Technologies and Environmental Policy》2017,19(10):2467-2477
This study explores design alternatives for the purification and possible reuse of low-volume organic solvents waste streams in pharmaceutical manufacturing. Solvent use has a large impact on the life cycle of pharmaceutical processes, as typically 80–90% of the total mass used in the production of an active pharmaceutical ingredient is attributed to solvent use. Solvents are not consumed in pharmaceutical processes so they exit the process as waste. These waste streams are usually disposed of using incineration; therefore, generating significant life cycle emissions from disposal and replacement of virgin solvent. Solvent recovery efforts are generally limited to large-volume waste streams. However, results show that solvents in low-volume streams can also be economically recovered using a versatile multi-campaign solvent recovery skid. Three different solvent waste streams were evaluated, and 85.3% reduction in total emissions and 86.3% reduction in operating costs were achieved. Investment in the solvent recovery system was determined to have a payback period of 4.5 years and a 28% IRR over 10 years. A life cycle impact assessment shows impacts on the human health, ecosystems, and resources categories have been reduced by 82.4, 85.1, and 87.1%, respectively. 相似文献
74.
Bioimaging: Shaping Luminescent Properties of Yb3+ and Ho3+ Co‐Doped Upconverting Core–Shell β‐NaYF4 Nanoparticles by Dopant Distribution and Spacing (Small 47/2017) 下载免费PDF全文
75.
Real‐time updating of structural mechanics models using Kalman filtering,modified constitutive relation error,and proper generalized decomposition 下载免费PDF全文
Basile Marchand Ludovic Chamoin Christian Rey 《International journal for numerical methods in engineering》2016,107(9):786-810
The paper aims at proposing a new strategy for real‐time identification or updating of structural mechanics models defined as dynamical systems. The main idea is to introduce the modified constitutive relation error concept, which is a practical tool that enables to efficiently solve identification problems with highly corrupted data, into the Kalman filtering, which is a classical framework for data assimilation. Furthermore, a PGD‐based model reduction method is performed in order to optimize capabilities of the online updating strategy. Performances of the proposed approach, in terms of robustness gain and computational cost reduction, are illustrated on several unsteady thermal applications. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
76.
77.
Unraveling Unprecedented Charge Carrier Mobility through Structure Property Relationship of Four Isomers of Didodecyl[1]benzothieno[3,2‐b][1]benzothiophene 下载免费PDF全文
Yusuke Tsutsui Guillaume Schweicher Basab Chattopadhyay Tsuneaki Sakurai Jean‐Baptiste Arlin Christian Ruzié Almaz Aliev Artur Ciesielski Alan R. Kennedy Vincent Lemaur Yoann Olivier Rachid Hadji Lionel Sanguinet Frédéric Castet Silvio Osella Dmytro Dudenko David Beljonne Jérôme Cornil Paolo Samorì Shu Seki Yves H. Geerts 《Advanced materials (Deerfield Beach, Fla.)》2016,28(33):7106-7114
78.
Single‐Molecule Magnets: Giant Hysteresis of Single‐Molecule Magnets Adsorbed on a Nonmagnetic Insulator (Adv. Mater. 26/2016) 下载免费PDF全文
79.
Gian Luigi Angrisani Piriya Taptimthong Susanne Elisabeth Thürer Christian Klose Hans Jürgen Maier Marc Christopher Wurz Kai Möhwald 《Advanced Engineering Materials》2018,20(9)
80.
Mónica Giménez‐Marqués Elena Bellido Thomas Berthelot Teresa Simón‐Yarza Tania Hidalgo Rosana Simón‐Vázquez África González‐Fernández José Avila Maria Carmen Asensio Ruxandra Gref Patrick Couvreur Christian Serre Patricia Horcajada 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(40)
Controlling the outer surface of nanometric metal–organic frameworks (nanoMOFs) and further understanding the in vivo effect of the coated material are crucial for the convenient biomedical applications of MOFs. However, in most studies, the surface modification protocol is often associated with significant toxicity and/or lack of selectivity. As an alternative, how the highly selective and general grafting GraftFast method leads, through a green and simple process, to the successful attachment of multifunctional biopolymers (polyethylene glycol (PEG) and hyaluronic acid) on the external surface of nanoMOFs is reported. In particular, effectively PEGylated iron trimesate MIL‐100(Fe) nanoparticles (NPs) exhibit suitable grafting stability and superior chemical and colloidal stability in different biofluids, while conserving full porosity and allowing the adsorption of bioactive molecules (cosmetic and antitumor agents). Furthermore, the nature of the MOF–PEG interaction is deeply investigated using high‐resolution soft X‐ray spectroscopy. Finally, a cell penetration study using the radio‐labeled antitumor agent gemcitabine monophosphate (3H‐GMP)‐loaded MIL‐100(Fe)@PEG NPs shows reduced macrophage phagocytosis, confirming a significant in vitro PEG furtiveness. 相似文献