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81.
Qiyi Fang Zhepeng Zhang Qingqing Ji Siya Zhu Yue Gong Yu Zhang Jianping Shi Xiebo Zhou Lin Gu Qian Wang Yanfeng Zhang 《Nano Research》2017,10(8):2761-2771
Molybdenum ditelluride (MoTe2),which is an important transition-metal dichalcogenide,has attracted considerable interest owing to its unique properties,such as its small bandgap and large Seebeck coefficient.However,the batch production of monolayer MoTe2 has been rarely reported.In this study,we demonstrate the synthesis of large-domain (edge length exceeding 30 μm),monolayer MoTe2 from chemical vapor deposition-grown monolayer MoS2 using a chalcogen atom-exchange synthesis route.An in-depth investigation of the tellurization process reveals that the substitution of S atoms by Te is prevalently initiated at the edges and grain boundaries of the monolayer MoS2,which differs from the homogeneous selenization of MoS2 flakes with the formation of alloyed Mo-S-Se hybrids.Moreover,we detect a large compressive strain (approximately-10%) in the transformed MoTe2 lattice,which possibly drives the phase transition from 2H to 1T'at the reaction temperature of 500 ℃.This phase change is substantiated by experimental facts and first-principles calculations.This work introduces a novel route for the templated synthesis of two-dimensional layered materials through atom substitutional chemistry and provides a new pathway for engineering the strain and thus the intriguing physics and chemistry. 相似文献
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83.
Ultrathin 2D Zirconium Metal–Organic Framework Nanosheets: Preparation and Application in Photocatalysis 下载免费PDF全文
Ting He Bing Ni Simin Zhang Yue Gong Haiqing Wang Lin Gu Jing Zhuang Wenping Hu Xun Wang 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(16)
Synthesizing ultrathin 2D metal–organic framework nanosheets in high yields has received increasing research interest but remains a great challenge. In this work, ultrathin zirconium‐porphyrinic metal–organic framework (MOF) nanosheets with thickness down to ≈1.5 nm are synthesized through a pseudoassembly–disassembly strategy. Owing to the their unique properties originating from their ultrathin thickness and highly exposed active sites, the as‐prepared ultrathin nanosheets exhibit far superior photocatalysis performance compared to the corresponding bulk MOF. This work highlights new opportunities in designing ultrathin MOF nanosheets and paves the way to expand the potential applications of MOFs. 相似文献
84.
Lili Gong Qi Zhang Liangjun Wang Jianfeng Wu Cheng Han Bo Lei Wei Chen Goki Eda Kuan Eng Johnson Goh Chorng Haur Sow 《Nano Research》2018,11(9):4574-4586
We demonstrate a facile and effective approach to significantly improve the photoluminescence of bulk MoS2 via laser thinning followed by gold particle decoration. Upon laser thinning of exfoliated bulk MoS2, photoluminescence emerges from the laser-thinned region. After further treatment with an AuCl3 solution, gold particles self-assemble on the laser-thinned region and thick edges, further increasing the fluorescence of bulk MoS2 28 times and the Raman response 3 times. Such fluorescence enhancement can be attributed to both surface plasmon resonance and p-type doping induced by gold particles. The combination of laser thinning and AuCl3 treatment enables the functionalization of bulk MoS2 for optoelectronic applications. It can also provide a viable strategy for mask-free and area-selective p-type doping on single MoS2 flakes. 相似文献
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86.
在现有医疗磁导航系统和地磁数据的信息检测中,针对磁场测量中遇到的有线传输布线困难及操作不便等情况,利用ZigBee无线收发芯片(CC2430)组成的信息无线传输模块,给出了一种磁场检测无线传输解决方案;在此基础上,通过实验测量,验证ZigBee无线模块对磁感(MI)传感器输出产生影响;确认实际干扰的存在,并将其值量化,提出一套消除无线传输对MI传感器影响的解决方案。 相似文献
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88.
Approximate closed‐form expression is derived for the scattering from dipole arrays based on the equivalent circuit theory. Then, a method is proposed for synthesis of dipole arrays to produce desired scattering pattern using genetic algorithm (GA). In the synthesis method, the element positions in an array are considered as the optimization parameter and the derived expression is used to evaluate the fitness function of GA. To assess the validity and efficiency of the proposed method, several linear dipole arrays are designed to obtain scattering pattern with low sidelobe level (SLL). A good agreement between the patterns calculated using the expression and simulated by FEKO validates the accuracy of the presented expression. In addition, the numerical results show that the maximum SLL of the scattering pattern is considerably reduced by optimization. © 2011 Wiley Periodicals, Inc. Int J RF and Microwave CAE, 2011. 相似文献
89.
为了实现图像安全、快速加密,设计了一种新的数字图像混沌加密算法.仿真结果表明,该算法在没有扩散函数的情况下也能很好地改变图像的直方图,可以有效地抵制已知(选择)明文攻击,而且只有1次左映射或者右映射的情况下,该方法具有高置乱程度、良好的扩散性能和足够大的密钥空间,可获得足够高的安全性. 相似文献
90.