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151.
152.
Adhitya Gandaryus Saputro Arifin Luthfi Maulana Fadjar Fathurrahman Ganes Shukri Muhammad Haris Mahyuddin Mohammad Kemal Agusta Triati Dewi Kencana Wungu Hermawan Kresno Dipojono 《International Journal of Hydrogen Energy》2021,46(27):14418-14428
We study the CO2 hydrogenation to methanol on subnanometer Pd7 and transition metal doped Pd6M (M = Cu, Ni, Pt, and Rh) clusters using a combination of density functional theory and microkinetic calculations. We find that, in general, the inclusion of transition metal dopants could decrease the activation energy of several important elementary reactions. This condition results in a significant improvement in the activity of the catalyst, especially for the Pd6Ni cluster. We find that the Pd6M clusters are more selective toward the formate pathway than the RWGS + CO hydrogenation pathway. We also compare the turnover frequency profiles of the clusters with that of the Cu(111) surface, representing the standard industrial catalyst. We find that the Pd6Ni cluster can successfully overcome the TOF of Cu(111) surface, even at the low-pressure condition. 相似文献
153.
High melt viscosity of thermoplastic matrices hinders the impregnation of fibers and their consolidation during fabrication of composites. In the present study, matrix (polypropylene) and reinforcement (jute) fibers were comingled at fiber to fiber level (fiber to matrix ratio of 30, 40, 50 and 60%) while making their nonwoven fabrics using dry laid process. Thermoforming process, in which polypropylene fibers are used and then melted for the development of composite plates. The results showed that the composite samples with 0.30 fiber volume fraction have higher mechanical properties (flexural, impact energy), while samples with 0.40 fiber volume fraction have higher tensile properties (tensile strength and modulus) due to good impregnation of fiber and better fiber-matrix interface. The composite having 0.30 fiber volume fraction has lowest value of moisture regain and diffusion coefficients than the other samples. Voids present in the microscopic images also confirmed the weak interface, when the fiber volume fraction increased up to 0.60. 相似文献