全文获取类型
收费全文 | 528篇 |
免费 | 25篇 |
专业分类
电工技术 | 23篇 |
综合类 | 3篇 |
化学工业 | 168篇 |
金属工艺 | 13篇 |
机械仪表 | 18篇 |
建筑科学 | 12篇 |
能源动力 | 19篇 |
轻工业 | 54篇 |
水利工程 | 1篇 |
石油天然气 | 1篇 |
无线电 | 46篇 |
一般工业技术 | 97篇 |
冶金工业 | 11篇 |
原子能技术 | 17篇 |
自动化技术 | 70篇 |
出版年
2023年 | 12篇 |
2022年 | 23篇 |
2021年 | 26篇 |
2020年 | 12篇 |
2019年 | 18篇 |
2018年 | 20篇 |
2017年 | 14篇 |
2016年 | 19篇 |
2015年 | 10篇 |
2014年 | 26篇 |
2013年 | 43篇 |
2012年 | 30篇 |
2011年 | 53篇 |
2010年 | 31篇 |
2009年 | 19篇 |
2008年 | 21篇 |
2007年 | 23篇 |
2006年 | 15篇 |
2005年 | 10篇 |
2004年 | 10篇 |
2003年 | 12篇 |
2002年 | 10篇 |
2001年 | 13篇 |
2000年 | 8篇 |
1999年 | 4篇 |
1998年 | 9篇 |
1997年 | 4篇 |
1996年 | 6篇 |
1995年 | 8篇 |
1994年 | 2篇 |
1993年 | 1篇 |
1992年 | 3篇 |
1991年 | 3篇 |
1990年 | 1篇 |
1989年 | 2篇 |
1987年 | 2篇 |
1986年 | 1篇 |
1985年 | 1篇 |
1984年 | 1篇 |
1983年 | 1篇 |
1982年 | 2篇 |
1981年 | 1篇 |
1980年 | 4篇 |
1979年 | 3篇 |
1978年 | 3篇 |
1977年 | 4篇 |
1976年 | 3篇 |
1975年 | 2篇 |
1972年 | 3篇 |
1970年 | 1篇 |
排序方式: 共有553条查询结果,搜索用时 7 毫秒
51.
Kazuaki Yanagisawa Keishiro Ito Chisato Katsuki Kei Kawashima Masashi Shirabe 《Scientometrics》2010,84(3):563-573
An outcome of nuclear safety research (NSR) done by JAERI (Japan Atomic Energy Research Institute) was case studied by the bibliometric method. (1) For LOCA (loss-of-coolant accident) a domestic share of JAERI in monoclinic research paper was 63% at the past (20) 1978–1982 but was decreased to 40% at the present 1998–2002. For co-authored papers a domestic share between JAERI and PS (public sectors) was zero at past (20) but increased to 4% at the present. Research cooperation is active between Tokyo University and JAERI or between JAERI and Nagoya University. (2) It is revealed that LOCA outputs born by NSR-JAERI reflected partly to those of the Safety Licensing Guidelines, however, a share of NSR-JAERI could not determined due to the lack of necessary information in the Guideline. 相似文献
52.
Wei Zhang Kenji Ochi Michiya Fujiki Masanobu Naito Masaaki Ishikawa Kei‐ichi Kaneto Wataru Takashima Akinori Saeki Shu Seki 《Advanced functional materials》2010,20(22):3941-3947
In this paper a simple, casting solution technique for the preparation of two‐dimensional (2D) arrays of very‐high molecular weight (MW) 1D‐Pc supramolecular inorganic polymers is described. The soluble fluoroaluminium tetra‐tert‐butylphthalocyanine (ttbPcAlF) is synthesized and characterized, which can be self‐assembled to form 2D arrays of very‐high‐MW 1D‐Pc supramolecular inorganic polymers. High‐resolution transmission electron microscopy (HRTEM) demonstrates that the 1D‐ttbPcAlF, having a cofacial ring spacing of ~0.36 nm and an interchain distance of ~1.7 nm, self‐assembles into 2D‐nanosheets (~140 nm in length, ~20 nm in width, and equivalent to MW of 3.2 × 105 g mol?1). The film cast from a 1,2‐dichloroethane (DCE) solution shows a minimum hole‐mobility of ~0.3 cm2 V?1 s?1 at room temperature by flash‐photolysis time‐resolved microwave conductivity (TRMC) measurements and a fairly high dark dc‐conductivity of ~1 × 10?3 S cm?1. 相似文献
53.
Yuji Yabuki Yoshitaka Mukaida Yoshinori Saito Kazunori Oshima Tatsuo Takahashi Eiichi Muroi Kei Hashimoto Yasushi Uda 《Food chemistry》2010
To characterise the composition of sulphur-containing constituents in Chinese chive (Allium tuberosum Rottler), GC–MS and HPLC analyses were carried out, using 12 varieties of Chinese origin, 4 varieties of Japanese origin and 6 commercially available cultivars. Five disulphides (dimethyl, allyl methyl, methyl 1-(E)-propenyl, diallyl, and allyl 1-(E)-propenyl), two trisulphides (dimethyl and allyl methyl), and two vinyldithiins (3-vinyl-[4H]-1,2- and 2-vinyl-[4H]-1,3-) were identified on the basis of their mass spectral and GC-retention data. Among the detected sulphur compounds, sulphides with a methyl group predominated over those with an allyl group. This was supported by the HPLC estimations, suggesting that all cultivars examined had much greater amounts of methiin than alliin. Also, two novel compounds were tentatively identified as [3H,4H]-1,2-dithiin and [2H,4H]-1,3-dithiin on the basis of their mass spectral features, GC-retention data, and some experimental results on their formation in reaction mixtures with different proportions of methiin and alliin. Their formation mechanism was proposed. 相似文献
54.
Kazuma Oikawa Kei Toyota Shigeaki Sakatani Yamato Hayashi Hirotsugu Takizawa 《Ceramics International》2019,45(4):4201-4207
In this study, new rGO-silica xerogel nanocomposites (SX-rGO) and its glass fiber reinforced composites (GFR-SX-rGO) were prepared, and its microstructure and thermal properties were evaluated. The raw material was a mixed dispersion prepared by adding 0.01–2.5?wt% of reduced graphene oxide (rGO) to waterglass (6% SiO2). A hydrogel was prepared via sol-gel reaction of this raw material, which was then immersed in hydrochloric acid, hydrophobized in a siloxane/2-propanol reaction system, and then dried at ambient pressure to obtain a hydrophobic carbon-silica xerogel composite. The obtained samples were characterized by N2 physisorption (at 77?K), solid 29Si Magic angle spinning nuclear magnetic resonance spectroscopy, Fourier-transform infrared spectroscopy, Raman spectroscopy, differential scanning calorimetry, thermogravimetric analysis, hydrophobicity, and thermal conductivity. It was found that as the amount of rGO was increased, the specific surface area of the nanocomposite decreased by ~25% from 535 to 403?cm2/g, and the average pore size and pore volume were almost halved. The thermal decomposition temperature of the SX-rGO was increased markedly by the addition of rGO. Moreover, the GFR-SX-rGO-0.5 showed low density (0.208?g/cm3), high contact angle (146°) and low thermal conductivity (0.0199?W/mK). 相似文献
55.
Dr. Aimee J. Marko Mykhaylo Dukh Dr. Nayan J. Patel Joseph R. Missert Prof. Dr. Tymish Ohulchanskyy Walter A. Tabaczynski Dr. Kei Ohkubo Prof. Dr. Shunichi Fukuzumi Prof. Dr. Rutao Yao Prof. Dr. Munawwar Sajjad Prof. Dr. Ravindra K. Pandey 《ChemMedChem》2019,14(16):1503-1513
Herein we report the synthesis, photophysical properties, positron emission tomography (PET) imaging and photodynamic therapy (PDT) efficacy of methyl 3-(1′-m-iodobenzyloxy)ethyl-3-devinyl-verdin 4 (with or without the 124I isotope). The PET imaging ability and ex vivo biodistribution of [124I] 4 were compared with the well-studied methyl [3-(1241′-m-iodobenzyloxy)ethyl]-3-devinyl-pyropheophorbide-a methyl ester (PET-ONCO or [124I] 2 ) and [18F]fluorodeoxyglucose ([18F]FDG) in BALB/c mice bearing colon-26 tumors. Whole-body PET images of [124I] 4 containing a fused methoxy cyclohexenone ring system showed excellent tumor contrast with time (72>48>24 h post-injection). Ex vivo biodistribution results indicate that relative to the current clinical standard [18F]FDG and [124I] 2 in 2 % ethanol formulation, [124I] 4 , at the same radioactive dose (25 μCi per mouse), showed higher tumor uptake at 24 h post-injection and longer tumor retention. In biological environments, compound 4 showed lower fluorescence and lower singlet oxygen yield than 2 , which is possibly due to higher aggregation caused by the presence of a fused cyclohexenone ring system, resulting in limited in vitro/in vivo PDT efficacy. Therefore, the chlorophyll-a analogue [124I] 4 provides easy access to a novel PET imaging agent (with no skin phototoxicity) to image cancer types—brain, renal carcinomas, pancreas—in which [18F]FDG shows limitations. 相似文献
56.
57.
Eiji Takeda Takao Watanabe Shinichiro Kimura Jiro Yugami Keiichi Haraguchi Kei Suzuki Katsuro Sasaki 《Microelectronics Reliability》2000,40(6)
The progress of silicon technology is opening the era of “systems on silicon” in which a large-scale memory, a CPU, and other logic macros will be integrated on a single chip. These kinds of chips, called system LSIs, have an especially promising future in mobile and multimedia applications but face inherent technical problems related to the reliability of ultrathin oxide film, conflict in the processing of different components, increased gate and subthreshold leakage currents, memory bottlenecks, and design complexity. This paper reviews the system LSIs and then introduces related technologies in processing, circuits, chip architecture, and design. It also discusses the influence of the system LSIs on business strategies. 相似文献
58.
Masahide Goto Kei Hagiwara Yoshinori Iguchi Hiroshi Ohtake Takuya Saraya Hiroshi Toshiyoshi Toshiro Hiramoto 《IEEJ Transactions on Electrical and Electronic Engineering》2014,9(3):329-333
We have developed a novel MOSFET that can transfer signals vertically without through‐silicon vias but by using a fully depleted silicon‐on‐insulator (FDSOI) structure with its source region connected to the back electrodes as well as the front ones. A prototype MOSFET fabricated using the backside anisotropic wet etching technique has confirmed that the electrical characteristics measured from the front and the back electrodes are identical. The subthreshold factor S of the prototype was found to be 64.5 mV/decade, suggesting a good switching performance. Since the double‐sided MOSFET has vertical signal‐transfer capability and excellent operating characteristics, it is expected to contribute to developing a More‐than‐Moore type device of three‐dimensional integration such as pixel‐parallel image sensors. © 2014 Institute of Electrical Engineers of Japan. Published by John Wiley & Sons, Inc. 相似文献
59.
Toda K Ohira S Tanaka T Nishimura T Dasgupta PK 《Environmental science & technology》2004,38(5):1529-1536
We describe a membrane-based collection/analysis system that differentially monitors H2S and CH3SH, and to which a conductometric SO2 analyzer using the same collector was coupled. A diffusion scrubber (DS) comprised of a Nafion tube collects H2S selectively while a porous polytetrafluoroethylene (pPTFE) DS collects both H2S and CH3SH. Both gases are measured via their ability to react with fluorescein mercuric acetate (FMA) which results in decreased fluorescence. The limited dynamic range of a negative signal procedure was overcome by using dual DS units comprised of short and long scrubbers, placed serially in the liquid flow line. Different DS designs and membrane materials were investigated. H2S, CH3SH, and SO2 from a biogenic point source were continuously measured, and the H2S/CH3SH data compared well with a standard procedure involving Tedlar bag collection, preconcentration and thermal desorption from a Tenax trap, and measurement by gas chromatography/flame photometric detection. Walkaround portability of the instrument and very large dynamic range measurement of H2S and SO2 were demonstrated around the Mt. Aso volcano. 相似文献
60.
Mixtures of styrene and n-butyl acrylate of various compositions were grafted onto cellulose and cellulose triacetate fibers preirradiated with γ-rays at 0°C in air. Monomer reactivity ratios of the grafted copolymers were found to be different from those of the nongrafted copolymers or those of AIBN-initiated copolymers. The active species initiating the graft copolymerization were trapped radicals for cellulose and peroxides for cellulose triacetate. Kinetic investigations of the graft copolymerization of styrene onto preirradiated cellulose triacetate fibers were also carried out, and it was found that the kinetic scheme for radical polymerization is also applicable to graft copolymerization in a heterogeneous system. 相似文献