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排序方式: 共有3449条查询结果,搜索用时 15 毫秒
61.
62.
Chloride and Indium‐Chloride‐Complex Inorganic Ligands for Efficient Stabilization of Nanocrystals in Solution and Doping of Nanocrystal Solids 下载免费PDF全文
Vladimir Sayevich Chris Guhrenz Maria Sin Volodymyr M. Dzhagan Alexander Weiz Daniel Kasemann Eike Brunner Michael Ruck Dietrich R. T. Zahn Karl Leo Nikolai Gaponik Alexander Eychmüller 《Advanced functional materials》2016,26(13):2163-2175
Here, the surface functionalization of CdSe and CdSe/CdS core/shell nanocrystals (NCs) with compact chloride and indium‐chloride‐complex ligands is reported. The ligands provide not only short interparticle distances but additionally control doping and passivation of surface trap states, leading to enhanced electronic coupling in NC‐based arrays. The solids based on these NCs show an excellent electronic transport behavior after heat treatment at the relatively low temperature of 190 °C. Indeed, the indium‐chlorido‐capped 4.5 nm CdSe NC based thin‐film field‐effect transistor reaches a saturation mobility of μ = 4.1 cm2 (V s)?1 accompanied by a low hysteresis, while retaining the typical features of strongly quantum confined semiconductor NCs. The capping with chloride ions preserves the high photoluminescence quantum yield ( ≈ 66%) of CdSe/CdS core/shell NCs even when the CdS shell is relatively thin (six monolayers). The simplicity of the chemical incorporation of chlorine and indium species via solution ligand exchange, the efficient electronic passivation of the NC surface, as well as their high stability as dispersions make these materials especially attractive for wide‐area solution‐processable fabrication of NC‐based devices. 相似文献
63.
Chelsea M. Phillips Svetlana M. Stamatovic Richard F. Keep Anuska V. Andjelkovic 《International journal of molecular sciences》2022,23(9)
Cerebral cavernous malformation (CCM) is a cerebromicrovascular disease that affects up to 0.5% of the population. Vessel dilation, decreased endothelial cell–cell contact, and loss of junctional complexes lead to loss of brain endothelial barrier integrity and hemorrhagic lesion formation. Leakage of hemorrhagic lesions results in patient symptoms and complications, including seizures, epilepsy, focal headaches, and hemorrhagic stroke. CCMs are classified as sporadic (sCCM) or familial (fCCM), associated with loss-of-function mutations in KRIT1/CCM1, CCM2, and PDCD10/CCM3. Identifying the CCM proteins has thrust the field forward by (1) revealing cellular processes and signaling pathways underlying fCCM pathogenesis, and (2) facilitating the development of animal models to study CCM protein function. CCM animal models range from various murine models to zebrafish models, with each model providing unique insights into CCM lesion development and progression. Additionally, these animal models serve as preclinical models to study therapeutic options for CCM treatment. This review briefly summarizes CCM disease pathology and the molecular functions of the CCM proteins, followed by an in-depth discussion of animal models used to study CCM pathogenesis and developing therapeutics. 相似文献
64.
It has been experimentally demonstrated by Faugère that his F5 algorithm is the fastest algorithm for calculating Gröbner bases. Computational efficiency of F5 is due to not only applying linear algebra but also using the new F5 criterion for revealing useless zero reductions. At the ISSAC 2010 conference, Gao, Guan, and Volny presented G2V, a new version of the F5 algorithm, which is simpler than the original version of the algorithm. However, the incremental structure of G2V used in the algorithm for applying the F5 criterion is a serious obstacle from the point of view of application of Buchberger’s second criterion. In this paper, a modification of the G2V algorithm is presented, which makes it possible to use both Buchberger criteria. To experimentally study computational effect of the proposed modification, we implemented the modified algorithm in Maple. Results of comparison of G2V and its modified version on a number of test examples are presented. 相似文献
65.
66.
In this paper we present an electromagnetism (EM) metaheuristic for solving NP hard Maximum Betweenness Problem (MBP). A new encoding scheme with appropriate objective functions is implemented. Specific representation of the individuals enables the EM operators to explore the searching space in a way that achieves high quality solutions. An effective 1-swap based local search procedure improved by the specific caching technique is performed on each EM point. The algorithm is tested both on real and artificial instances from the literature. Experimental results show that the proposed EM approach achieves all previously known optimal solutions, except one, and achieves the best-known solutions or outperforms other approaches on all large-scale instances, except two. Provided statistical analysis indicates that the EM approach is significantly better than other approaches. 相似文献
67.
Vladimir Ivanovich Lysenko Sergey Bardakhanov Alexey Korchagin Nikolay Kuksanov Alexander Lavrukhin Rustam Salimov Sergey Fadeev Vladislav Cherepkov Mikhail Veis Andrey Nomoev 《Bulletin of Materials Science》2011,34(4):677-681
Electron-beam evaporation of various natural and industrial materials in the atmosphere of different gases at atmospheric pressure can be used for the synthesis of nanosize powders. These powders are characterized by high purity and may exhibit unusual properties. In particular, nanopowders of silicon dioxide and oxide (SiO2, SiO), magnesia (MgO), alumina (Al2O3), titania (TiO2), gadolinium oxide (Gd2O3), various metals (tantalum, molybdenum, nickel, aluminium, copper, silver), semiconductor (Si), nitrides (AlN, TiN), and some other substances had been produced. The process of nanopowder synthesis is highly effective; in particular, the yield of oxides can exceed ten kilograms per hour. 相似文献
68.
Filak LK Mühlgassner G Bacher F Roller A Galanski M Jakupec MA Keppler BK Arion VB 《Organometallics》2011,30(2):273-283
The synthesis of new modified indolo[3,2-c]quinoline ligands L(1)-L(8) with metal-binding sites is reported. By coordination to ruthenium- and osmium-arene moieties 16 complexes of the type [(η(6)-p-cymene)M(L)Cl]Cl (1a,b-8a,b), where M is Ru(II) or Os(II) and L is L(1)-L(8), have been prepared. All compounds were comprehensively characterized by elemental analysis, electrospray ionization mass spectrometry, IR, UV-vis, and NMR spectroscopy, thermogravimetric analysis, and single-crystal X-ray diffraction (2a, 4a, 4b, 5a, 7a, and 7b). The complexes were tested for antiproliferative activity in vitro in three human cancer cell lines, namely, CH1 (ovarian carcinoma), SW480 (colon adenocarcinoma), and A549 (non-small-cell lung cancer), yielding IC(50) values in the submicromolar or low micromolar range. 相似文献
69.
70.
Alexey A. Roenko Vladimir V. Lukin Igor Djurović Xu Zhengguang 《Signal, Image and Video Processing》2009,3(2):157-170
A novel adaptive clipping technique for filtering a constant amplitude frequency modulated (FM) signal embedded in non-Gaussian
noise is proposed. It is based on the analysis and processing of the estimate of probability density function of a FM signal
realization. As a result, modifications of two robust estimators of FM signal amplitude are proposed. It is shown that these
estimators can be used for Gaussian and non-Gaussian heavy-tail environments. The proposed clipping technique can exploit
one or another obtained robust estimate of the signal amplitude for adaptive setting a threshold. Analysis of signal estimate
accuracy for different noise environments is carried out. Comparative analysis of the obtained methods and known approaches
based on scanning window nonlinear filtering and optimal robust L-DFT form is performed. It is demonstrated that the usage
of clipping-based technique leads to the considerable improvement of the FM signal filtering efficiency in comparison to the
aforementioned known approaches for different noise environments and a wide range of input SNR values. 相似文献