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11.
Eric Jorge Thierry Chartier Phillippe Boch 《Journal of the American Ceramic Society》1990,73(8):2552-2554
Ultrasonication is very effective in dispersing alumina and barium titanate slurries. When optimum conditions are used, very short durations (2 to 3 min) are enough to achieve well-dispersed, stable suspensions. 相似文献
12.
This study examines the incorporation of highly unsaturated n−3 fatty acids (HUFA) into triacylglycerols (TAG) of brown adipose
tissue (BAT), and their effect on the positional distribution of saturated (SFA) and of unsaturated (UFA) 16- or 18-carbon
fatty acids. To this end, rats were fed a fish oil diet for up to four weeks. The stereospecific analysis of TAG was based
on generation ofsn-1,2- andsn-2,3-acylglycerols by Grignard degradation, followed by synthesis of phosphatidic acid and specific hydrolysis with phospholipase
A2. From the end of the first week of fish oil feeding, a steady-state in the fatty acid composition of TAG in BAT was reached.
HUFA concentration increased 30-fold, mainly at the expense of n−9 UFA and of SFA. The amount of SFA decreased selectively
at position 3, where these fatty acids were progressively replaced by n−3 HUFA. By contrast, the amount of UFA decreased at
all positions, and their positional distribution was not affected. About 60% of HUFA was incorporated at position 3. Nearly
twice as much 22∶6n−3 was incorporated into TAG than had been previously observed in white adipose tissue (WAT) [Leray, C.,
Raclot, T., and Groscolas, R. (1993)Lipids 28, 279–284]. At the steady-state, the distribution of HUFA was characterized by high proportions of 22∶6n−3 and 20∶5n−3 in
position 3. Moreover, in each position of TAG, a steady level was reached rapidly (within 1 wk). It is concluded that, during
fish-oil feeding, fatty acids in TAG of BAT show characteristic time-course changes that lead to a characteristic composition
and a tissue-specific positional distribution. This suggests that adipose tissue has its own specificity in controlling the
build-up of TAG stores, which is likely to be regulated by the specificity of acylating enzymes as well as molecular rearrangements. 相似文献
13.
We present dynamic studies of surface reactions using video-Field Ion Microscopy (FIM) along with Pulsed Field Desorption
Mass Spectrometry (PFDMS). Catalytic water formation is followed using rhodium and platinum 3D field emitter crystals for
the oxidation of hydrogen with either oxygen (Rh) or NO (Pt). Strongly non-linear dynamics are observed with nanoscale spacial
resolution. For both reactions quasi-oscillatory behaviour exists under certain conditions of temperatures and partial pressures.
An influence of the probing electric field is observed and possibly essential in establishing oscillatory behaviour. Local
chemical probing of selected surface areas with up to 400 atomic surface sites proves catalytic water formation to take place.
Since water ions (H2O+/H3O+) cause image formation of the O2–H2 reaction on Rh, respective videos provide space-time resolved information on the catalytically active sites. Atom-probe data
also reveal that the surface of the Rh sample reversibly switches from a metallic to an oxidized state during oscillations.
As to the NO–H2 reaction on Pt, fast ignition phenomena are observed to precede wave fronts. After catalytic water formation, NO molecules
diffuse into emptied areas and cause high image brightness. Depending on the size of the Pt crystal, the reaction may ignite
in planes or kinked ledges along the <100> zone lines. Thus FIM provides clear experimental evidence that kinks are more reactive
than steps in the catalytic NO + H2 reaction. Pt surface oxidation occurs and has probably been underestimated in previous FIM studies. 相似文献
14.
Alain Le Mehaute Gilles Crepy Georges Marcellin Thierry Hamaide Alain Guyot 《Polymer Bulletin》1985,14(3-4):233-237
Summary The room temperature conductivity of lithium salts dissolved in polyethylene oxide, proposed as polymer electrolytes, is shown to decrease drastically upon storage. The crystallization process, which is responsible for that ageing, can be blocked, if two further components are added : an elastomer copolymer butadiene-acrylonitrile and a macromer of polyoxyethylene. In addition, a crosslinking process must be carried out. 相似文献
15.
Adam Jacobson Fan Zeng David Smith Nigel Boswell Thierry Peynot Michael Milford 《野外机器人技术杂志》2021,38(1):5-27
Robustly and accurately localizing vehicles in underground mines is particularly challenging due to the unavailability of GPS, variable and often poor lighting conditions, visual aliasing in long tunnels, and airborne dust and water. In this paper, we present a novel, infrastructure‐less, multisensor localization method for robust autonomous operation within underground mines. The proposed method integrates with existing mine site commissioning and operation procedures and includes both an offline map‐building process and an online localization algorithm. The approach combines the strengths of visual‐based place recognition, LIDAR‐based localization, and odometry in a particle filter fusion process. We provide an extensive experimental validation using new large data sets acquired in two operational Australian underground hard‐rock mines (including a 600m‐deep multilevel mine with approximately 33 km of mapping data and 7 km of vehicle localization) by actual mining vehicles during production operations. We demonstrate a significant increase in localization accuracy over prior state‐of‐the‐art SLAM research systems and real‐time operation, with processing times in the order of 10 Hz. We present results showing a mean error of 0.68 m from the Queensland Mine data set and 1.32 m from the New South Wales Mine data set and at least 86% reduction in error compared with prior state of the art. We also analyze the impact of the particle filter parameters with respect to localization accuracy. Together this study represents a new approach to positioning systems for currently deployed autonomous vehicles within underground mine environments. 相似文献
16.
Hamza El Marouazi Benoit van der Schueren Damien Favier Anaëlle Bolley Samuel Dagorne Thierry Dintzer Izabela Janowska 《应用聚合物科学杂志》2021,138(44):51300
Four series of polylactide (PLA) based composite films containing horizontally aligned few layer graphene (FLG) flakes of high aspect ratio and adsorbed albumin are prepared. The mechanical and thermal properties varies with percentage, dispersion degree and size of FLG flakes. Great improvement up to 290% and 360% of tensile modulus and strength respectively were obtained for the composite containing high lateral size of FLG at 0.17% wt, and up to 60% and 80% for the composite with very well dispersed 0.02% wt FLG. The composites of PLA and PEG-PLLA containing very well dispersed FLG flakes at 0.07% wt are ductile showing enhancement of elongation at break up to respectively 80% and 88%. Relatively high electrical conductivity, 5 × 10−3 S/cm, is measured for PLA film charged with 3% of FLG. 相似文献
17.
Mechanisms of nanostructure and metastable phase formations in the surface melted layers of a HCPEB-treated D2 steel 总被引:1,自引:0,他引:1
This work investigates the mechanism of surface modification associated with the high-current pulsed electron beam (HCPEB) treatment of a D2 steel with increasing numbers of pulses. The surface layers were melted and resolidified but the treated surfaces showed very different features. This variation is essentially due to the different levels of homogeneity and carbide dissolution. It is demonstrated that the presence of carbides served as nucleation sites for the surface eruption phenomenon that creates craters on the surface. After a sufficient number of pulses, most of the carbides in the surface layer were dissolved and an almost crater-free homogeneous melted layer consisting of a very stable nano-austenite structure was formed. The HCPEB technique is thus demonstrated to be a versatile technique for surface microstructure modification involving, in the case of steels, austenite stabilization and ultrafine grain formation. 相似文献
18.
Terrain traversability estimation is a fundamental requirement to ensure the safety of autonomous planetary rovers and their ability to conduct long‐term missions. This paper addresses two fundamental challenges for terrain traversability estimation techniques. First, representations of terrain data, which are typically built by the rover's onboard exteroceptive sensors, are often incomplete due to occlusions and sensor limitations. Second, during terrain traversal, the rover‐terrain interaction can cause terrain deformation, which may significantly alter the difficulty of traversal. We propose a novel approach built on Gaussian process (GP) regression to learn, and consequently to predict, the rover's attitude and chassis configuration on unstructured terrain using terrain geometry information only. First, given incomplete terrain data, we make an initial prediction under the assumption that the terrain is rigid, using a learnt kernel function. Then, we refine this initial estimate to account for the effects of potential terrain deformation, using a near‐to‐far learning approach based on multitask GP regression. We present an extensive experimental validation of the proposed approach on terrain that is mostly rocky and whose geometry changes as a result of loads from rover traversals. This demonstrates the ability of the proposed approach to accurately predict the rover's attitude and configuration in partially occluded and deformable terrain. 相似文献
19.
Flow profile measurement in microchannel using the optical feedback interferometry sensing technique 总被引:1,自引:1,他引:0
Lucie Campagnolo Milan Nikolić Julien Perchoux Yah Leng Lim Karl Bertling Karine Loubière Laurent Prat Aleksandar D. Rakić Thierry Bosch 《Microfluidics and nanofluidics》2013,14(1-2):113-119
The need to accurately measure flow profiles in microfluidic channels is well recognised. In this work, we present a new optical feedback interferometry (OFI) flow sensor that accurately measures local velocity in fluids and enables reconstruction of a velocity profile inside a microchannel. OFI is a self-aligned interferometric technique that uses the laser as both the transmitter and the receiver thus offering high sensitivity, fast response, and a simple and compact optical design. The system described here is based on a commercial semiconductor laser and has been designed to achieve a micrometer-range spatial resolution. The sensor performance was validated by reconstructing the velocity profile inside a circular cross-section flow-channel with 320 $\upmu $ m internal diameter, with a relative error smaller than 1.8 %. The local flow velocity is directly measured, thus avoiding the need for model based profile calculation and uncertainties inherent to this approach. The system was validated by successfully extracting the flow profiles in both Newtonian and shear-thinning liquids. 相似文献
20.
Tao Wang Daming Zheng Karol Vegso Nada Mrkyvkova Peter Siffalovic Thierry Pauporté 《Advanced functional materials》2023,33(43):2304659
The development of an efficient fabrication route to achieve high-resolution perovskite pixel array is key for large-scale flexible image sensor devices. Herein, a high-resolution and stable 10 × 10 flexible PDs array based on formamidinium(FA+) and phenylmethylammonium (PMA+) quasi-2D (PMA)2FAPb2I7 (n = 2) perovskite is demonstrated by developing SiO2-assisted hydrophobic and hydrophilic treatment process on polyethylene terephthalate substrate. By introducing Au nanoparticles (Au NPs), the perovskite film quality is improved and grain boundaries are reduced. The mechanism by which Au NPs upgrade the photoelectric quality of perovskite is mainly revealed by glow discharge-optical emission spectroscopy (GD-OES) and grazing-incidence wide-angle X-ray scattering (GIWAXS). To further improve the photoelectric performance of the devices, a post-treatment strategy with formamidinium chloride (FACl) is used . The optimized flexible PDs arrays show excellent optoelectronic properties with a high responsivity of 4.7 A W−1, a detectivity of 6.3 × 1012 Jones, and a broad spectral sensitivity. The device also exhibits excellent electrical stability even under severe bending and excellent flexural strength, as well as excellent environmental stability. Finally, the integrated flexible PDs arrays are used as sensor pixels in an imaging system to obtain high-resolution imaging patterns, demonstrating the imaging capability of the PDs arrays. 相似文献