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61.
Highly Conductive,Air‐Stable Silver Nanowire@Iongel Composite Films toward Flexible Transparent Electrodes 下载免费PDF全文
62.
63.
Xiaojian?Liu Zhen?Zheng Chunqing?WangEmail author Wei?Liu Lingchao?Kong 《Journal of Materials Science: Materials in Electronics》2016,27(10):10065-10069
Ultrafine Ag–Cu nanoparticles (NPs) have been synthesized by a rapid one-step reduction within only 10 min. Effects of temperature and dispersants on the phases and morphology of Ag–Cu NPs were investigated. Results showed that citric acid exhibited an advantageous nature to avoid the formation of Cu2O and form uniform morphology over PVP. The average particle size of the Ag–Cu NPs synthesized simply in ice-cubes bath could be controlled in 8.6 nm about a quarter of that synthesized at room temperature. The synthesized Ag–Cu NPs presented alloy states near the eutectic composition of 72:28. Due to the lower Ostwald ripening rate and citric acid protection, smaller Ag–Cu NPs were achieved in ice-cube bath. Results also showed that the ultrafine Ag–Cu NPs could be expected to sinter at about 330 °C which was much lower than the eutectic temperature (779 °C) of bulk Ag–Cu alloy. The ultrafine Ag–Cu NPs could be applied as potential die attach materials for SiC power devices. 相似文献
64.
Yuxia Kong Jigong Hao Dan Xu 《Journal of Materials Science: Materials in Electronics》2016,27(11):11256-11261
High aspect ratio patelike NaNbO3 particles with pure perovskite structure have been successfully synthesized by topochemical microcrystal conversion (TMC) from plate-like precursor particles of the layer-structured Bi2.5Na3.5Nb5O18. By changing the Bi2.5Na3.5Nb5O18/Na2CO3 ratio, large and thin NaNbO3 particles with a thickness of approximately 0.5 μm and a width of approximately 20 μm were obtained. The obtained NaNbO3 particles is quite suitable for fabricating textured (K0.5Na0.5)NbO3-based ceramics. Using the fine platelike NaNbO3 particles as templates, dense <001> -oriented (K0.5Na0.5)NbO3-0.5 mol %MnO2 ceramics with high texture quality (Lotgering factor F 001 = 87 %) and excellent piezoelectric properties were produced by templated grain growth. Compared with randomly oriented ceramics, textured samples show greatly enhanced properties. The room-temperature strain S, the piezoelectric coefficient d 33 * and d 33 reach up to 0.093 %, 233 pm/V and 195pC/N, respectively, which are all about 1.5 times larger than those of non-textured ceramics. 相似文献
65.
Monitoring the Dynamic Process of Formation of Plasmonic Molecular Junctions during Single Nanoparticle Collisions 下载免费PDF全文
Jing Guo Jie Pan Shuai Chang Xuewen Wang Na Kong Wenrong Yang Jin He 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(15)
The capability to study the dynamic formation of plasmonic molecular junction is of fundamental importance, and it will provide new insights into molecular electronics/plasmonics, single‐entity electrochemistry, and nanooptoelectronics. Here, a facile method to form plasmonic molecular junctions is reported by utilizing single gold nanoparticle (NP) collision events at a highly curved gold nanoelectrode modified with a self‐assembled monolayer. By using time‐resolved electrochemical current measurement and surface‐enhanced Raman scattering spectroscopy, the current changes and the evolution of interfacial chemical bonding are successfully observed in the newly formed molecular tunnel junctions during and after the gold NP “hit‐n‐stay” and “hit‐n‐run” collision events. The results lead to an in‐depth understanding of the single NP motion and the associated molecular level changes during the formation of the plasmonic molecular junctions in a single NP collision event. This method also provides a new platform to study molecular changes at the single molecule level during electron transport in a dynamic molecular tunnel junction. 相似文献
66.
Imparting Designer Biorecognition Functionality to Metal–Organic Frameworks by a DNA‐Mediated Surface Engineering Strategy 下载免费PDF全文
Weiyu Ning Zhenghan Di Yingjie Yu Pingmei Zeng Chunzhi Di Daquan Chen Xueqian Kong Guangjun Nie Yuliang Zhao Lele Li 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(11)
Surface functionality is an essential component for processing and application of metal–organic frameworks (MOFs). A simple and cost‐effective strategy for DNA‐mediated surface engineering of zirconium‐based nanoscale MOFs (NMOFs) is presented, capable of endowing them with specific molecular recognition properties and thus expanding their potential for applications in nanotechnology and biotechnology. It is shown that efficient immobilization of functional DNA on NMOFs can be achieved via surface coordination chemistry. With this strategy, it is demonstrated that such porphyrin‐based NMOFs can be modified with a DNA aptamer for targeting specific cancer cells. Furthermore, the DNA–NMOFs can facilitate the delivery of therapeutic DNA (e.g., CpG) into cells for efficient recognition of endosomal Toll‐like receptor 9 and subsequent enhanced immunostimulatory activity in vitro and in vivo. No apparent toxicity is observed with systemic delivery of the DNA–NMOFs in vivo. Overall, these results suggest that the strategy allows for surface functionalization of MOFs with different functional DNAs, extending the use of these materials to diverse applications in biosensor, bioimaging, and nanomedicine. 相似文献
67.
Yi-Chao Zou Zhi-Gang Chen Enze Zhang Fantai Kong Yan Lu Lihua Wang John Drennan Zhongchang Wang Faxian Xiu Kyeongjae Cho Jin Zou 《Nano Research》2018,11(2):696-706
Identification of atomic disorders and their subsequent control has proven to be a key issue in predicting, understanding, and enhancing the properties of newly emerging topological insulator materials. Here, we demonstrate direct evidence of the cation antisites in single-crystal SnBi2Te4 nanoplates grown by chemical vapor deposition, through a combination of sub-ångström-resolution imaging, quantitative image simulations, and density functional theory calculations. The results of these combined techniques revealed a recognizable amount of cation antisites between Bi and Sn, and energetic calculations revealed that such cation antisites have a low formation energy. The impact of the cation antisites was also investigated by electronic structure calculations together with transport measurement. The topological surface properties of the nanoplates were further probed by angle-dependent magnetotransport, and from the results, we observed a two-dimensional weak antilocalization effect associated with surface carriers. Our approach provides a pathway to identify the antisite defects in ternary chalcogenides and the application potential of SnBi2Te4 nanostructures in next-generation electronic and spintronic devices. 相似文献
68.
In this paper, the axial-flux permanent magnet driver is modeled and analyzed in a simple and novel way under three-dimensional cylindrical coordinates. The inherent three-dimensional characteristics of the device are comprehensively considered, and the governing equations are solved by simplifying the boundary conditions. The axial magnetization of the sector-shaped permanent magnets is accurately described in an algebraic form by the parameters, which makes the physical meaning more explicit than the purely mathematical expression in general series forms. The parameters of the Bessel function are determined simply and the magnetic field distribution of permanent magnets and the air-gap is solved. Furthermore, the field solutions are completely analytical, which provides convenience and satisfactory accuracy for modeling a series of electromagnetic performance parameters, such as the axial electromagnetic force density, axial electromagnetic force, and electromagnetic torque. The correctness and accuracy of the analytical models are fully verified by three-dimensional finite element simulations and a 15 kW prototype and the results of calculations, simulations, and experiments under three methods are highly consistent. The influence of several design parameters on magnetic field distribution and performance is studied and discussed. The results indicate that the modeling method proposed in this paper can calculate the magnetic field distribution and performance accurately and rapidly, which affords an important reference for the design and optimization of axial-flux permanent magnet drivers. 相似文献
69.
Highly efficient, widely tunable, 10-Hz parametric amplifier pumped by frequency-doubled femtosecond Ti:sapphire laser pulses 总被引:5,自引:0,他引:5
We report a 10-Hz, highly efficient, widely tunable (from the visible to the IR), broadband femtosecond optical parametric generator and optical parametric amplifier (OPA) in BBO, LBO, and CBO crystals pumped by the frequency-doubled output of a regeneratively amplified Ti:sapphire laser at 400 nm. The output of the system is continuously tunable from 440 nm to 2.5 mum with a maximum overall efficiency of ~25% at 670 nm and an optical conversion efficiency of more than 36% in the OPA stage. The effects of the seed beam energy, the type of the crystal and the crystal length, and the pumping energy of the output of the OPA, such as the optical efficiency, the bandwidth, the pulse duration, and the group velocity mismatch between the signal and the idler and between the seeder and the pump, are investigated. The results provide useful information for optimization of the design of the system. 相似文献
70.
An efficient microfluidic sorter: implementation of double meandering micro striplines for magnetic particles switching 总被引:1,自引:1,他引:0
Tian Fook Kong Huan Shin E Hendrik Santoso Sugiarto Hwi Fen Liew Xinghua Wang Wen Siang Lew Nam-Trung Nguyen Yong Chen 《Microfluidics and nanofluidics》2011,10(5):1069-1078
The ability to trap, manipulate, and separate magnetic beads has become one of the key requirements in realizing an integrated
magnetic lab-on-chip biosensing system. In this article, we present the design and fabrication of an integrated magneto-fluidic
device for sorting magnetic particles with a sorting efficiency of up to 95%. The actuation and manipulation of magnetic beads
are realized using microfabricated square meandering current-carrying micro striplines. The current is alternated between
two neighboring micro striplines to switch the magnetic beads to either one of the two outlets. We performed a series of parametric
study to investigate the effect of applied current, flow rate, and switching frequency on the sorting efficiency. Experimental
results reveal that the sorting efficiency is proportional to the square of current applied to the stripline, and decreases
with increasing buffer flow rate and switching frequency. Such phenomena agree well with our theoretical analysis and simulation
result. The fastest switching rate, which is limited by the microchannel geometry and bead velocity, is 2 Hz. 相似文献