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111.
Correlation between ionic conductivity and fluidity of polymer gel electrolytes containing NH4CF3SO3
Nonaqueous polymer gel electrolytes containing ammonium triflate (NH4CF3SO3) and dimethylacetamide (DMA) with polymethylmethacrylate (PMMA) as the gelling polymer have been synthesized which show high
value of conductivity (~ 10-2 S/cm) at 25°C. The conductivity of polymer gel electrolytes containing different concentrations of NH4CF3SO3 shows a small decrease with the addition of PMMA and this has been correlated with the variation of fluidity of these gel
electrolytes. The small decrease in conductivity with PMMA addition shows that polymer plays the role of stiffener and this
is supported by FTIR results which also indicates the absence of any active interaction between polymer and NH4CF3SO3 in these gel electrolytes. 相似文献
112.
113.
A methodology is described for evolving a Rough-fuzzy multi layer perceptron with modular concept using a genetic algorithm to obtain a structured network suitable for both classification and rule extraction. The modular concept, based on "divide and conquer" strategy, provides accelerated training and a compact network suitable for generating a minimum number of rules with high certainty values. The concept of variable mutation operator is introduced for preserving the localized structure of the constituting knowledge-based subnetworks, while they are integrated and evolved. Rough set dependency rules are generated directly from the real valued attribute table containing fuzzy membership values. Two new indices viz., "certainty" and "confusion" in a decision are defined for evaluating quantitatively the quality of rules. The effectiveness of the model and the rule extraction algorithm is extensively demonstrated through experiments alongwith comparisons. 相似文献
114.
Konark: A system and protocols for device independent, peer-to-peer discovery and delivery of mobile services 总被引:1,自引:0,他引:1
115.
Incorporating Ancestors' Influence in Genetic Algorithms 总被引:1,自引:1,他引:1
A new criterion of fitness evaluation for Genetic Algorithms is introduced where the fitness value of an individual is determined by considering its own fitness as well as those of its ancestors. Some guidelines for selecting the weighting coefficients for quantifying the importance to be given to the fitness of the individual and its ancestors are provided. This is done both heuristically and automatically under fixed and adaptive frameworks. The Schema Theorem corresponding to the proposed concept is derived. The effectiveness of this new methodology is demonstrated extensively on the problems of optimizing complex functions including a noisy one and selecting optimal neural network parameters. 相似文献
116.
Some new indexes of cluster validity 总被引:18,自引:0,他引:18
Bezdek J.C. Pal N.R. 《IEEE transactions on systems, man, and cybernetics. Part B, Cybernetics》1998,28(3):301-315
We review two clustering algorithms (hard c-means and single linkage) and three indexes of crisp cluster validity (Hubert's statistics, the Davies-Bouldin index, and Dunn's index). We illustrate two deficiencies of Dunn's index which make it overly sensitive to noisy clusters and propose several generalizations of it that are not as brittle to outliers in the clusters. Our numerical examples show that the standard measure of interset distance (the minimum distance between points in a pair of sets) is the worst (least reliable) measure upon which to base cluster validation indexes when the clusters are expected to form volumetric clouds. Experimental results also suggest that intercluster separation plays a more important role in cluster validation than cluster diameter. Our simulations show that while Dunn's original index has operational flaws, the concept it embodies provides a rich paradigm for validation of partitions that have cloud-like clusters. Five of our generalized Dunn's indexes provide the best validation results for the simulations presented. 相似文献
117.
Though the application of bimetallic nanoparticles is becoming increasingly important, the local atomistic structure of such alloyed particles, which is critical for tailoring their properties, is not yet very clearly understood. In this work, we present detailed study on the atomistic structure of Au-Cu nanoparticles so as to determine their most stable configurations and the conditions for obtaining clusters of different structural variants. The dynamic behavior of these nanoparticles upon local heating is investigated. AuCu nanoparticles are characterized by high resolution transmission electron microscopy (HRTEM) and energy filtering elemental composition mapping (EFECM), which allowed us to study the internal structure and the elemental distribution in the particles. Quantum mechanical approaches and classic molecular dynamics methods are applied to model the structure and to determine the lowest energy configurations, the corresponding electronic structures, and understand structural transition of clusters upon heating, supported by experimental evidences. Our theoretical results demonstrate only the core/shell bimetallic structure have negative heat of formation, both for decahedra and octahedral, and energetically favoring core/shell structure is with Au covering the core of Cu, whose reverse core/shell structure is not stable and may transform back at a certain temperature. Experimental evidences corroborate these structures and their structural changes upon heating, demonstrating the possibility to manipulate the structure of such bimetallic nanoparticles using extra stimulating energy, which is in accordance with the calculated coherence energy proportions between the different configurations. 相似文献
118.
Shukla R Banerjee P Sharma SK Das R Deb P Prabaharan T Das B Adhikary B Verma R Shyam A 《The Review of scientific instruments》2011,82(10):106103
The experimental results of an air-core pulse transformer are presented, which is very compact (<10 Kg in weight) and is primed by a capacitor bank that is fabricated in such a way that the capacitor bank with its switch takes the shape of single-turn rectangular shaped primary of the transformer. A high voltage capacitor assembly (pulse-forming-line capacitor, PFL) of 5.1 nF is connected with the secondary of transformer. The transformer output voltage is 160 kV in its second peak appearing in less than 2 μS from the beginning of the capacitor discharge. The primary capacitor bank can be charged up to a maximum of 18 kV, with the voltage delivery of 360 kV in similar capacitive loads. 相似文献
119.
Effect of shielding gas mixture on gas metal arc welding of HSLA steel using solid and flux-cored wires 总被引:1,自引:0,他引:1
S. Mukhopadhyay T.K. Pal 《The International Journal of Advanced Manufacturing Technology》2006,29(3-4):262-268
In this work, gas metal arc welding of high strength-low alloy (HSLA) steel with solid- and flux-cored arc welding wires using
different shielding gas compositions was performed. The composition of filler wire and shielding gas in gas metal arc welds
of HSLA steel determines the inclusion characteristics, microstructure and mechanical properties. Thus, acceptable weld metal
properties in HSLA steel using gas metal arc welding (GMAW) process could be achieved with the proper combination of filler
wire and shielding gas composition. 相似文献
120.
Ayesh Madushanka Niraj Verma Marek Freindorf Elfi Kraka 《International journal of molecular sciences》2022,23(20)
Dengue fever (DF), dengue hemorrhagic fever (DHF), and dengue shock syndrome (DSS) cause serious public health problems, with nearly 390 million people affected and 20,000 deaths per year in tropical and subtropical countries. Despite numerous attempts, no antiviral drug or vaccine is currently available to combat the manifestation. The challenge of discovering an efficient vaccine is enhanced by the surplus presence of efficient vectors and drug resistance from the virus. For centuries, papaya (Carica papaya) extracts have been traditionally used to treat DF, DHF, and DSS. In the present study, we systematically investigated seven compounds isolated from papaya leaf extract with regard to their potential as inhibitors for non-structural (NS) proteins, NS3 and NS5, which play a crucial role in viral RNA replication. The computational tools applied stretched across classical molecular docking, molecular dynamics (MD) simulations and SwissADME used to calculate binding affinities; binding free energies; Absorption, Distribution, Metabolism, and Excretion (ADME); and drug-likeness properties, thus, identifying Kaempferol, Chlorogenic acid, and Quercetin as potential candidates, with Kaempferol and Quercetin scoring best. Therefore, for the Kaempferol and Quercetin complexes, hybrid quantum mechanical/molecular mechanical (QM/MM) geometry and frequency calculations were performed, followed by the local mode analysis developed in our group to quantify Kaempferol-NS and Quercetin-NS hydrogen bonding. Given the non-toxic nature and the wide availability of the Kaempferol and Quercetin papaya extract in almost all of the susceptible regions, and our results showing high NS3 and NS5 binding affinities and energies, strong hydrogen bonding with both NS3 and NS5, and excellent ADME properties, we suggest Kaempferol and Quercetin as a strong NS3 and NS5 inhibitor to be further investigated in vitro. 相似文献