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71.
Silvia G. Motti Manuel Kober-Czerny Marcello Righetto Philippe Holzhey Joel Smith Hans Kraus Henry J. Snaith Michael B. Johnston Laura M. Herz 《Advanced functional materials》2023,33(32):2300363
Metal halide perovskite (MHP) semiconductors have driven a revolution in optoelectronic technologies over the last decade, in particular for high-efficiency photovoltaic applications. Low-dimensional MHPs presenting electronic confinement have promising additional prospects in light emission and quantum technologies. However, the optimisation of such applications requires a comprehensive understanding of the nature of charge carriers and their transport mechanisms. This study employs a combination of ultrafast optical and terahertz spectroscopy to investigate phonon energies, charge-carrier mobilities, and exciton formation in 2D (PEA)2PbI4 and (BA)2PbI4 (where PEA is phenylethylammonium and BA is butylammonium). Temperature-dependent measurements of free charge-carrier mobilities reveal band transport in these strongly confined semiconductors, with surprisingly high in-plane mobilities. Enhanced charge-phonon coupling is shown to reduce charge-carrier mobilities in (BA)2PbI4 with respect to (PEA)2PbI4. Exciton and free charge-carrier dynamics are disentangled by simultaneous monitoring of transient absorption and THz photoconductivity. A sustained free charge-carrier population is observed, surpassing the Saha equation predictions even at low temperature. These findings provide new insights into the temperature-dependent interplay of exciton and free-carrier populations in 2D MHPs. Furthermore, such sustained free charge-carrier population and high mobilities demonstrate the potential of these semiconductors for applications such as solar cells, transistors, and electrically driven light sources. 相似文献
72.
Sunny Chilankamol Das Satyajit Martin Kevin J. M. Coussy Philippe 《Journal of Signal Processing Systems》2022,94(9):895-912
Journal of Signal Processing Systems - Research interest and industry investment in edge computing solutions have increased dramatically in recent years. Consequent quest for balanced performance,... 相似文献
73.
Koen Nickmans Gerardus M. Bögels Carlos Sánchez‐Somolinos Jeffrey N. Murphy Philippe Leclère Ilja K. Voets Albertus P. H. J. Schenning 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(33)
While self‐assembled molecular building blocks could lead to many next‐generation functional organic nanomaterials, control over the thin‐film morphologies to yield monolithic sub‐5 nm patterns with 3D orientational control at macroscopic length scales remains a grand challenge. A series of photoresponsive hybrid oligo(dimethylsiloxane) liquid crystals that form periodic cylindrical nanostructures with periodicities between 3.8 and 5.1 nm is studied. The liquid crystals can be aligned in‐plane by exposure to actinic linearly polarized light and out‐of‐plane by exposure to actinic unpolarized light. The photoalignment is most efficient when performed just under the clearing point of the liquid crystal, at which the cylindrical nanostructures are reoriented within minutes. These results allow the generation of highly ordered sub‐5 nm patterns in thin films at macroscopic length scales, with control over the orientation in a noncontact fashion. 相似文献
74.
Berg Alexander Caroff Philippe Shahid Naeem Lockrey Mark N. Yuan Xiaoming Borgström Magnus T. Tan Hark Hoe Jagadish Chennupati 《Nano Research》2017,10(2):672-682
Ternary Ⅲ-Ⅴ nanowires (NWs) cover a wide range of wavelengths in the solar spectrum and would greatly benefit from being synthesized as position-controlled arrays for improved vertical yield,reprodudbility,and tunable optical absorption.Here,we report on successful selective-area epitaxy of metal-particle-free vertical InxGa1-xP NW arrays using metal-organic vapor phase epitaxy and detail their optical properties.A systematic growth study establishes the range of suitable growth parameters to obtain uniform NW growth over a large array.The optical properties of the NWs were characterized by room-temperature cathodoluminescence spectroscopy.Tunability of the emission wavelength from 870 nm to approximately 800 nm was achieved.Transmission electron microscopy and energy dispersive X-ray measurements performed on crosssection samples revealed a pure wurtzite crystal structure with very few stacking faults and a slight composition gradient along the NW growth axis. 相似文献
75.
76.
Athanasios C. Rakitzis Petros E. Maravelakis Philippe Castagliola 《Quality and Reliability Engineering International》2016,32(2):465-483
Zero‐inflated probability models are used to model count data that have an excessive number of zeros. These models are mostly useful in modeling high‐yield or health‐related processes. The zero‐inflated binomial distribution is an extension of the ordinary binomial distribution that takes into account the excess of zeros. In this paper, one‐sided cumulative sum (CUSUM)‐type control charts are proposed for monitoring increases or decreases in the parameter p of a zero‐inflated binomial process. The results of an extensive numerical study concerning the statistical design of the proposed schemes as well as their practical implementation are provided. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
77.
Kim Phuc Tran Philippe Castagliola Giovanni Celano 《Quality and Reliability Engineering International》2016,32(5):1853-1869
In many fields, there is the need to monitor quality characteristics defined as the ratio of two random variables. The design and implementation of control charts directly monitoring the ratio stability is required for the continuous surveillance of these quality characteristics. In this paper, we propose two one‐sided exponentially weighted moving average (EWMA) charts with subgroups having sample size n > 1 to monitor the ratio of two normal random variables. The optimal EWMA smoothing constants, control limits, and ARLs have been computed for different values of the in‐control ratio and correlation between the variables and are shown in several figures and tables to discuss the statistical performance of the proposed one‐sided EWMA charts. Both deterministic and random shift sizes have been considered to test the two one‐sided EWMA charts' sensitivity. The obtained results show that the proposed one‐sided EWMA control charts are more sensitive to process shifts than other charts already proposed in the literature. The practical application of the proposed control schemes is discussed with an illustrative example. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
78.
Huay Woon You Michael B. C. Khoo Philippe Castagliola Abdul Haq 《Quality and Reliability Engineering International》2016,32(5):1913-1927
Many quality characteristics have means and standard deviations that are not independent. Instead, the standard deviations of these quality characteristics are proportional to their corresponding means. Thus, monitoring the coefficient of variation (CV), for these quality characteristics, using a control chart has gained remarkable attention in recent years. This paper presents a side sensitive group runs chart for the CV (called the SSGR CV chart). The implementation and optimization procedures of the proposed chart are presented. Two optimization procedures are developed, i.e. (i) by minimizing the average run length (ARL) when the shift size is deterministic and (ii) by minimizing the expected average run length (EARL) when the shift size is unknown. An application of the SSGR CV chart using a real dataset is also demonstrated. Additionally, the SSGR CV chart is compared with the Shewhart CV, runs rules CV, synthetic CV and exponentially weighted moving average CV charts by means of ARLs and standard deviation of the run lengths. The performance comparison is also conducted using EARLs when the shift size is unknown. In general, the SSGR CV chart surpasses the other charts under comparison, for most upward and downward CV shifts. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
79.
Athanasios C. Rakitzis Philippe Castagliola Petros E. Maravelakis 《Quality and Reliability Engineering International》2016,32(5):1837-1851
In this work, we propose and study general inflated probability distributions that can be used for modelling and monitoring unusual count data. The considered models extend the well‐known zero‐inflated Poisson distribution because they allow the excess of values, other than zero. Four simple upper‐sided control schemes are considered for the monitoring of count data based on the proposed general inflated Poisson distributions, and their performance is evaluated under various out‐of‐control situations. The usefulness of the considered models and techniques is illustrated via two real‐data examples, while practical guidelines are provided as well. Copyright © 2015 John Wiley & Sons, Ltd. 相似文献
80.
Microfluidic Manipulation of Core/Shell Nanoparticles for Oral Delivery of Chemotherapeutics: A New Treatment Approach for Colorectal Cancer
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Mohammad Mahdi Hasani‐Sadrabadi Shahrouz Taranejoo Erfan Dashtimoghadam Ghasem Bahlakeh Fatemeh Sadat Majedi Jules John VanDersarl Mohsen Janmaleki Fatemeh Sharifi Arnaud Bertsch Kerry Hourigan Lobat Tayebi Philippe Renaud Karl I. Jacob 《Advanced materials (Deerfield Beach, Fla.)》2016,28(21):4134-4141