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101.
Monitoring the Dynamic Process of Formation of Plasmonic Molecular Junctions during Single Nanoparticle Collisions 下载免费PDF全文
Jing Guo Jie Pan Shuai Chang Xuewen Wang Na Kong Wenrong Yang Jin He 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(15)
The capability to study the dynamic formation of plasmonic molecular junction is of fundamental importance, and it will provide new insights into molecular electronics/plasmonics, single‐entity electrochemistry, and nanooptoelectronics. Here, a facile method to form plasmonic molecular junctions is reported by utilizing single gold nanoparticle (NP) collision events at a highly curved gold nanoelectrode modified with a self‐assembled monolayer. By using time‐resolved electrochemical current measurement and surface‐enhanced Raman scattering spectroscopy, the current changes and the evolution of interfacial chemical bonding are successfully observed in the newly formed molecular tunnel junctions during and after the gold NP “hit‐n‐stay” and “hit‐n‐run” collision events. The results lead to an in‐depth understanding of the single NP motion and the associated molecular level changes during the formation of the plasmonic molecular junctions in a single NP collision event. This method also provides a new platform to study molecular changes at the single molecule level during electron transport in a dynamic molecular tunnel junction. 相似文献
102.
103.
To make health care more responsive to patient needs, insight into patient priorities is needed. A systematic literature review, using electronic and manual searches, was made of studies on patient priorities with regard to primary health care. Data-extraction was performed by two researchers, followed by systematic analyses of study features. 57 studies were included. The aspects of care and methods used showed a wide variation. Aspects most often included were "informativeness", "humaneness" and "competence/accuracy". Based on an analysis of 19 studies, the following aspects were seen by patients as most important in more than 50% of the studies that included them: "humaneness", "competence/accuracy", "patients' involvement in decisions", "time for care", "other aspects of availability/accessibility", "informativeness", "exploring patients' needs", "other aspects of relation and communication" and "availability of special services". 相似文献
104.
在满足机构许用压力角条件下,采用0.618法最优确定盘状摆动凸轮机械的最小基圆半径。 相似文献
105.
The effect of a carbon containing atmosphere on the microstructure and mechanical properties of Fe-32Mn-9.4Al-1C-1.27Si alloy was investigated in this work. Surface oxide nodules and grain boundary oxides were found to form on this alloy when it was annealed in carbon-containing air at 1050 °C for 1 h. The oxidation reaction was thought to be the result of the green rot attack process. This alloy was embrittled severely by the carbon-containing air through the formation of surface oxide nodules and grain boundary oxide. The carbon-containing air enhanced the oxidation rate of this alloy at 1050 °C. The structure of the oxide nodules formed on this alloy in the carbon-containing air was similar to that observed on a FeMnAl alloy heated in 1000 °C air for 24 h. 相似文献
106.
Gregory Gutin Eun Jung Kim Matthias Mnich Anders Yeo 《Journal of Computer and System Sciences》2010,76(8):872-878
We study ordinal embedding relaxations in the realm of parameterized complexity. We prove the existence of a quadratic kernel for the Betweenness problem parameterized above its tight lower bound, which is stated as follows. For a set V of variables and set C of constraints “vi is between vj and vk”, decide whether there is a bijection from V to the set {1,…,|V|} satisfying at least |C|/3+κ of the constraints in C. Our result solves an open problem attributed to Benny Chor in Niedermeier's monograph “Invitation to Fixed-Parameter Algorithms”. The betweenness problem is of interest in molecular biology. An approach developed in this paper can be used to determine parameterized complexity of a number of other optimization problems on permutations parameterized above or below tight bounds. 相似文献
107.
To provide both a high payload capacity and a good stego-image quality, a high payload frequency-based reversible image hiding (HPFRIH) method was presented in this paper. These performances can be achieved by transforming a cover image from the spatial domain into the frequency domain through Haar digital wavelet transform (HDWT) method followed by an adaptive arithmetic coding method to encode the HDWT coefficients in a high-frequency band. The HPFRIH method was used to conceal both the compressed data and the secret data in the high-frequency band. This simple method can completely reconstruct the cover image only from the stego-image. Moreover, experimental results showed that the HPFRIH method offers both impressive hiding capacity and satisfied stego-image quality. 相似文献
108.
Jung Hyeon Bae Gun Hee Kim Woong Hee Jeong Hyun Jae Kim 《Journal of the Society for Information Display》2011,19(5):404-409
Abstract— Non‐volatile memory effects of an all‐solution‐processed oxide thin‐film transistor (TFT) with ZnO nanoparticles (NPs) as the charge‐trapping layer are reported. The device was fabricated by using a soluble MgInZnO active channel on a ZrHfOx gate dielectric. ZnO NPs were used as the charge‐trapping site at the gate‐insulator—channel interface, and Al was used for source and drain electrodes. Transfer characteristics of the device showed a large clockwise hysteresis, which can be used to demonstrate its memory function due to electron trapping in the ZnO NP charge‐trapping layer. This memory effect has the potential to be utilized as a memory application on displays and disposable electronics. 相似文献
109.
110.
Sentiment-oriented contextual advertising 总被引:2,自引:2,他引:0
Web advertising (Online advertising), a form of advertising that uses the World Wide Web to attract customers, has become
one of the world’s most important marketing channels. This paper addresses the mechanism of Content-based advertising (Contextual advertising), which refers to the assignment of relevant ads to a generic web page, e.g., a blog post. As blogs become a platform for
expressing personal opinion, they naturally contain various kinds of expressions, including both facts and comments of both
a positive and negative nature. Besides, in line with the major tenet of Web 2.0 (i.e., user-centric), we believe that the web-site owners would be willing to be in charge of the ads which are positively related to their contents.
Hence, in this paper, we propose the utilization of sentiment detection to improve Web-based contextual advertising. The proposed
sentiment-oriented contextual advertising (SOCA) framework aims to combine contextual advertising matching with sentiment
analysis to select ads that are related to the positive (and neutral) aspects of a blog and rank them according to their relevance.
We experimentally validate our approach using a set of data that includes both real ads and actual blog pages. The results
indicate that our proposed method can effectively identify those ads that are positively correlated with the given blog pages. 相似文献