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71.
This paper is a modified version of a lecture which describes the synthesis, structure and reactivity of some neutral molecules of stellar significance. The neutrals are formed in the collision cell of a mass spectrometer following vertical Franck-Condon one electron oxidation of anions of known bond connectivity. Neutrals are characterised by conversion to positive ions and by extensive theoretical studies at the CCSD(T)/aug-cc-pVDZ//B3LYP/6-31G(d) level of theory. Four systems are considered in detail, viz (i) the formation of linear C(4) and its conversion to the rhombus C(4), (ii) linear C(5) and the atom scrambling of this system when energised, (iii) the stable cumulene oxide CCCCCO, and (iv) the elusive species O(2)C-CO. This paper is not intended to be a review of interstellar chemistry: examples are selected from our own work in this area. 相似文献
72.
Personality theories facilitate integrating the five principles and deducing hypotheses for testing.
Comments on the original article "A New Big Five: Fundamental Principles for an Integrative Science of Personality," by Dan P. McAdams and Jennifer L. Pals (see record 2006-03947-002). In presenting their view of personality science, McAdams and Pals (April 2006) elaborated the importance of five principles for building an integrated science of personality. These principles are stances on evolution and human nature, dispositional signatures, characteristic adaptations, life narratives, and the differential role of culture. Their main emphasis involved differentiating these principles and indicating that they are all relevant to understanding personality. The discussion by McAdams and Pals certainly illuminates the various aspects of personality, but it also cries out for some greater, more systematic integration of the five principles into particular kinds of personality. It is not yet possible, in their approach, to identify different types of personality orientation and to evaluate the relative effectiveness of these orientations. As presented, their approach may be considered a start but hardly a finish. Here, the current author suggests that the metatheory of personality theories that he has proposed (Maddi, 1969/1996) could accelerate the needed integration of the five proposed principles. (PsycINFO Database Record (c) 2010 APA, all rights reserved) 相似文献
73.
Pasqua D’Ambra Daniela di Serafino Salvatore Filippone 《Computers & Mathematics with Applications》2013,65(3):352-361
We present a comparative study of parallel Schwarz preconditioners in the solution of linear systems arising in a Large Eddy Simulation (LES) procedure for turbulent plane channel flows. This procedure applies a time-splitting technique to suitably filtered Navier–Stokes equations, in order to decouple the continuity and momentum equations, and uses a semi-implicit scheme for time integration and finite volumes for space discretisation. This approach requires the solution of four sparse linear systems at each time step, accounting for a large part of the overall simulation; hence the linear system solvers are a crucial component in the whole procedure. Several preconditioners are applied in the simulation of a reference test case for the LES community, using discretisation grids of different sizes, with the aim of analysing the effects of different algorithmic choices defining the preconditioners, and identifying the most effective ones for the selected problem. The preconditioners, coupled with the GMRES method, are run within SParC-LES, a recently developed LES code based on the PSBLAS and MLD2P4 libraries for parallel sparse matrix computations and preconditioning. 相似文献
74.
Conjugated copolymers are important materials for organic light-emitting diodes. Here, an investigation of the photophysical and charge-transporting properties of the prototypical poly(p-phenylene vinylene) based copolymer SuperYellow (SY) is reported. The study also investigated the effect of processing conditions by comparing the properties of spin-coated and solution-cast films. For both types of films, the results of time-resolved fluorescence and photoluminescence quantum yield measurements are similar. The high photoluminescence quantum yield of 60% and its independence of processing conditions shows the effectiveness of the bulky side groups in preventing concentration quenching of fluorescence. Time of flight measurements of charge mobility in both spin-coated and solution-cast films also showed similar results, with mobilities in the range 10?6–10?7 cm2/V s for both films. These results provide important information about a widely used copolymer and show that a good polymer light-emitting diode material can have low mobility. 相似文献
75.
Sabine Barrat Salvatore Tabbone 《Journal of Visual Communication and Image Representation》2010,21(4):355-363
In this paper, we propose a probabilistic graphical model to represent weakly annotated images. We consider an image as weakly annotated if the number of keywords defined for it is less than the maximum number defined in the ground truth. This model is used to classify images and automatically extend existing annotations to new images by taking into account semantic relations between keywords. The proposed method has been evaluated in visual-textual classification and automatic annotation of images. The visual-textual classification is performed by using both visual and textual information. The experimental results, obtained from a database of more than 30,000 images, show an improvement by 50.5% in terms of recognition rate against only visual information classification. Taking into account semantic relations between keywords improves the recognition rate by 10.5%. Moreover, the proposed model can be used to extend existing annotations to weakly annotated images, by computing distributions of missing keywords. Semantic relations improve the mean rate of good annotations by 6.9%. Finally, the proposed method is competitive with a state-of-art model. 相似文献
76.
77.
Paolo Ghetti Ubaldo De Robertis Salvatore DAntone Marco Villani Emo Chiellini 《Fuel》1985,64(7):950-955
A series of coals of different rank has been characterized by surface area measurements performed by sorption of both nitrogen and carbon dioxide. While the data obtained with nitrogen do not discriminate among the different coal samples, those based on carbon dioxide sorption do give a significant distinction between the samples. This technique has also been applied to the determination of the surface area of coal samples quenched after stepwise combustion in air atmosphere. It has been possible to establish a useful correlation between the latter data and the burning profile measured by derivative thermogravimetry. The aim of the present study was to gain a better understanding of the coal combustion process on a laboratory scale which could reasonably be extended to combustion plants. The results presented are relevant to some of the multivalent aspects inherent in the coal combustion process and some valuable information has been gained in respect of characterization of solid fuels. 相似文献
78.
Robust ordinal regression in preference learning and ranking 总被引:1,自引:0,他引:1
Salvatore Corrente Salvatore Greco Miłosz Kadziński Roman Słowiński 《Machine Learning》2013,93(2-3):381-422
Multiple Criteria Decision Aiding (MCDA) offers a diversity of approaches designed for providing the decision maker (DM) with a recommendation concerning a set of alternatives (items, actions) evaluated from multiple points of view, called criteria. This paper aims at drawing attention of the Machine Learning (ML) community upon recent advances in a representative MCDA methodology, called Robust Ordinal Regression (ROR). ROR learns by examples in order to rank a set of alternatives, thus considering a similar problem as Preference Learning (ML-PL) does. However, ROR implements the interactive preference construction paradigm, which should be perceived as a mutual learning of the model and the DM. The paper clarifies the specific interpretation of the concept of preference learning adopted in ROR and MCDA, comparing it to the usual concept of preference learning considered within ML. This comparison concerns a structure of the considered problem, types of admitted preference information, a character of the employed preference models, ways of exploiting them, and techniques to arrive at a final ranking. 相似文献
79.
Davide Marano Gaetano Palumbo Salvatore Pennisi 《Analog Integrated Circuits and Signal Processing》2010,65(2):289-298
The present paper addresses a new compact low-power high-speed output buffer amplifier topology for large-size liquid crystal
display applications. The suggested buffer achieves fast driving performance, draws a low quiescent current during static
operation and offers a rail-to-rail common-mode input range. The circuit provides enhanced slewing capabilities with a limited
power consumption by simultaneously exploiting the push–pull output sections of two basic complementary-type input amplifiers
to realize a dual-path push–pull operation of the output stage. An auxiliary biasing network integrated in the input differential
stage allows the quiescent bias conditions of the class-AB output stage to be inherently controlled without additional current
dissipation. Post-layout simulation results confirm that the proposed amplifier can drive a 1-nF column line load within a
0.9-μs settling time under a 3-V full voltage swing, while drawing only 3.5-μA quiescent current. Monte Carlo simulations
are finally carried out, showing a good degree of robustness of the proposed output buffer against process and mismatch variations. 相似文献
80.
Giovanna Rassu Elisabetta Gavini Gianpiera Spada Salvatore Marceddu 《Drug development and industrial pharmacy》2013,39(11):1178-1187
The preparation of ketoprofen spray-dried microspheres can be affected by the long drug recrystallization time. Polymer type and drug–polymer ratio as well as manufacturing parameters affect the preparation. The purpose of this work was to evaluate the possibility to obtain ketoprofen spray-dried microspheres using the Eudragit® RS and RL; the influence of the spray-drying parameters on morphology, dimension, and physical stability of microspheres was studied. Ketoprofen microspheres based on Eudragit® blend can be prepared by spray-drying and the nebulization parameters do not influence significantly particle properties; nevertheless, they can be affected by drying and storage methods. No effect of the container material is found. 相似文献