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91.
Editable Supercapacitors with Customizable Stretchability Based on Mechanically Strengthened Ultralong MnO2 Nanowire Composite 下载免费PDF全文
Zhisheng Lv Yifei Luo Yuxin Tang Jiaqi Wei Zhiqiang Zhu Xinran Zhou Wenlong Li Yi Zeng Wei Zhang Yanyan Zhang Dianpeng Qi Shaowu Pan Xian Jun Loh Xiaodong Chen 《Advanced materials (Deerfield Beach, Fla.)》2018,30(2)
Although some progress has been made on stretchable supercapacitors, traditional stretchable supercapacitors fabricated by predesigning structured electrodes for device assembling still lack the device‐level editability and programmability. To adapt to wearable electronics with arbitrary configurations, it is highly desirable to develop editable supercapacitors that can be directly transferred into desirable shapes and stretchability. In this work, editable supercapacitors for customizable shapes and stretchability using electrodes based on mechanically strengthened ultralong MnO2 nanowire composites are developed. A supercapacitor edited with honeycomb‐like structure shows a specific capacitance of 227.2 mF cm?2 and can be stretched up to 500% without degradation of electrochemical performance, which is superior to most of the state‐of‐the‐art stretchable supercapacitors. In addition, it maintains nearly 98% of the initial capacitance after 10 000 stretch‐and‐release cycles under 400% tensile strain. As a representative of concept for system integration, the editable supercapacitors are integrated with a strain sensor, and the system exhibits a stable sensing performance even under arm swing. Being highly stretchable, easily programmable, as well as connectable in series and parallel, an editable supercapacitor with customizable stretchability is promising to produce stylish energy storage devices to power various portable, stretchable, and wearable devices. 相似文献
92.
Jing Peng Yuhua Liu Xiao Luo Jiajing Wu Yue Lin Yuqiao Guo Jiyin Zhao Xiaojun Wu Changzheng Wu Yi Xie 《Advanced materials (Deerfield Beach, Fla.)》2019,31(19)
The development of transition metal dichalcogenides has greatly accelerated research in the 2D realm, especially for layered MoS2. Crucially, the metallic MoS2 monolayer is an ideal platform in which novel topological electronic states can emerge and also exhibits excellent energy conversion and storage properties. However, as its intrinsic metallic phase, little is known about the nature of 2D 1T′‐MoS2, probably because of limited phase uniformity (<80%) and lateral size (usually <1 µm) in produced materials. Herein, solution processing to realize high phase‐purity 1T′‐MoS2 monolayers with large lateral size is demonstrated. Direct chemical exfoliation of millimeter‐sized 1T′ crystal is introduced to successfully produce a high‐yield of 1T′‐MoS2 monolayers with over 97% phase purity and unprecedentedly large size up to tens of micrometers. Furthermore, the large‐sized and high‐quality 1T′‐MoS2 nanosheets exhibit clear intrinsic superconductivity among all thicknesses down to monolayer, accompanied by a slow drop of transition temperature from 6.1 to 3.0 K. Prominently, unconventional superconducting behavior with upper critical field far beyond the Pauli limit is observed in the centrosymmetric 1T′‐MoS2 structure. The results open up an ideal approach to explore the properties of 2D metastable polymorphic materials. 相似文献
93.
Chen J Luo Y Hong L Ling Y Pang J Fang Y Wei K Gao X 《Journal of materials science. Materials in medicine》2011,22(3):547-555
A superior drug controlled release system capable of achieving efficient osteogenesis is in imperative demand because of limited
bone substitute tissue for the treatment of bone defect. In the present study, we investigated the potential of using poly(ε-caprolactone)–hydroxyapatite
(PCL–HA) composite microspheres as an injectable bone repair vehicle by controlled release of alendronate (AL), a medicine
that belongs to the bisphosphonates family. The PCL/HA–AL microspheres were prepared with solid/oil/water emulsion technique,
which included two processes: (1) AL was loaded on the hydroxyapatite nanoparticles; (2) the HA–AL complex was built in the
PCL matrix. The spherical PCL/HA–AL microspheres were characterized with its significantly improved encapsulation efficiency
of hydrophilic AL and better sustained release. Human bone mesenchymal stem cells (hMSCs) were cultured on the surface of
these microspheres and exhibited high proliferative profile. Specifically, in osteogenic medium, hMSCs on the surface of PCL/HA–AL
microspheres displayed superior osteogenic differentiation which was verified by alkaline phosphatase activity assay. In conclusion,
by presenting strong osteogenic commitment of hMSCs in vitro, the PCL/HA–AL microspheres have the potential to be used as
an injectable vehicle for local therapy of bone defect. 相似文献
94.
95.
系统以工控机为中心,配以高性能的模块化外设组成一体化的计算机控制系统。采用温度控制外环和电流平衡控制内环的双环路结构来具体实现交流电弧炉温度和三相电流平衡的智能集成控制。外环采用模糊、神经网络和优化决策共同控制,内环则采用模糊专家解耦控制。系统能实时自适应炉况状态的变化,提高生产效率,降低电能及电极消耗。实际运行证明该系统具有良好的鲁棒性和实时性。 相似文献
96.
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98.
Li Guo Lin Jia Lulu Luo Xinru Xu Yangyang Xiang Yujie Ren Dekang Ren Lulu Shen Tingming Liang 《International journal of molecular sciences》2022,23(13)
Circular RNAs (circRNAs), a class of new endogenous non-coding RNAs (ncRNAs), are closely related to the carcinogenic process and play a critical role in tumor metastasis. CircRNAs can lay the foundation for tumor metastasis via promoting tumor angiogenesis, make tumor cells gain the ability of migration and invasion by regulating epithelial-mesenchymal transition (EMT), interact with immune cells, cytokines, chemokines, and other non-cellular components in the tumor microenvironment, damage the normal immune function or escape the immunosuppressive network, and further promote cell survival and metastasis. Herein, based on the characteristics and biological functions of circRNA, we elaborated on the effect of circRNA via circRNA-associated competing endogenous RNA (ceRNA) network by acting as miRNA/isomiR sponges on tumor angiogenesis, cancer cell migration and invasion, and interaction with the tumor microenvironment (TME), then explored the potential interactions across different RNAs, and finally discussed the potential clinical value and application as a promising biomarker. These results provide a theoretical basis for the further application of metastasis-related circRNAs in cancer treatment. In summary, we briefly summarize the diverse roles of a circRNA-associated ceRNA network in cancer metastasis and the potential clinical application, especially the interaction of circRNA and miRNA/isomiR, which may complicate the RNA regulatory network and which will contribute to a novel insight into circRNA in the future. 相似文献
99.
本文在现有网络分析的基础上,进行了EDGE数据网的规划,并通过仿真对规划结果进行了验证,最后对语音和数据网络的资源配置方法进行了研究,提出了相应的资源配置方法。 相似文献
100.
流域水质直接关系到人体健康和生态安全。以萍水河向阳湖至何雁桥段为研究对象,分析其水质空间特征,综合4种方法进行水质评价,进一步利用多元统计和级别差方法对比分析水质评价结果。结果表明:1)COD、NH3-N、TP和TN的最高浓度位于赤山桥处;上游(向阳湖-桥头村)和下游(赤山桥-何雁桥)总体水质较好,部分采样点TN、Fe和Mn轻度超标,污染程度明显弱于中游(桥头村-赤山桥)。2)最差水质级别均为Ⅴ类或劣Ⅴ类水,污染程度属严重污染及以上;单因子评价法确定总氮(TN)为首要污染指标;主成分分析法确定2个主成分,可解释为营养盐污染指标和地质沉积环境指标。3)4种方法两两之间呈显著正相关,相关系数为0.937~0.994,但水质级别表现出明显的差异性;级差法结果表明,3种综合水质评价方法的水质级别顺序为:内梅罗污染指数法<综合污染指数法<主成分分析法。研究成果可为流域水质评价工作和研究提供参考,同时为流域水资源开发利用和水环境保护及综合治理提供科学依据。 相似文献