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21.
通过结合网站设计初期的网站结构和典型用例的预先定义,构建一个基于Web日志数据的用户访问数据分析系统。该系统(AS-UAB,Analysis System of User Access Behaviors)通过对网站结构和典型用例的预先植入,利用该领域最新的研究方法和结论,为网站相关人员提供可视化的用户访问信息统计及趋势预测,网站结构设计及交互设计上存在的问题及改进建议等通用功能和个性化定制功能。 相似文献
22.
不法分子为了逃避过滤,将不良信息中的敏感关键词进行变形。为了识别这些变形的关键词,提出了一种柔性过滤算法。在此基础上,利用浏览器帮助对象(BHO),构建了一个中文网页内容柔性过滤器,用于实时过滤由变形关键词生成的不良网页。该过滤器改善了传统过滤器不能过滤变形关键词的现状,是对传统的基于关键词过滤方法的补充。 相似文献
24.
Wireless Personal Communications - With the rapid development of information technology, issues such as network security and privacy protection have attracted more and more attention. The... 相似文献
25.
26.
Computational Economics - The study aims to analyze and forecast Internet financial risks based on the model based on deep learning and the Back Propagation Neural Network (BPNN). First, the theory... 相似文献
27.
Monitoring the Dynamic Process of Formation of Plasmonic Molecular Junctions during Single Nanoparticle Collisions 下载免费PDF全文
Jing Guo Jie Pan Shuai Chang Xuewen Wang Na Kong Wenrong Yang Jin He 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(15)
The capability to study the dynamic formation of plasmonic molecular junction is of fundamental importance, and it will provide new insights into molecular electronics/plasmonics, single‐entity electrochemistry, and nanooptoelectronics. Here, a facile method to form plasmonic molecular junctions is reported by utilizing single gold nanoparticle (NP) collision events at a highly curved gold nanoelectrode modified with a self‐assembled monolayer. By using time‐resolved electrochemical current measurement and surface‐enhanced Raman scattering spectroscopy, the current changes and the evolution of interfacial chemical bonding are successfully observed in the newly formed molecular tunnel junctions during and after the gold NP “hit‐n‐stay” and “hit‐n‐run” collision events. The results lead to an in‐depth understanding of the single NP motion and the associated molecular level changes during the formation of the plasmonic molecular junctions in a single NP collision event. This method also provides a new platform to study molecular changes at the single molecule level during electron transport in a dynamic molecular tunnel junction. 相似文献
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29.
Owing to the strong affinity of thiols to Au and Ag, they are often employed to modify the surfaces of nanoparticles (NPs). Recently, these strong ligand-interface interactions have been employed to control NP growth, and this technique has emerged as a unique modulation strategy for creating unconventional plasmonic hybrid nanostructures. In these systems, the roles of the non-mercapto components of the thiol molecules and their structures are still unknown. Therefore, we herein present our investigation into this phenomenon. Primary amino (–NH2) groups in thiols are found to play a key role in regulating growth kinetics, i.e., in accelerating Ag deposition on Au NPs. The–NH2 groups are thought to bring Ag ions to the particle surface by coordinating to them, and thereby assist their reduction. The effect of molecular structure is non-trivial and thus provides the possibility of selective thiol detection. Based on the dependence of kinetic modulation on the non-mercapto components and molecular structures of molecules, we demonstrate the highly sensitive and specific detection of cysteine (limit of detection: 6 nM) in a mixture of 19 natural amino acids based on Ag growth on Au nanospheres. In addition, based on this modulation effect, we reveal the entrapping of chiral thiols within the growth layer through their plasmonic circular dichroism (PCD) responses. We believe that thiol-based growth regulation has great potential for creating plasmonic nanostructures with novel functionalities. 相似文献
30.
Molecular dynamic model of nanofluid between flat plates under shear flow conditions was built. The nanofluid model consisted
of 12 spherical copper nanoparticles with each particle diameter of 4 nm and argon atoms as base liquid. The Lennard–Jones
(LJ) potential function was adopted to deal with the interactions between atoms. Thus, the motion states of nanoparticles
during the process of flowing were obtained and the flow behaviors of nanofluid between flat plates at different moments could
be analyzed. The simulation results showed that an absorption layer of argon atoms existed surrounding each nanoparticle and
would accompany with the particle to move. The absorption layer contributed little to the flow of nanoparticles but much to
the heat transferring in nanofluids. Another phenomenon observed during shear flowing process was that the nanoparticles would
vibrate and rotate besides main flowing with liquid argon and these micro-motions could strengthen partial flowing in nanofluids. 相似文献