Extreme-ultraviolet interferometry at 15.5 nm using multilayer optics

The development of multilayer mirror technology capable of operating in the range of 3-30 nm and the construction of thin membranes with excellent uniformity and strength have made it possible to design and implement a Mach-Zehnder interferometer operating at 15.5 nm. We have tested this interferometer by using a soft x-ray laser as a source, and we show its use in probing high-density plasmas.     

Electrocatalysis of Fe-N-C Bonds Driving Reliable Interphase and Fast Kinetics for Phosphorus Anode in Sodium-Ion Batteries

Phosphorus exhibits high capacity and low redox potential, making it a promising anode material for future sodium-ion batteries. However, its practical applications are confined by poor durability and sluggish kinetics. Herein, an innovative in-situ electrochemically self-driven strategy is presented to embed phosphorus nanocrystal (≈10 nm) into a Fe-N-C-rich 3D carbon framework (P/Fe-N-C). This strategy enables rapid and high-capacity sodium ion storage. Through a combination of experimental assistance and theoretical calculations, a novel synergistic catalytic mechanism of Fe-N-C is reasonably proposed. In detail, the electrochemical formation of Fe-N-C catalytic sites facilitates the release of fluorine in ester-based electrolyte, inducing Na⁺-conducting-enhanced solid-electrolyte interphase. Furthermore, it also effectively induces the dissociation energy of the P-P bond and promotes the reaction kinetics of P anode. As a result, the unconventional P/Fe-N-C anode demonstrates outstanding rate-capability (267 mAh g⁻¹ at 100 A g⁻¹) and cycling stability (72%, 10 000 cycles). Notably, the assembled pouch cell achieves high-energy density of 220 Wh kg⁻¹.     

New Polymerized Small Molecular Acceptors with Non-Aromatic π-Conjugated Linkers for Efficient All-Polymer Solar Cells

Developing new polymerized small molecular acceptor (PSMA) is pivotal for improving the performance of all-polymer solar cells. On the basis of this newly developed CH-series small molecule acceptors, two PSMAs are reported herein (namely PZC16 and PZC17, respectively). To reduce the molecular torsion caused by the traditional aromatic π-bridges, non-aromatic conjugated units (ethynyl for PZC16 and vinylene for PZC17) are adopted as the linkers and their effect on the photo-physical properties as well as the device performance are systematically investigated. Both polymer acceptors exhibit co-planar molecular conformation, along with broad absorption ranges and suitable energy levels. In comparison with the PM6:PZC16 film, the PM6:PZC17 film exhibits more uniform phase separation in morphology with a distinct bi-continuous network and better crystallinity. The PM6:PZC17-binary-based devices exhibit a satisfactory PCE of 16.33%, significantly higher than 9.22% of the PZC16-based devices. Impressively, PM6:PZC17-based large area device (ca. 1 cm²) achieves an excellent PCE of 15.14%, which is among the top performance for reported all-polymer solar cells (all-PSCs).     

Event-triggered control for stochastic systems with multiple delays

This paper investigates the stabilization problem for continuous-time stochastic systems with multiple delays under continuous event-triggered mechanisms, of which both static case and dynamic case are considered individually. In order to avoid zeno phenomenon in every sample path, a suspension time after each successful execution is forced for our event-triggered mechanisms, resulting in intermittent detection of system states. Under such control strategy, we deduce mean square exponential stability of stochastic systems with multiple delays by means of Hanalay-type inequality and obtain a delay-dependent-based and less-conservative stabilization criterion without involving the upper bound of time delays. Besides, a co-design procedure is proposed for linear controller and event-triggered mechanisms. In the end, an illustrative example is presented to show effectiveness of the proposed co-design procedure and contrasts the system performance under static and dynamic event-triggered mechanisms.     

An SPH-based mass transfer model for simulating hydraulic characteristics and mass transfer process of dammed rivers

Engineering with Computers - Aerated flow characterized by complex mass transfer processes with multiple hydraulic properties is a common enviro-hydraulics phenomenon, which have a variety of...     

Infrared target tracking based on proximal robust principal component analysis method

Applied Intelligence - Infrared target tracking plays an important role in both civil and military fields. The main challenges in designing a robust and high-precision tracker for infrared...     

Three-dimensional elasticity solution of layered plates with viscoelastic interlayers

An analytical solution for simply supported layered plates with viscoelastic interlayers under a transverse load is proposed. The deformation of each plate layer is described by the exact three-dimensional elasticity equations. The viscoelastic property of interlayer is simulated by the generalized Maxwell model. The constitutive relation of the interlayer is simplified by the quasi-elastic approximation, which significantly simplifies the analytical process. The solution of stress and displacement fields with undetermined coefficients is derived by solving a group of ordinary differential equations. The undetermined coefficients can be efficiently deduced by using the recursive matrix technique for the plate with any number of layers. The practical convergence is observed during numerical tests. The comparison analysis indicates that the present solution has a close agreement with the finite element solution. However, the solution based on the Mindlin–Reissner hypothesis is significantly different from the present solution for thick plates. Finally, the effect of interlayer thickness on stress and displacement distributions of a five-layer plate is discussed in detail.     

Hollow Pd/MOF Nanosphere with Double Shells as Multifunctional Catalyst for Hydrogenation Reaction

A new type of hollow nanostructure featured double metal‐organic frameworks shells with metal nanoparticles (MNPs) is designed and fabricated by the methods of ship in a bottle and bottle around the ship. The nanostructure material, hereinafter denoted as Void@HKUST‐1/Pd@ZIF‐8, is confirmed by the analyses of photograph, transmission electron microscopy, scanning electron microscopy, powder X‐ray diffraction, inductively coupled plasma, and N₂ sorption. It possesses various multifunctionally structural characteristics such as hollow cavity which can improve mass transfer, the adjacent of the inner HKUST‐1 shell to the void which enables the matrix of the shell to host and well disperse MNPs, and an outer ZIF‐8 shell which acts as protective layer against the leaching of MNPs and a sieve to guarantee molecular‐size selectivity. This makes the material eligible candidates for the heterogeneous catalyst. As a proof of concept, the liquid‐phase hydrogenation of olefins with different molecular sizes as a model reaction is employed. It demonstrates the efficient catalytic activity and size‐selectivity of Void@HKUST‐1/Pd@ZIF‐8.