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951.
Ke Wu Zhe Li Jibo Tang Xianglong Lv Hailing Wang Ruichun Luo Pan Liu Lihua Qian Shunping Zhang Songliu Yuan 《Nano Research》2018,11(8):4123-4132
Photoluminescence (PL) of transition metal dichalcogenides (TMDs) can be engineered by controlling the density of defects, which provide active sites for electron-hole recombination, either radiatively or non-radiatively. However, the implantation of defects by external stimulation, such as uniaxial tension and irradiation, tends to introduce local damages or structural non-homogeneity, which greatly degrades their luminescence properties and impede their applicability in constructing optoelectronic devices. In this paper, we present a strategy to introduce a controllable level of defects into the MoS2 monolayers by adding a hydrogen flow during the chemical vapor deposition, without sacrificing their luminescence characteristics. The density of the defect is controlled directly by the concentration of hydrogen. For an appropriate hydrogen flux, the monolayer MoS2 sheets have three times stronger PL emission at the excitonic transitions, compared with those samples with nearly perfect crystalline structure. The defect-bounded exciton transitions at lower energies arising in the defective samples and are maximized when the total PL is the strongest. However, the B exciton, exhibits a monotonic decline as the defect density increases. The Raman spectra of the defective MoS2 reveal a redshift (blueshift) of the in-plane (out-of-plane) vibration modes as the hydrogen flux increases. All the evidence indicates that the generated defects are in the form of sulfur vacancies. This study renders the high-throughput synthesis of defective MoS2 possible for catalysis or light emitting applications. 相似文献
952.
Lili Gong Qi Zhang Liangjun Wang Jianfeng Wu Cheng Han Bo Lei Wei Chen Goki Eda Kuan Eng Johnson Goh Chorng Haur Sow 《Nano Research》2018,11(9):4574-4586
We demonstrate a facile and effective approach to significantly improve the photoluminescence of bulk MoS2 via laser thinning followed by gold particle decoration. Upon laser thinning of exfoliated bulk MoS2, photoluminescence emerges from the laser-thinned region. After further treatment with an AuCl3 solution, gold particles self-assemble on the laser-thinned region and thick edges, further increasing the fluorescence of bulk MoS2 28 times and the Raman response 3 times. Such fluorescence enhancement can be attributed to both surface plasmon resonance and p-type doping induced by gold particles. The combination of laser thinning and AuCl3 treatment enables the functionalization of bulk MoS2 for optoelectronic applications. It can also provide a viable strategy for mask-free and area-selective p-type doping on single MoS2 flakes. 相似文献
953.
Liu Daobin Wu Chuanqiang Chen Shuangming Ding Shiqing Xie Yaofeng Wang Changda Wang Tao Haleem Yasir A. ur Rehman Zia Sang Yuan Liu Qin Zheng Xusheng Wang Yu Ge Binghui Xu Hangxun Song Li 《Nano Research》2018,11(4):2217-2228
Nano Research - Atomically dispersed catalysts have attracted attention in energy conversion applications because their efficiency and chemoselectivity for special catalysis are superior to those... 相似文献
954.
Zan Wu Zhang Qiaochu Xu Hu Liao Fuyou Guo Zhongxun Deng Jianan Wan Jing Zhu Hao Chen Lin Sun Qingqing Ding Shijin Zhou Peng Bao Wenzhong Zhang David Wei 《Nano Research》2018,11(7):3739-3745
Nano Research - A spin-coating method was applied to obtain thinner and smoother PEO/LiClO4 polymer electrolyte films (EFs) with a lower level of crystallization than those obtained using a... 相似文献
955.
Han Wenjie Qin Xianying Wu Junxiong Li Qing Liu Ming Xia Yue Du Hongda Li Baohua Kang Feiyu 《Nano Research》2018,11(2):892-904
Nano Research - Porous Fe3O4/carbon microspheres (PFCMs) were successfully fabricated via a facile electrospray method and subsequent heat treatment, using ferrous acetylacetonate, carbon nanotubes... 相似文献
956.
Xiaoying Cheng Xuyang Cao Zhenyu Wu Zhiping Ying Duncan Camilleri Xudong Hu 《Advanced Engineering Materials》2023,25(19):2300341
Carbon fiber-reinforced polymer (CFRP) materials are widely applied in various areas as key structure components. The structural health monitoring of the CFRP components is crucial to prevent catastrophic failure. However, the nonplane surfaces of CFRP components hinder the attaching of monitoring sensors with hard substrates. Therefore, the substrate conditions for sensor preparation are mainly considered in this study. To adapt the proposed sensors to the curved substrate, including nondevelopable surfaces, electrospinning method is used to prepare conformal piezoresistive fiber films, in which polymethyl methacrylate is served as the matrix and carbon nanotubes are utilized as the conductive filler. The piezoresistive fibers covered on CFRP substrates have a gauge factor up to 207.95 and can response to the strain less than 0.05%. Moreover, the sensor also has high durability and the ability to follow the dynamic excitation signals with as high as 50 Hz. 相似文献
957.
Yike Li Zhenhua Wu Congcan Shi Yizhuo Xu Aotian Chen Bin Su 《Advanced Engineering Materials》2023,25(20):2300703
Flush toilets waste a significant amount of water every day due to the unavoidable adhesions between human waste and the toilet surfaces. Super-slippery surfaces can repel complex fluids and various viscoelastic solids, however, are easily broken by mechanical abrasions. Herein, the fabrication of an abrasion-resistant super-slippery flush toilet (ARSFT) is reported using a selective laser sintering 3D printing technology. Unlike traditional super-slippery surfaces with limited thicknesses which can be easily worn away, the powder-sintered strategy endows the ARSFT not only with a self-supporting 3D complex shape but also with a porous structure that can accommodate considerable lubricants for an abrasion-resistant super-slippery property. As a result, the as-prepared ARSFT remains clean after contacting with various liquids such as milk, yogurt, highly sticky honey, and starch gel mixed congee, demonstrating excellent repellence to complex fluids. Besides liquids, the ARSFT exhibits a high resistance to sticky synthetic feces. Notably, even after being abraded to 1,000 cycles of abrasion using sandpaper, the ARSFT maintains its record-breaking super-slippery capability. The concept of the 3D-printed object with a superior abrasion-resistant slippery ability will improve the development of super-slippery materials and further save water consumption in the human society. 相似文献
958.
Physiological signals indicate a person’s physical and mental state at any given time. Accordingly, many studies extract physiological signals from the human body with non-contact methods, and most of them require facial feature points. However, under COVID-19, wearing a mask has become a must in many places, so how non-contact physiological information measurements can still be performed correctly even when a mask covers the facial information has become a focus of research. In this study, RGB and thermal infrared cameras were used to execute non-contact physiological information measurement systems for heart rate, blood pressure, respiratory rate, and forehead temperature for people wearing masks due to the pandemic. Using the green (G) minus red (R) signal in the RGB image, the region of interest (ROI) is established in the forehead and nose bridge regions. The photoplethysmography (PPG) waveforms of the two regions are obtained after the acquired PPG signal is subjected to the optical flow method, baseline drift calibration, normalization, and bandpass filtering. The relevant parameters in Deep Neural Networks (DNN) for the regression model can correctly predict the heartbeat and blood pressure. In addition, the temperature change in the ROI of the mask after thermal image processing and filtering can be used to correctly determine the number of breaths. Meanwhile, the thermal image can be used to read the temperature average of the ROI of the forehead, and the forehead temperature can be obtained smoothly. The experimental results show that the above-mentioned physiological signals of a subject can be obtained in 6-s images with the error for both heart rate and blood pressure within 2%~3% and the error of forehead temperature within ±0.5°C. 相似文献
959.
Jiabin Liu Jiawei Deng Yangyang Zhu Xiaokang Geng Lifu Zhang Sang Young Jeong Dan Zhou Han Young Woo Dong Chen Feiyan Wu Lie Chen 《Advanced materials (Deerfield Beach, Fla.)》2023,35(1):2208008
With the great potential of the all-polymer solar cells for large-area wearable devices, both large-area device efficiency and mechanical flexibility are very critical but attract limited attention. In this work, from the perspective of the polymer configurations, two types of terpolymer acceptors PYTX-A and PYTX-B (X = Cl or H) are developed. The configuration difference caused by the replacement of non-conjugated units results in distinct photovoltaic performance and mechanical flexibility. Benefiting from a good match between the intrinsically slow film-forming of the active materials and the technically slow film-forming of the blade-coating process, the toluene-processed large-area (1.21 cm2) binary device achieves a record efficiency of 14.70%. More importantly, a new parameter of efficiency stretchability factor (ESF) is proposed for the first time to comprehensively evaluate the overall device performance. PM6:PYTCl-A and PM6:PYTCl-B yield significantly higher ESF than PM6:PY-IT. Further blending with non-conjugated polymer donor PM6-A, the best ESF of 3.12% is achieved for PM6-A:PYTCl-A, which is among the highest comprehensive performances. 相似文献
960.