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51.
Postawa Z Czerwinski B Szewczyk M Smiley EJ Winograd N Garrison BJ 《Analytical chemistry》2003,75(17):4402-4407
The mechanism of enhanced desorption initiated by 15-keV C60 cluster ion bombardment of a Ag single crystal surface is examined using molecular dynamics computer simulations. The size of the model microcrystallite of 165,000 atoms and the sophistication of the interaction potential function yields data that should be directly comparable with experiment. The C60 model was chosen since this source is now being used in secondary ion mass spectrometry experiments in many laboratories. The results show that a crater is formed on the Ag surface that is approximately 10 nm in diameter, a result very similar to that found for Au3 bombardment of Au. The yield of Ag atoms is approximately 16 times larger than for corresponding atomic bombardment with 15-keV Ga atoms, and the yield of Ag3 is enhanced by a factor of 35. The essential mechanistic reasons for these differences is that the C60 kinetic energy is deposited closer to the surface, with the deeply penetrating energy propagation occurring via a nondestructive pressure wave. The numbers predicted by the model are testable by experiment, and the approach is extendable to include the study of organic overlayers on metals, a situation of growing importance to the SIMS community. 相似文献
52.
Bartlomiej Gawin 《Information Systems Management》2017,34(4):347-358
ABSTRACTThis study investigates data sources for Business Intelligence solutions, which provide a foundation for holistic analyses, optimization, and forecasting of electrical power consumption within Facility Management for retail facilities networks. A multiple case study among Polish subsidiaries of Sweden, France, and UK-based companies along with a domestic Polish has been conducted. The authors identify, verify, and organize the determinants augmenting an energy efficiency-oriented decision-making process and introduce a set of potential benchmarking scenarios for managing it. 相似文献
53.
Marianna Sledzinska Bartlomiej Graczykowski Jeremie Maire Emigdio Chavez‐Angel Clivia M. Sotomayor‐Torres Francesc Alzina 《Advanced functional materials》2020,30(8)
The central concept in phononics is the tuning of the phonon dispersion relation, or phonon engineering, which provides a means of controlling related properties such as group velocity or phonon interactions and, therefore, phonon propagation, in a wide range of frequencies depending on the geometries and sizes of the materials. Phononics exploits the present state of the art in nanofabrication to tailor dispersion relations in the range of GHz for the control of elastic waves/phonons propagation with applications toward new information technology concepts with phonons as state variable. Moreover, phonons provide an adaptable approach for supporting a coherent coupling between different state variables, and the development of nanoscale optomechanical systems during the last decade attests this prospect. The most extended approach to manipulate the phonon dispersion relation is introducing an artificial periodic modulation of the elastic properties, which is referred to as phononic crystal (PnC). Herein, the focus is on the recent experimental achievements in the fabrication and application of 2D PnCs enabling the modification of the dispersion relation of surface and membrane modes, and presenting phononic bandgaps, waveguiding, and confinement in the hypersonic regime. Furthermore, these artificial materials offer the potential of modifying and controlling the heat flow to enable new schemes in thermal management. 相似文献
54.
55.
Barbara Gil Janusz Janas Ewa Woch Zbigniew Olejniczak Jerzy Datka Bogdan Sulikowski 《Catalysis Today》2008,137(2-4):174
The role of the initial acidity of ferrierite type zeolite on the status of cobalt and the catalytic activity of CoFER and InCoFER was investigated. Two FER zeolites were used: NH4FER without any pretreatment (FER-1) and the same zeolite, dehydroxylated at 825 K (FER-2). Dehydroxylation removed most of the Si–OH–Al groups, therefore the resulting zeolite revealed practically no ion exchange capacity. The status of cobalt was followed by IR spectroscopy with probe molecules: CO (a probe for Co2+) and NO (a probe for Co3+). The introduction of cobalt by solid-state ion exchange produced divalent cobalt in exchange positions and in the form of oxide-like clusters, their respective concentration was determined by quantitative IR experiments of CO sorption. The amount of Co3+, present in CoFER-1 and InCoFER-1, was also determined. All these forms of cobalt were practically absent from CoFER-2 and InCoFER-2. The NO conversion and selectivity to N2 of CoFER-2 in CH4-SCR-NO was poor, indicating the essential role of the initial acidity of the ferrierite matrix on the formation of catalytically active Co species. The introduction of indium into CoFER only slightly increased the NO conversion and shifted the reaction path from NO2 towards N2 formation for FER-1, while greatly improved the catalytic performance of the FER-2 series. 相似文献
56.
Bartlomiej Winiarski Richard M. Langford Jiawan Tian Yoshihiko Yokoyama Peter K. Liaw Philip J. Withers 《Metallurgical and Materials Transactions A》2010,41(7):1743-1751
Residual stresses in crystalline or glassy materials often play a key role in the performance of advanced devices and components.
However, stresses in amorphous materials cannot easily be determined at the micron scale by diffraction, or by other conventional
laboratory methods. In this article, a technique for mapping residual stress profiles in amorphous materials with high spatial
definition is presented. By applying a focused ion beam (FIB)–based semidestructive mechanical relaxation method, the stresses
are mapped in a peened and fatigued bulk metallic glass (BMG) (Zr50Cu40Al10 at. pct). The residual stresses are inferred using finite element analysis (FEA) of the surface relaxations, as measured
by digital image correlation (DIC), that occur when a microslot is micromachined by FIB. Further, we have shown that acceptable
accuracy can in most cases be achieved using a simple analytical model of the slot. It was found that the fatigue cycling
significantly changes the distribution of compressive residual stresses with depth in the plastically deformed surface layer.
Our observations point to the scalability of this method to map residual stresses in volumes as small as 1 × 1 × 0.2 μm3 or less. 相似文献
57.
58.
Wireless Personal Communications - In this paper we present an original adaptive task scheduling system, which optimizes the energy consumption of mobile devices using machine learning mechanisms... 相似文献
59.
Microcrystals of desired sizes are important in a range of processes and materials, including controlled drug release, production of pharmaceutics and food, bio- and photocatalysis, thin-film solar cells and antibacterial fabrics. The growth of microcrystals can be controlled by a variety of agents, such as multivalent ions, charged small molecules, mixed cationic-anionic surfactants, polyelectrolytes and other polymers, micropatterned self-assembled monolayers, proteins and also biological organisms during biomineralization. However, the chief limitation of current approaches is that the growth-modifying agents are typically specific to the crystalizing material. Here, we show that oppositely charged nanoparticles can function as universal surfactants that control the growth and stability of microcrystals of monovalent or multivalent inorganic salts, and of charged organic molecules. We also show that the solubility of the microcrystals can be further tuned by varying the thickness of the nanoparticle surfactant layers and by reinforcing these layers with dithiol crosslinks. 相似文献
60.
Karolina Górnicka Xin Gui Bartlomiej Wiendlocha Loi T. Nguyen Weiwei Xie Robert J. Cava Tomasz Klimczuk 《Advanced functional materials》2021,31(3):2007960
Superconductivity was first observed more than a century ago, but the search for new superconducting materials remains a challenge. The Cooper pairs in superconductors are ideal embodiments of quantum entanglement. Thus, novel superconductors can be critical for both learning about electronic systems in condensed matter and for possible application in future quantum technologies. Here two previously unreported materials, NbIr2B2 and TaIr2B2, are presented with superconducting transitions at 7.2 and 5.2 K, respectively. They display a unique noncentrosymmetric crystal structure, and for both compounds the magnetic field that destroys the superconductivity at 0 K exceeds one of the fundamental characteristics of conventional superconductors (the “Pauli limit”), suggesting that the superconductivity may be unconventional. Supporting this experimentally based deduction, first-principle calculations show a spin-split Fermi surface due to the presence of strong spin–orbit coupling. These materials may thus provide an excellent platform for the study of unconventional superconductivity in intermetallic compounds. 相似文献