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121.
Gian Luigi Angrisani Piriya Taptimthong Susanne Elisabeth Thürer Christian Klose Hans Jürgen Maier Marc Christopher Wurz Kai Möhwald 《Advanced Engineering Materials》2018,20(9)
122.
Patterning of Discotic Liquid Crystals with Tunable Molecular Orientation for Electronic Applications 下载免费PDF全文
Cheng Zou Jingxia Wang Meng Wang Yuchen Wu Kehua Gu Zhihao Shen Guirong Xiong Huai Yang Lei Jiang Tomiki Ikeda 《Small (Weinheim an der Bergstrasse, Germany)》2018,14(21)
The large‐area formation of functional micropatterns with liquid crystals is of great significance for diversified applications in interdisciplinary fields. Meanwhile, the control of molecular alignment in the patterns is fundamental and prerequisite for the adequate exploitation of their photoelectric properties. However, it would be extremely complicated and challenging for discotic liquid crystals (DLCs) to achieve the goal, because they are insensitive to external fields and surface chemistry. Herein, a simple method of patterning and aligning DLCs on flat substrates is disclosed through precise control of the formation and dewetting of the capillary liquid bridges, within which the DLC molecules are confined. Large‐area uniform alignment occurs spontaneously due to directional shearing force when the solvent is slowly evaporated and programmable patterns could be directly generated on desired substrates. Moreover, the in‐plane column direction of DLCs is tunable by slightly tailoring their chemical structures which changes their self‐assembly behaviors in liquid bridges. The patterned DLCs show molecular orientation–dependent charge transport properties and are promising for templating self‐assembly of other materials. The study provides a facile method for manipulation of the macroscopic patterns and microscopic molecular orientation which opens up new opportunities for electronic applications of DLCs. 相似文献
123.
Visual Immunoassays: Layered Aggregation with Steric Effect: Morphology‐Homogeneous Semiconductor MoS2 as an Alternative 2D Probe for Visual Immunoassay (Small 7/2018) 下载免费PDF全文
124.
Single point incremental forming: state-of-the-art and prospects 总被引:1,自引:0,他引:1
Joost R. Duflou Anne-Marie Habraken Jian Cao Rajiv Malhotra Markus Bambach Dave Adams Hans Vanhove Amirahmad Mohammadi Jack Jeswiet 《International Journal of Material Forming》2018,11(6):743-773
Incremental sheet metal forming in general and Single Point Incremental Forming (SPIF) specifically have gone through a period of intensive development with growing attention from research institutes worldwide. The result of these efforts is significant progress in the understanding of the underlying forming mechanisms and opportunities as well as limitations associated with this category of flexible forming processes. Furthermore, creative process design efforts have enhanced the process capabilities and process planning methods. Also, simulation capabilities have evolved substantially. This review paper aims to provide an overview of the body of knowledge with respect to Single Point Incremental Forming. Without claiming to be exhaustive, each section aims for an up-to-date state-of-the-art review with corresponding conclusions on scientific progress and outlook on expected further developments. 相似文献
125.
Susanna Monti Giovanni Barcaro Luca Sementa Vincenzo Carravetta Hans Ågren 《Nano Research》2018,11(4):1757-1767
The self-assembling properties, stability, and dynamics of hybrid nanocarriers (gold nanoparticles (AuNPs) functionalized with cysteine-based peptides) in solution are studied through a series of classical molecular dynamics simulations based on a recently parametrized reactive force field. The results reveal, at the atomic level, all the details regarding the peptide adsorption mechanisms, nanoparticle stabilization, aggregation, and sintering. The data confirm and explain the experimental findings and disclose aspects that cannot be scrutinized by experiments. The biomolecules are both chemisorbed and physisorbed; self-interactions of the adsorbates and formation of stable networks of interconnected molecules on the AuNP surfaces limit substrate reconstructions, protect the AuNPs from the action of the solvent, and prevent direct interactions of the gold surfaces. The possibility of agglomeration of the functionalized nanoparticles, compared with the sintering of the bare supports in a water solution, is demonstrated through relatively long simulations and fast steered dynamics. The analysis of the trajectories reveals that the AuNPs were well stabilized by the peptides. This prevented particle sintering and kept the particles far apart; however, part of their chains could form interconnections (crosslinks) between neighboring gold vehicles. The excellent agreement of these results with the literature confirm the reliability of the method and its potential application to the modeling of more complex materials relevant to the biomedical sector. 相似文献
126.
Yi-Chao Zou Zhi-Gang Chen Enze Zhang Fantai Kong Yan Lu Lihua Wang John Drennan Zhongchang Wang Faxian Xiu Kyeongjae Cho Jin Zou 《Nano Research》2018,11(2):696-706
Identification of atomic disorders and their subsequent control has proven to be a key issue in predicting, understanding, and enhancing the properties of newly emerging topological insulator materials. Here, we demonstrate direct evidence of the cation antisites in single-crystal SnBi2Te4 nanoplates grown by chemical vapor deposition, through a combination of sub-ångström-resolution imaging, quantitative image simulations, and density functional theory calculations. The results of these combined techniques revealed a recognizable amount of cation antisites between Bi and Sn, and energetic calculations revealed that such cation antisites have a low formation energy. The impact of the cation antisites was also investigated by electronic structure calculations together with transport measurement. The topological surface properties of the nanoplates were further probed by angle-dependent magnetotransport, and from the results, we observed a two-dimensional weak antilocalization effect associated with surface carriers. Our approach provides a pathway to identify the antisite defects in ternary chalcogenides and the application potential of SnBi2Te4 nanostructures in next-generation electronic and spintronic devices. 相似文献
127.
We performed Raman measurements at 18 K and pressures up to 25 GPa in order to construct a tentative phase diagram of the (N
2)1–x
:(O
2)x
–system at low temperatures. We varied the composition of the mixed system over the whole concentration range. Here we focused on the systems with high nitrogen concentration and pressures above 2 GPa. It is known that at room temperature oxygen is highly solvable in the –phase of N
2. The experimental results show that oxygen suppresses the disorder–order transition –N
2. 相似文献
128.
Michael Buro Hans Kleine Büning 《Annals of Mathematics and Artificial Intelligence》1996,18(2):243-260
We investigate properties ofk-resolution, a restricted version of resolution in which one parent clause must have length at mostk. Starting from a unit-preference strategy, we compare minimal proof lengths of unit-resolution and unrestricted resolution. In particular, we show that the speed-up by using resolution is bound by
if the shortest unit-resolution refutation needst steps. Next we present an algorithm which decides whether the empty clause can be deduced by 2-resolution from a formula and has time complexity O(length()4). Finally we describe effects onk-resolution if a formula is transformed intot-CNF and show that extended 3-resolution is complete and sound. 相似文献
129.
This paper presents a new approach to reconstruct curved solids composed of elementary volumes intersecting with one another from three-view engineering drawings. Intersection curves arising from two intersecting curved surfaces are mostly higher order spatial curves, which cannot be described exactly by 2D orthographic projections and normally represented as smooth curves passing through several key points or even simplified as arcs or lines. Approximated sketches of higher order intersection curves in 2D views result in the invalidation of existing methods that need the exact projection information as input. Based on some heuristic hints, our method is able to recover the complete and correct half-profiles of the intersecting elementary volumes using the least traces left by them, which ensure the correctness of solution solids constructed finally. Several examples are provided to show the validation of the described method. 相似文献
130.