Effect of Sintering Temperature on Magnetic and Electrical Properties of GdBaCo<Subscript>2</Subscript><Emphasis Type="Italic">O</Emphasis><Subscript>5 + <Emphasis Type="Italic">δ</Emphasis></Subscript>

In this study, we report the results of an investigation into the sintering temperature dependence of magnetic and transport properties for GdBaCo₂ O _{5 + δ} synthesized through a sol-gel method. The lowering of sintering temperature leads to the increase of oxygen content and the reduction of grain size. The increase of oxygen content results in the enhancement of magnetic interactions and the weakening of Coulomb repulsion effect, while the reduction of grain size improves the magnetoresistance effect. Metal-insulator transition accompanied with spin-state transition is observed in all samples.     

Comparison of gas sensing properties based on hollow and porous α-Fe<Subscript>2</Subscript>O<Subscript>3</Subscript> nanotubes

Hollow and porous α-Fe₂O₃ nanotubes were successfully synthesized by single nozzle electrospinning method followed by annealing treatment. The crystal structures and morphologies of the as-prepared materials were characterized by X-ray diffraction and scanning electron microscopy, respectively. The as-prepared materials were applied to construct gas sensor devices which gas sensing properties were further investigated. The obtained results revealed that porous α-Fe₂O₃ nanotube gas sensors exhibit a markedly enhanced gas sensing performance compared with hollow α-Fe₂O₃ nanotube gas sensors, which was about three times higher to 100 ppm acetone at 240 °C. Interestingly, hollow and porous α-Fe₂O₃ nanotube gas sensors both showed fast response–recovery time and good selectivity, but the porous ones possessed the shorter recovery time. The improved properties could be attributed to the unique morphology of porous nanotubes. Thus, further improvement of performance in metal-oxide-semiconductors materials could be realized by preparation the unique porous structures of nanotubes. Moreover, it is expected that porous metal-oxide-semiconductors nanotubes could be further design as promising candidates for gas sensing materials.     

Graphene oxide-decorated Fe<Subscript>2</Subscript>(MoO<Subscript>4</Subscript>)<Subscript>3</Subscript> microflowers as a promising anode for lithium and sodium storage

Mixed transition metal oxides (MTMOs) have received intensive attention as promising anode materials for lithium-ion batteries (LIBs) and sodium-ion batteries (SIBs). In this work, we demonstrate a facile one-step water-bath method for the preparation of graphene oxide (GO) decorated Fe₂(MoO₄)₃ (FMO) microflower composite (FMO/GO), in which the FMO is constructed by numerous nanosheets. The resulting FMO/GO exhibits excellent electrochemical performances in both LIBs and SIBs. As the anode material for LIBs, the FMO/GO delivers a high capacity of 1,220 mAh·g^–1 at 200 mA·g^–1 after 50 cycles and a capacity of 685 mAh·g^–1 at a high current density of 10 A·g^–1. As the anode material for SIBs, the FMO/GO shows an initial discharge capacity of 571 mAh·g^–1 at 100 mA·g^–1, maintaining a discharge capacity of 307 mAh·g^–1 after 100 cycles. The promising performance is attributed to the good electrical transport from the intimate contact between FMO and graphene oxide. This work indicates that the FMO/GO composite is a promising anode for high-performance lithium and sodium storage.

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MHSACAE-CNN在噪声下的电机轴承故障诊断

电机的运行情况复杂,实际运行工况下会有大量的噪声,导致其轴承故障诊断精度下降。为了改善这一问题,提出了一种基于多头自注意力机制的一维全卷积自编码网络（One-dimensional Fully Convolutional Autoencoding Network Basedon Multi-head Self-attention,MHSACAE）与卷积神经网络（Convolutional Neural Network,CNN）结合的轴承故障诊断方法。该方法先采用MHSACAE网络进行降噪,再通过CNN进行故障诊断。其中MHSACAE去噪网络采用无监督训练的方式,充分考虑了实际工况和序列数据内在联系,在实现对噪声的滤除效果的同时,最大限度地保留下了原始的故障信息,使得CNN可以实现在噪声情况下对电机轴承故障的高精度诊断。通过与其他轴承故障诊断方法在噪声情况下进行对比,证明提出的方法具有更好的效果。     

Regulation of Polymer Configurations Enables Green Solvent-Processed Large-Area Binary All-Polymer Solar Cells With Breakthrough Performance and High Efficiency Stretchability Factor

With the great potential of the all-polymer solar cells for large-area wearable devices, both large-area device efficiency and mechanical flexibility are very critical but attract limited attention. In this work, from the perspective of the polymer configurations, two types of terpolymer acceptors PYTX-A and PYTX-B (X = Cl or H) are developed. The configuration difference caused by the replacement of non-conjugated units results in distinct photovoltaic performance and mechanical flexibility. Benefiting from a good match between the intrinsically slow film-forming of the active materials and the technically slow film-forming of the blade-coating process, the toluene-processed large-area (1.21 cm²) binary device achieves a record efficiency of 14.70%. More importantly, a new parameter of efficiency stretchability factor (ESF) is proposed for the first time to comprehensively evaluate the overall device performance. PM6:PYTCl-A and PM6:PYTCl-B yield significantly higher ESF than PM6:PY-IT. Further blending with non-conjugated polymer donor PM6-A, the best ESF of 3.12% is achieved for PM6-A:PYTCl-A, which is among the highest comprehensive performances.     

一款基于APA300的创新型FPGA实验板

基于Actel公司Flash型FPGA芯片APA300设计并实现一款创新型FPGA实验板.该实验板包括2片互通的APA300、丰富的外围设备和常用外部设备端口,还提供与外部电路连接的扩展接口,能够开展多种创新性实验,并可作为科学预研的平台.在详细介绍了实验板各部分的实现原理和电路连接图后,给出了实验板的两个典型创新性实验示例:协处理器密码机和MP3播放器.