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91.
Maruyama S Murakami Y Shibuta Y Miyauchi Y Chiashi S 《Journal of nanoscience and nanotechnology》2004,4(4):360-367
Recent advances in high-purity and high-yield catalytic chemical vapor deposition (CVD) generation of single-walled carbon nanotubes (SWNTs) from alcohol are comprehensively presented and discussed on the basis of results obtained from both experimental and numerical investigations. We have uniquely adopted alcohol as a carbon feedstock, and this has resulted in high-quality, low-temperature synthesis of SWNTs. This technique can produce SWNTs even at a very low temperature of 550 degrees C, which is about 300 degrees C lower than the conventional CVD methods in which methane or acetylene is typically used. We demonstrate the excellence of the proposed alcohol catalytic CVD method for high-yield production of SWNTs when Fe-Co on USY-zeolite powder was used as a catalyst. At optimum CVD conditions, a SWNT yield of more than 40 wt % was achieved over the weight of the catalytic powder within the reaction time of 120 min. In addition to the advantages for mass production, this method is also suitable for the direct synthesis of high-quality SWNTs on Si and quartz substrates when combined with the newly developed liquid-based "dip-coat" technique to mount catalytic metals on the surface of substrates. This method allows easy and costless loading of catalytic metals without the need for any support or underlayer materials that were usually required in previous studies for the generation of a sufficient quantity of SWNTs on an Si surface. Finally, the result of molecular dynamics simulation for the SWNT growth process is presented to obtain a fundamental insight into the initial growth mechanism on the catalytic particles. 相似文献
92.
Eric A. Grulke Kazuhiro Yamamoto Kazuhiro Kumagai Ines Häusler Werner Österle Erik Ortel Vasile-Dan Hodoroaba Scott C. Brown Christopher Chan Jiwen Zheng Kenji Yamamoto Kouji Yashiki Nam Woong Song Young Heon Kim Aleksandr B. Stefaniak D. Schwegler-Berry Victoria A. Coleman Åsa K. Jämting Arnold J. Stromberg 《Advanced Powder Technology》2017,28(7):1647-1659
93.
Qian Liu Shohei Kumagai Sergei Manzhos Yingqian Chen Indunil Angunawela Masrur Morshed Nahid Krishna Feron Steven E. Bottle John Bell Harald Ade Jun Takeya Prashant Sonar 《Advanced functional materials》2020,30(34)
To achieve semiconducting materials with high electron mobility in organic field‐effect transistors (OFETs), low‐lying energy levels (the highest occupied molecular orbital (HOMO) and the lowest unoccupied molecular orbital (LUMO)) and favorable molecular packing and ordering are two crucial factors. Here, it is reported that the incorporation of pyridine and selenophene into the backbone of a diketopyrrolopyrrole (DPP)‐based copolymer produces a high‐electron‐mobility semiconductor, PDPPy‐Se. Compared with analogous polymers based on other DPP derivatives and selenophene, PDPPy‐Se features a lower LUMO that can decrease the electron transfer barrier for more effective electron injection, and simultaneously a lower HOMO that, however, can increase the hole transfer barrier to suppress the hole injection. Combined with thermal annealing at 240 °C for thin film morphology optimization to achieve large‐scale crystallite domains with tight molecular packing for effective charge transport along the conducting channel, OFET devices fabricated with PDPPy‐Se exhibit an n‐type‐dominant performance with an electron mobility (μe) as high as 2.22 cm2 V?1 s?1 and a hole/electron mobility ratio (μh/μe) of 0.26. Overall, this study demonstrates a simple yet effective approach to boost the electron mobility in organic transistors by synergistic use of pyridine and selenophene in the backbone of a DPP‐based copolymer. 相似文献
94.
Summary A theoretical study is presented for the stability characteristics of the laminar free convection boundary layer flow along a vertical porous (permeable) flat plate subjected to a constant heat flux. The disturbance equations are solved numerically on the basis of the linear stability theory for a wide range of values of the modified Grashof number,G, and some values of the suction or injection parameterX when the Prandtl number, Pr, is 0.73 (air). These solutions indicate the important role of the parametersG andX on the flow and heat transfer characteristics. It is found that the present results are in very good agreement with those from the open literature. 相似文献
95.
Guisheng Zhai Shohei Okuno Joe Imae Tomoaki Kobayashi 《Journal of Intelligent and Robotic Systems》2011,63(2):309-322
In this paper, we study a consensus problem for multi-agent systems via dynamic output feedback control. The entire system
is decentralized in the sense that each agent can only obtain output information from its neighbor agents. For practical purpose,
we assume that actuator limitation exists, and require that the consensus be achieved among the agents at a specified convergence
rate. By using an appropriate coordinate transformation, we reduce the consensus problem on hand to solving a strict matrix
inequality, and then propose to use the homotopy based method for solving the matrix inequality. It turns out that our algorithm
includes the existing graph Laplacian based algorithm as a special case. 相似文献
96.
We used the method of moments (MoM), which is a numerical electromagnetic field computation method, to study the surge characteristics of twisted pair single‐phase electric power lines. The results show that wires stranded with less than several turns per meter have almost the same surge characteristics as parallel lines, but the surge impedance decreases in tens of % when the number of strands increases. To verify the simulation results, we measured the surge characteristics of a model line of twisted pair experimentally, and there is good accordance between them. It is possible to simulate the surge in twisted pair covered with polymer dielectric insulators by MoM. Moreover, we studied the surge characteristics of twisted pair which is inserted into a metal tube. According to the results, the effect of the strand is smaller than that in free space without the metal pipe. There are two propagation modes in common mode: fast surge and slow surge. Few influences of the number of strands on the surge velocity occur in the fast propagation surge, but the increase of the surge impedance and the slowdown of the propagation speed are caused by twining in the slow propagation mode. © 2009 Wiley Periodicals, Inc. Electr Eng Jpn, 167(3): 1–9, 2009; Published online in Wiley InterScience ( www.interscience.wiley.com ). DOI 10.1002/eej.20737 相似文献
97.
98.
Encapsulation of lead-free Sn/Zn/Bi solder alloy particles by coating with wax powder for improving oxidation resistance 总被引:2,自引:0,他引:2
Tomohiro Iwasaki Jeong Hwan Kim Shohei Mizuhashi Munetake Satoh 《Journal of Electronic Materials》2005,34(5):647-654
An encapsulation treatment of lead-free Sn/Zn/Bi solder powder was investigated for improving the oxidation resistance. Sn-8mass%Zn-3mass%Bi
alloy particles were coated with a wax (12-hydroxystearic acid) powder by means of a dry mechanical treatment method using
a ball mill. In order to determine the optimum operating conditions of the ball mill in the wax-coating treatments, the compressive
energy required for deforming a single Sn/Zn/Bi alloy particle was measured with an unconfined compression tester and the
mechanical energy applied to the alloy particles in the ball mill was estimated using the results of the compression test.
The optimum operating conditions were determined based on both the applied energy and the flowability of solder pastes, and
the wax-coated alloy particles maintaining the spherical shape were obtained under the conditions. The wettability test and
the solder balling test for the solder pastes containing the wax-coated alloy particles stored at room temperature in air
were carried out to evaluate the oxidation resistance performance. The wax-coated alloy particles had an excellent wettability
compared with the original alloy particles, and the oxidation resistance of the Sn/Zn/Bi solder powder was improved by the
encapsulation treatment. 相似文献
99.
A new four-step thermochemical cycle based on calcium and iodine is proposed for the decomposition of water. The chemical reactions comprising the cycle are: the redox reaction of iodine with calcium hydroxide; the thermal decomposition of calcium iodate; the hydrolysis of calcium iodide; and the thermal decomposition of hydrogen iodide. Experimental verification of each of these reactions and an evaluation of the thermal efficiency of the process based on the material and energy balances for a proposed flow sheet are also presented. 相似文献
100.