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961.
5 nm Silver Nanoparticles Amplify Clinical Features of Atopic Dermatitis in Mice by Activating Mast Cells 下载免费PDF全文
HanGoo Kang Seungjae Kim Kwang Hoon Lee Shan Jin Seo Hyeong Kim Kangtaek Lee Hyungjoon Jeon Young‐Geon Song Sang‐Won Lee Jinwon Seo Soomin Park In‐Hong Choi 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(9)
The triggering effect of silver nanoparticles (NPs) on the induction of allergic reactions is evaluated, by studying the activation of mast cells and the clinical features of atopic dermatitis in a mouse model. Granule release is induced in RBL‐2H3 mast cells by 5 nm, but not 100 nm silver NPs. Increases in the levels of reactive oxygen species (hydrogen peroxide and mitochondrial superoxide) and intracellular Ca++ in mast cells are induced by 5 nm silver NPs. In a mouse model of atopic dermatitis induced by a mite allergen, the skin lesions are more severe and appear earlier in mice treated simultaneously with 5 nm silver NPs and allergen compared with mice treated with allergen alone or 100 nm silver NPs and allergen. The histological findings reveal that number of tryptase‐positive mast cells and total IgE levels in the serum increase in mice treated with 5 nm silver NPs and allergen. The results in this study indicate that cotreatment with 5 nm silver NPs stimulates mast cell degranulation and induces earlier and more severe clinical alterations in allergy‐prone individuals. 相似文献
962.
963.
Rational Design and Synthesis of Extremely Efficient Macroporous CoSe2–CNT Composite Microspheres for Hydrogen Evolution Reaction 下载免费PDF全文
Jin Koo Kim Gi Dae Park Jung Hyun Kim Seung‐Keun Park Yun Chan Kang 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(27)
Uniquely structured CoSe2–carbon nanotube (CNT) composite microspheres with optimized morphology for the hydrogen‐evolution reaction (HER) are prepared by spray pyrolysis and subsequent selenization. The ultrafine CoSe2 nanocrystals uniformly decorate the entire macroporous CNT backbone in CoSe2–CNT composite microspheres. The macroporous CNT backbone strongly improves the electrocatalytic activity of CoSe2 by improving the electrical conductivity and minimizing the growth of CoSe2 nanocrystals during the synthesis process. In addition, the macroporous structure resulting from the CNT backbone improves the electrocatalytic activity of the CoSe2–CNT microspheres by increasing the removal rate of generated H2 and minimizing the polarization of the electrode during HER. The CoSe2–CNT composite microspheres demonstrate excellent catalytic activity for HER in an acidic medium (10 mA cm?2 at an overpotential of ≈174 mV). The bare CoSe2 powders exhibit moderate HER activity, with an overpotential of 226 mV at 10 mA cm?2. The Tafel slopes for the CoSe2–CNT composite and bare CoSe2 powders are 37.8 and 58.9 mV dec?1, respectively. The CoSe2–CNT composite microspheres have a slightly larger Tafel slope than that of commercial carbon‐supported platinum nanoparticles, which is 30.2 mV dec–1. 相似文献
964.
A Novel and Facile Route to Synthesize Atomic‐Layered MoS2 Film for Large‐Area Electronics 下载免费PDF全文
Stephen Boandoh Soo Ho Choi Ji‐Hoon Park So Young Park Seungho Bang Mun Seok Jeong Joo Song Lee Hyeong Jin Kim Woochul Yang Jae‐Young Choi Soo Min Kim Ki Kang Kim 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(39)
High‐quality and large‐area molybdenum disulfide (MoS2) thin film is highly desirable for applications in large‐area electronics. However, there remains a challenge in attaining MoS2 film of reasonable crystallinity due to the absence of appropriate choice and control of precursors, as well as choice of suitable growth substrates. Herein, a novel and facile route is reported for synthesizing few‐layered MoS2 film with new precursors via chemical vapor deposition. Prior to growth, an aqueous solution of sodium molybdate as the molybdenum precursor is spun onto the growth substrate and dimethyl disulfide as the liquid sulfur precursor is supplied with a bubbling system during growth. To supplement the limiting effect of Mo (sodium molybdate), a supplementary Mo is supplied by dissolving molybdenum hexacarbonyl (Mo(CO)6) in the liquid sulfur precursor delivered by the bubbler. By precisely controlling the amounts of precursors and hydrogen flow, full coverage of MoS2 film is readily achievable in 20 min. Large‐area MoS2 field effect transistors (FETs) fabricated with a conventional photolithography have a carrier mobility as high as 18.9 cm2 V?1 s?1, which is the highest reported for bottom‐gated MoS2‐FETs fabricated via photolithography with an on/off ratio of ≈105 at room temperature. 相似文献
965.
Photonic Reactions Leading to Fluorescence in a Polymeric System Induced by the Photothermal Effect of Magnetite Nanoparticles Using a 780 nm Multiphoton Laser 下载免费PDF全文
Bum Chul Park Hee‐Dae Kim June Park Yu Jin Kim Young Keun Kim 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(37)
Recently, polymer‐coated magnetite (Fe3O4) nanoparticles (NPs) are extensively studied for applications in therapeutics or diagnostics using photothermal effect. Therefore, it is essential to understand the interactions between Fe3O4 NPs and polymers when optical stimuli are applied. Herein, the photonic reactions of Fe3O4 NPs and polymer composites upon application of a 780 nm multiphoton laser are analyzed. The photonic reactions produce unique results including fluorescence from conformationally changed polymer and low‐temperature phase transformation of Fe3O4 NPs. Typically, π‐conjugated chains are formed, inducing fluorescence through a series of main and side‐chain cleavage reactions of polymers with the aliphatic chain. In addition, fluorescence is detected in the cellular system by photonic reactions between Fe3O4 NPs and biomolecules. After multiphoton laser irradiation, light emission is detected near the intracellular Fe3O4 NPs, and a stronger intensity is observed in large‐sized NPs. 相似文献
966.
Designing Metallic and Insulating Nanocrystal Heterostructures to Fabricate Highly Sensitive and Solution Processed Strain Gauges for Wearable Sensors 下载免费PDF全文
Woo Seok Lee Seung‐Wook Lee Hyungmok Joh Mingi Seong Haneun Kim Min Su Kang Ki‐Hyun Cho Yun‐Mo Sung Soong Ju Oh 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(47)
All‐solution processed, high‐performance wearable strain sensors are demonstrated using heterostructure nanocrystal (NC) solids. By incorporating insulating artificial atoms of CdSe quantum dot NCs into metallic artificial atoms of Au NC thin film matrix, metal–insulator heterostructures are designed. This hybrid structure results in a shift close to the percolation threshold, modifying the charge transport mechanism and enhancing sensitivity in accordance with the site percolation theory. The number of electrical pathways is also manipulated by creating nanocracks to further increase its sensitivity, inspired from the bond percolation theory. The combination of the two strategies achieves gauge factor up to 5045, the highest sensitivity recorded among NC‐based strain gauges. These strain sensors show high reliability, durability, frequency stability, and negligible hysteresis. The fundamental charge transport behavior of these NC solids is investigated and the combined site and bond percolation theory is developed to illuminate the origin of their enhanced sensitivity. Finally, all NC‐based and solution‐processed strain gauge sensor arrays are fabricated, which effectively measure the motion of each finger joint, the pulse of heart rate, and the movement of vocal cords of human. This work provides a pathway for designing low‐cost and high‐performance electronic skin or wearable devices. 相似文献
967.
Solar Cells: Multidimensional Anodized Titanium Foam Photoelectrode for Efficient Utilization of Photons in Mesoscopic Solar Cells (Small 34/2017) 下载免费PDF全文
968.
Carbon Nanodot‐Sensitized Modulation of Alzheimer's β‐Amyloid Self‐Assembly,Disassembly, and Toxicity 下载免费PDF全文
You Jung Chung Kayoung Kim Byung Il Lee Chan Beum Park 《Small (Weinheim an der Bergstrasse, Germany)》2017,13(34)
The self‐assembly of amyloidogenic peptides into β‐sheet‐rich aggregates is a general feature of many neurodegenerative diseases, including Alzheimer's disease, which signifies the need for the effective attenuation of amyloid aggregation toward alleviating amyloid‐associated neurotoxicity. This study reports that photoluminescent carbon nanodots (CDs) can effectively suppress Alzheimer's β‐amyloid (Aβ) self‐assembly and function as a β‐sheet breaker disintegrating preformed Aβ aggregates. This study synthesizes CDs using ammonium citrate through one‐pot hydrothermal treatment and passivates their surface with branched polyethylenimine (bPEI). The bPEI‐coated CDs (bPEI@CDs) exhibit hydrophilic and cationic surface characteristics, which interact with the negatively charged residues of Aβ peptides, suppressing the aggregation of Aβ peptides. Under light illumination, bPEI@CDs display a more pronounced effect on Aβ aggregation and on the dissociation of β‐sheet‐rich assemblies through the generation of reactive oxygen species from photoactivated bPEI@CDs. The light‐triggered attenuation effect of Aβ aggregation using a series of experiments, including photochemical and microscopic analysis, is verified. Furthermore, the cell viability test confirms the ability of photoactivated bPEI@CDs for the suppression of Aβ‐mediated cytotoxicity, indicating bPEI@CDs' potency as an effective anti‐Aβ neurotoxin agent. 相似文献
969.
DNA Imaging: DNA Binding Peptide Directed Synthesis of Continuous DNA Nanowires for Analysis of Large DNA Molecules by Scanning Electron Microscope (Small 2/2017) 下载免费PDF全文
970.
Biomolecular regulatory networks are organised around hubs, which can interact with a large number of targets. These targets compete with each other for access to their common hubs, but whether the effect of this competition would be significant in magnitude and in function is not clear. In this review, the authors discuss recent in vivo studies that analysed the system level retroactive effects induced by target competition in microRNA and mitogen‐activated protein kinase regulatory networks. The results of these studies suggest that downstream targets can regulate the overall state of their upstream regulators, and thus cannot be ignored in analysing biomolecular networks.Inspec keywords: reviews, RNA, molecular biophysics, enzymesOther keywords: target‐mediated reverse signalling, mitogen‐activated protein kinase regulatory networks, biomolecular regulatory networks, microRNA regulatory networks, review, in vivo study 相似文献