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101.
102.
Yiqian Du Zhikai Yan Wenbin You Qiaoqiao Men Guanyu Chen Xiaowei Lv Yuyang Wu Kaicheng Luo Biao Zhao Jincang Zhang Renchao Che 《Advanced functional materials》2023,33(34):2301449
Surface chemistry and interlayer engineering determines the electrical properties of 2D MXene. However, it remains challenging to regulate the surface and interfacial chemistry of MXene simultaneously. Herein, simultaneous modulation of Ti3C2Tx MXene surface termination and layer spacing by alkali treatment are achieved. The electrical and electromagnetic properties of Ti3C2Tx are investigated in detail with respect to KOH and ammonia concentration dependence. A high concentration of KOH caused the Ti3C2Tx layer spacing to expand to 13.7 Å and the surface O/F ratio to increase to 33.84. Because of its weaker ionization effect, ammonia provides finer tuning compared to the drastic intercalation of KOH with a thorough sweeping of the F-containing groups. Ti3C2Tx is enriched with conductive -OH termination after ammonia treatment, which achieves an effective balance with the increased interlayer resistance. Therefore, NH3H2O-Ti3C2Tx achieves broad-band impedance matching and exhibits an efficient microwave loss of −49.1 dB at a low thickness of 1.7 mm, with an effective frequency bandwidth of 3.9 GHz. The results herein optimize the electrical properties of Ti3C2Tx using surface and interfacial chemistry to achieve broad microwave absorption, providing a framework for enhancing the electromagnetic wave loss of intrinsic MXene. 相似文献
103.
Haitao Hu Dan Li Wenbin Dai Qiao Jin Dong Wang Jian Ji Ben Zhong Tang Zhe Tang 《Advanced functional materials》2023,33(19):2213134
Compared to conventional photothermal therapy (PTT) which requires hyperthermia higher than 50 °C, mild-temperature PTT is a more promising antitumor strategy with much lower phototoxicity to neighboring normal tissues. However, the therapeutic efficacy of mild-temperature PTT is always restricted by the thermoresistance of cancer cells. To address this issue, a supramolecular drug nanocarrier is fabricated to co-deliver nitric oxide (NO) and photothermal agent DCTBT with NIR-II aggregation-induced emission (AIE) characteristic for mild-temperature PTT. NO can be effectively released from the nanocarriers in intracellular reductive environment and DCTBT is capable of simultaneously producing reactive oxygen species (ROS) and hyperthermia upon 808 nm laser irradiation. The generated ROS can further react with NO to produce peroxynitrite (ONOOˉ) bearing strong oxidization and nitration capability. ONOOˉ can inhibit the expression of heat shock proteins (HSP) to reduce the thermoresistance of cancer cells, which is necessary to achieve excellent therapeutic efficacy of DCTBT-based PTT at mild temperature (<50 °C). The antitumor performance of ONOOˉ-potentiated mild-temperature PTT is validated on subcutaneous and orthotopic hepatocellular carcinoma (HCC) models. This research puts forward an innovative strategy to overcome thermoresistance for mild-temperature PTT, which provides new inspirations to explore ONOOˉ-sensitized tumor therapy strategies. 相似文献
104.
Kong Chao Ou Weihua Gong Xiaofeng Li Weian Han Jie Yao Yi Xiong Jiahao 《中国邮电高校学报(英文版)》2022,29(6):73-82
Face anti-spoofing is used to assist face recognition system to judge whether the detected face is real face or fake face. In the traditional face anti-spoofing methods, features extracted by hand are used to describe the difference between living face and fraudulent face. But these handmade features do not apply to different variations in an unconstrained environment. The convolutional neural network (CNN) for face deceptions achieves considerable results. However, most existing neural network-based methods simply use neural networks to extract single-scale features from single-modal data, while ignoring multi-scale and multi-modal information. To address this problem, a novel face anti-spoofing method based on multi-modal and multi-scale features fusion ( MMFF) is proposed. Specifically, first residual network ( Resnet )-34 is adopted to extract features of different scales from each modality, then these features of different scales are fused by feature pyramid network (FPN), finally squeeze-and-excitation fusion ( SEF) module and self-attention network ( SAN) are combined to fuse features from different modalities for classification. Experiments on the CASIA-SURF dataset show that the new method based on MMFF achieves better performance compared with most existing methods. 相似文献
105.
传统频谱扩展与压缩(SSC)盲移频干扰的阶数为整数,为了实现精确的位置干扰,需要调整不同的处理延时,在实际应用中存在一定的局限性.该文对整数阶盲移频技术进行了改进,提出了一种基于非整数阶SSC盲移频的LFM雷达干扰技术.该技术在干扰机处理延时不变的情况下,通过改变SSC盲移频的阶数来实现精确的位置干扰.该文推导了一种高效的非整数阶SSC盲移频干扰实现方法,同时通过Newman序列控制信号的初相来减小压制干扰信号的峰均比(PAPR).仿真结果表明,该文算法在指定干扰机处理延时的情况下,可以实现假目标欺骗干扰和相参密集压制干扰,能够有效对抗脉冲压缩体制雷达,具有较好的工程应用价值. 相似文献
106.
以氧化石墨烯(GO)为原料,尿素为氮掺杂剂,采用固/气界面水热反应的方式,即在反应釜内将GO抽滤得到的氧化石墨烯纸(GOP)与尿素分解产生的氨蒸气相互作用,成功制备出自支撑氮掺杂石墨烯纸(NGP)。通过X射线衍射(XRD)、扫描电子显微镜(SEM)、拉曼光谱(RS)、X射线光电子能谱(XPS)和电化学测试对样品进行形貌结构及电化学性能的表征。测试结果表明:水热条件下尿素能有效地实现氧化石墨烯纸的氮掺杂,氮掺杂量为7.89%;氮掺杂石墨烯纸在100mA/g和500mA/g的电流密度下,充放电循环100周之后,放电比容量可分别保持在288mAh/g和190mAh/g。采用改进的固/气界面水热反应法制备的氮掺杂石墨烯纸较未掺杂石墨烯纸可逆比容量提高了近2.5倍,具有良好的循环稳定性,可为制备高性能的柔性锂离子电池负极材料提供新方法。 相似文献
107.
108.
Boolean networks are widely used to model gene regulatory networks and to design therapeutic intervention strategies to affect the long‐term behavior of systems. Here, the authors investigate the 1 bit perturbation, which falls under the category of structural intervention. The authors’ idea is that, if and only if a perturbed state evolves from a desirable attractor to an undesirable attractor or from an undesirable attractor to a desirable attractor, then the size of basin of attractor of a desirable attractor may decrease or increase. In this case, if the authors obtain the net BOS of the perturbed states, they can quickly obtain the optimal 1 bit perturbation by finding the maximum value of perturbation gain. Results from both synthetic and real biological networks show that the proposed algorithm is not only simpler and but also performs better than the previous basin‐of‐states (BOS)‐based algorithm by Hu et al..Inspec keywords: perturbation theory, genetics, Boolean functionsOther keywords: optimal perturbation, perturbed states, Boolean network, gene regulatory networks, basin‐of‐states‐based algorithm, state‐transition diagram, structural intervention, perturbation gain, synthetic biological networks, real biological networks, 1 bit perturbation 相似文献
109.
Qi Jia Xin Ou Manuel Langer Benjamin Schreiber Jörg Grenzer Pablo F. Siles Raul D. Rodriguez Kai Huang Ye Yuan Alireza Heidarian René Hübner Tiangui You Wenjie Yu Kilian Lenz Jürgen Lindner Xi Wang Stefan Facsko 《Nano Research》2018,11(7):3519-3528
A nanofabrication method for the production of ultra-dense planar metallic nanowire arrays scalable to wafer-size is presented. The method is based on an efficient template deposition process to grow diverse metallic nanowire arrays with extreme regularity in only two steps. First, III–V semiconductor substrates are irradiated by a low-energy ion beam at an elevated temperature, forming a highly ordered nanogroove pattern by a “reverse epitaxy” process due to self-assembly of surface vacancies. Second, diverse metallic nanowire arrays (Au, Fe, Ni, Co, FeAl alloy) are fabricated on these III–V templates by deposition at a glancing incidence angle. This method allows for the fabrication of metallic nanowire arrays with periodicities down to 45 nm scaled up to wafer-size fabrication. As typical noble and magnetic metals, the Au and Fe nanowire arrays produced here exhibited large anisotropic optical and magnetic properties, respectively. The excitation of localized surface plasmon resonances (LSPRs) of the Au nanowire arrays resulted in a high electric field enhancement, which was used to detect phthalocyanine (CoPc) in surface-enhanced Raman scattering (SERS). Furthermore, the Fe nanowire arrays showed a very high in-plane magnetic anisotropy of approximately 412 mT, which may be the largest in-plane magnetic anisotropy field yet reported that is solely induced via shape anisotropy within the plane of a thin film. 相似文献
110.
L Tonella BJ Walsh JC Sanchez K Ou MR Wilkins M Tyler S Frutiger AA Gooley I Pescaru RD Appel JX Yan A Bairoch C Hoogland FS Morch GJ Hughes KL Williams DF Hochstrasser 《Canadian Metallurgical Quarterly》1998,19(11):1960-1971
The combination of two-dimensional polyacrylamide gel electrophoresis (2-D PAGE), computer image analysis and several protein identification techniques allowed the Escherichia coli SWISS-2DPAGE database to be established. This is part of the ExPASy molecular biology server accessible through the WWW at the URL address http://www.expasy.ch/ch2d/ch2d-top.html . Here we report recent progress in the development of the E. coli SWISS-2DPAGE database. Proteins were separated with immobilized pH gradients in the first dimension and sodium dodecyl sulfate-polyacrylamide gel electrophoresis in the second dimension. To increase the resolution of the separation and thus the number of identified proteins, a variety of wide and narrow range immobilized pH gradients were used in the first dimension. Micropreparative gels were electroblotted onto polyvinylidene difluoride membranes and spots were visualized by amido black staining. Protein identification techniques such as amino acid composition analysis, gel comparison and microsequencing were used, as well as a recently described Edman "sequence tag" approach. Some of the above identification techniques were coupled with database searching tools. Currently 231 polypeptides are identified on the E. coli SWISS-2DPAGE map: 64 have been identified by N-terminal microsequencing, 39 by amino acid composition, and 82 by sequence tag. Of 153 proteins putatively identified by gel comparison, 65 have been confirmed. Many proteins have been identified using more than one technique. Faster progress in the E. coli proteome project will now be possible with advances in biochemical methodology and with the completion of the entire E. coli genome. 相似文献