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31.
Isabella S. Romero Nathan P. Bradshaw Jesse D. Larson Sean Y. Severt Sandra J. Roberts Morgan L. Schiller Janelle M. Leger Amanda R. Murphy 《Advanced functional materials》2014,24(25):3866-3873
Single‐component, metal‐free, biocompatible, electromechanical actuator devices are fabricated using a composite material composed of silk fibroin and poly(pyrrole) (PPy). Chemical modification techniques are developed to produce free‐standing films with a bilayer‐type structure, with unmodified silk on one side and an interpenetrating network (IPN) of silk and PPy on the other. The IPN formed between the silk and PPy prohibits delamination, resulting in a durable and fully biocompatible device. The electrochemical stability of these materials is investigated through cyclic voltammetry, and redox sensitivity to the presence of different anions is noted. Free‐end bending actuation performance and force generation within silk‐PPy composite films during oxidation and reduction in a biologically relevant environment are investigated in detail. These silk–PPy composites are stable to repeated actuation, and are able to generate forces comparable with natural muscle (>0.1 MPa), making them ideal candidates for interfacing with biological tissues. 相似文献
32.
Rafael Schmitt Markus Kubicek Eva Sediva Morgan Trassin Mads C. Weber Antonella Rossi Herbert Hutter Jens Kreisel Manfred Fiebig Jennifer L. M. Rupp 《Advanced functional materials》2019,29(5)
Memristive devices based on mixed ionic–electronic resistive switches have an enormous potential to replace today's transistor‐based memories and Von Neumann computing architectures thanks to their ability for nonvolatile information storage and neuromorphic computing. It still remains unclear however how ionic carriers are propagated in amorphous oxide films at high local electric fields. By using memristive model devices based on LaFeO3 with either amorphous or epitaxial nanostructures, we engineer the structural local bonding units and increase the oxygen‐ionic diffusion coefficient by one order of magnitude for the amorphous oxide, affecting the resistive switching operation. We show that only devices based on amorphous LaFeO3 films reveal memristive behavior due to their increased oxygen vacancy concentration. We achieved stable resistive switching with switching times down to microseconds and confirm that it is predominantly the oxygen‐ionic diffusion character and not electronic defect state changes that modulate the resistive switching device response. Ultimately, these results show that the local arrangement of structural bonding units in amorphous perovskite films at room temperature can be used to largely tune the oxygen vacancy (defect) kinetics for resistive switches (memristors) that are both theoretically challenging to predict and promising for future memory and neuromorphic computing applications. 相似文献
33.
Existence conditions are given for maximum likelihood (ML) parameter estimates for several families of 2-parameter software-reliability Poisson-process models. For each such model, the ML equations can be expressed in terms of one equation in one unknown. Bounds are given on solutions to these one equation problems to serve as initial intervals for search algorithms like bisection. Uniqueness of the solutions is established in some cases. Solutions are also tabulated for certain simple cases. Results are given for ungrouped failure data (exact times are available for all failures). ML estimation problems for such a situation are treated as limiting cases of problems based on failure times grouped into intervals of decreasing mesh 相似文献
34.
Juliet A Kauffman E N Clare Mills Gary M Brett Roger J Fido Arthur S Tatham Peter R Shewry Akiko Onishi Michael O Proudlove Michael R A Morgan 《Journal of the science of food and agriculture》1994,66(3):345-355
Eight monoclonal antibodies (mAb) recognising barley polypeptides have been identified from a library developed to wheat prolamins. The specificity or the mAb has been determined using enzyme-linked immunosorbent assay (ELISA) and immunoblotting. Six were of broad specificity, recognising D, B, C and γ-hordeins to varying degrees by both techniques. IFRN 0610 preferentially recognised γ-hordeins by ELISA but was highly specific for this hordein group by immunoblotting. Another mAb, IFRN 0624, bound to a Mr ∽ 18000 polypeptide belonging to the CM protein (trypsin/α-amylase inhibitor) family by immunoblotting. This, or a related protein, was detected by 0624 in all hordein fractions using ELISA. These mAb, together with two others described previously and found to recognise the repeat motif of C hordein, were used in ELISA and immunoblot analysis of Octyl-Sepharose fractions of lager foam. Hordein polypeptides were found in all foam fractions, indicating that much foam protein originates from the malt. The CM-like protein was found present in a virtually unmodified form. In contrast, the repeat motif of C hordein was not detected, indicating that it had either been destroyed or masked by other beer constituents. The foam stabilising agent, propylene glycol alginate (PGA), increased the apparent hydrophobicity of hordein fragments suggesting that at least part of the activity of PGA is mediated by interactions with the hordein components of foam. 相似文献
35.
Kraft paper is used extensively in the electricity supply industry for the insulation of HV apparatus, such as transformers, capacitors and cables. Because of the fibrous nature of the paper, many layers are stacked or rolled to obtain the required electric strength. The insulation is thus a combination of cellulose and an impregnating fluid, which may be a liquid, a gas or vacuum. The dielectric properties of such a system depend on the dryness, temperature, frequency and the degree of mechanical compression. Although the effects of moisture, temperature and frequency on the dielectric properties of kraft paper have been studied, very little work has been done on the effect of compressive stress, particularly long-term effects. Results are presented of measurements, in the frequency range 50 Hz to 20 kHz, of the effects of compressive stress and temperature on the real and imaginary parts of the complex relative permittivity of a multilayer stack of dry kraft paper under vacuum. The variations of the dc resistance with compressive stress and temperature also are reported. Results are given of the variation of the dielectric properties of a stack of paper following a step change in either the temperature or the air pressure. The long-term variations are attributed to the slow diffusion of ions through the stack, particularly those held at the interfaces between layers 相似文献
36.
T. N. Morgan 《Journal of Electronic Materials》1991,20(1):63-70
I describe the vacancy-interstitial model ofDX centers, in which the substitutional donor atoms relax toward interstitial sites when they capture electrons. This appears
to be the only known model ofDX centers which can account for the structure observed by Mooneyet al. in DLTS spectra of dilute Al
x
Ga1-x
As alloys. By comparing its predictions with the DLTS and Hall data from Al
x
Ga1-x
As alloys of low Al content one can establish values for many of the relevant parameters, such as the enthalpies and entropies
(degeneracies) associated with sites surrounded by differing numbers of Al atoms. The data also show that the distribution
of donor configurations among the four available neighboring interstitial sites does not attain thermal equilibrium among
states of differing energies before being released, although transitions (through tunneling) among states of equal energy
may be possible. The model is seen to be consistent with those treated theoretically by Chadi and Chang forDX and by Dabrowski and Scheffler for EL2 centers. 相似文献
37.
J. Chambers C. P. Morgan P. R. White K. Mori D. E. Finnegan D. B. Pinniger 《Journal of chemical ecology》1990,16(12):3353-3372
Antennal and behavioral responses of the rust-red grain beetle,Cryptolestes ferrugineus, and the flat grain beetle,C. pusillus, to synthetic samples of the macrocyclic lactones reported to comprise their aggregation pheromones were investigated. Electroantennogram (EAG) recordings were obtained successfully from both species for the first time. Females of both species showed larger EAGs than males. The EAGs ofC. ferrugineus showed a high degree of specificity for conspecific aggregation pheromone components;C. pusillus showed much less specificity. Behavioral tests were conducted using two-choice pitfall bioassays. Separation of the results into the two effects of activity stimulation and direction finding showed that both effects contributed to the overall response, although sometimes to different extents. The strain ofC. pusillus studied responded equally well to both components of its pheromone, whereas it had been reported previously that only one was active, the other acting as a Synergist and eliciting no response when tested alone. With both species, behavioral response was elicited with a single lactone, suggesting that it might not be necessary to use both components for field use. Particularly surprising was thatC. pusillus showed a greater response to the pheromone components ofC. ferrugineus than to its own. Aeration of the two species and thermal desorption of the collected volatiles confirmed production of the expected lactones, and aeration of authentic lactones showed that the response was not due to the C.ferrugineus pheromone components being markedly more volatile. This response, which seems to be an actual preference, is the first to be discovered among the cucujid beetles and encourages optimism that a practical lure for various species may not need to be as complex as originally feared. 相似文献
38.
Tyler R. Harrison Susan E. Morgan Lisa V. Chewning Elizabeth A. Williams Joshua B. Barbour Mark J. Di Corcia LaShara A. Davis 《The Journal of communication》2011,61(3):535-555
This article advances the beginnings of a general theory of organizational features to aid in understanding why health campaigns that work well in one organization may be ineffectual in another organization. The physical, social, and information structures of organizations are theorized to create an interaction environment that is distinct to each organization and that influences health campaigns. To test this argument, an organ donation campaign was conducted in 46 organizations. Multilevel modeling yielded mixed findings. Physical structure was negatively associated with signing an organ donor card. Social structure and information structure were positively associated with communication with coworkers about donation and communicative peer influence. Industry type was positively associated with knowledge change. 相似文献
39.
K. Autio L. Mannonen K. Pietil M. Koskinen M. Suka-aho M. Linko A. Morgan 《Journal of the Institute of Brewing》1996,102(6):427-432
The effects of purified Trichoderma reesei endo-xylanase, XYN II and endoglucanases, EG I and EG II on the cell walls of embedded barley cross sections were studied. The cell walls were stained with Calcofluor which is specific for (1–3)(1–4)-β-D-glucans (mixed-linked β-glucans) in histochemical applications. Whereas endosperm cell walls remained highly fluorescent after incubation with buffer, the aleurone cell walls were only weakly fluorescent. Both EG I and EG II were effective in degrading the outer endosperm cell walls, but had little or no effect on the inner endosperm and aleurone cell walls. Corresponding sections incubated with XYN II showed highly intensive fluorescence of aleurone cell walls suggesting that the surface of alaurone cell walls contains a high level of xylan which is removed by xylanase treatment exposing a layer rich in mixed linked β-glucans. This indicates that arabinoxylans and β-glucans in the aleurone cell walls of barley exist as separate, macroscopic layers. Xylanase did not have any Influence on the microstructure of endosperm cell walls which are rich in mixed linked β-glucans. However, incubation with EG II after xylanase treatment caused the aleurone cell walls to become very thin. 相似文献
40.
This paper continues the study of variation between varieties in some properties of barley and malt and examines protein-related characters and moisture uptake. Initial rate of moisture uptake was more closely related to enzyme activities than maximum moisture content. Significant varietal variation was found in all characters and this variation was greater than environmental variation with the exception of grain nitrogen concentration. In the endosperm endopeptidase activity was the character most highly correlated with malt hot water extract (HWE). The combined influence of protein- and β-glucan-related characters was investigated and the relative influence of each group of characters on HWE varied in different sections of the grain. In the endosperm the protein- and β-glucan-related characters accounted for 30% and 60% of the variation in HWE respectively. 相似文献