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71.
72.
Marine Harguindeguy Claire Antonelli Marie-Pierre Belleville José Sanchez-Marcano Céline Pochat-Bohatier 《应用聚合物科学杂志》2021,138(2):49669
Millimeter-size beads of gelatin are manufactured by dripping process to give enzyme supports qualified for micropollutants biodegradation in alternative wastewater treatment. The bead diameter is dependent on the tip diameter, the gelatin solution viscosity and the swelling of polymer chains in the collecting bath. Chemical crosslinking was performed with glutaraldehyde using optimal concentration to give mechanical and thermal properties suitable for application in stirred reactor in aqueous medium. Laccases from Trametes versicolor are grafted on the gelatin beads with glutaraldehyde. Sixty percentage of the initial enzymatic activity, evaluated by the oxidation of 2′-Azino-bis(3-ethylbenzothiazoline-6-sulfonic acid)diammonium salt (ABTS) is maintained after 10 successive cycles of reaction. Thermal stability at 60°C of immobilized biocatalysts is improved when compared to free enzymes (45% vs 10% of relative activity after 6 h of incubation). The simplicity of the procedure to form gelatin beads and their properties make them promising bio-based and biodegradable support for enzyme immobilization. 相似文献
73.
Luciana Gampert Miranda Carolina Pereira Peglow Victória Cardoso Deorristt Geórgia Campos Sales Neto Ariela Milbrath Cardoso Suzana Frighetto Ferrarini Marçal José Rodrigues Pires 《应用聚合物科学杂志》2021,138(7):49842
The use of polymeric films incorporated with zeolite-TiO2 composites associated with UV radiation can be an alternative in the removal of volatile organic compounds (VOCs) through the adsorption and photodegradation processes. This study produced poly(lactic acid) (PLA) films incorporated with 13× zeolite, TiO2, and 13×-TiO2 zeolite composite to remove n-butanol and evaluate the by-products generated in the process. The results showed that 13× zeolite and TiO2 added individually or as a composite to PLA, gave the polymer matrix a significant increase in the removal capacity of n-butanol. The best performance was presented by the zeolite-TiO2, composite, confirming a synergistic effect. However, the formation of CO and CO2 exceeded the expected values, with the verification that the polymeric matrix underwent photodegradation action by TiO2. The polymeric film only containing zeolite is the most suitable for the removal of VOCs, as it did not present degradation of the PLA, generating a lower concentration of by-products. 相似文献
74.
Alejandro Ávila-Ortega José Pablo Avalos-Hernández Rudy Trejo-Tzab Andrés Iván Oliva Juan Antonio Juárez-Moreno 《应用聚合物科学杂志》2021,138(30):50737
Among several oil/water emulsion separation technologies, the utilization of nanoparticle-decorated membranes with diverse functionalities has received considerable attention in recent years, particularly if the antifouling capacity can be improved. In this article, we propose a new membrane based on surface-hydrolyzed polyacrylonitrile electrospun membranes and/or decorated with amine-functionalized Si-MCM-41 nanoparticles to be used as oil/water emulsion separation treatment and to determine their antifouling ability. X-Ray photoelectron spectrometry, attenuated total reflectance Fourier transform infrared spectroscopy, and toluidine blue O assay, scanning electron microscopy, contact angle measurements for oil under water and thermogravimetry were used for characterizing the membranes and an assay of permeability was developed to quantify the diffusion of oil molecules across the electrospun membrane. The electrospun and/or decorated membranes showed an underwater oleophobic wettability, which can separate oil-in-water emulsions with 87% separation efficiency, results of fouling experiments, evaluated in terms of rejection and flux recovery ratio, exhibited good antifouling ability, but the membrane decoration process did not lead to superior outcomes compared with undecorated membranes. 相似文献
75.
BRINKSMEIER Ekkard WALTER André NOWAG Lutz S 《金属热处理》2004,29(8):66-72
通过旋转试验和有限元分析介绍了工件在切削加工过程中产生的畸变情况,分析了工件的装夹方式、切削速度、切削深度和进刀量对100Cr6钢环圆度的影响。通过去应力退火释放冷加工诱发的残余应力后工件的圆度与切削参数有关。另外测试了被试验环的表面残余应力,其表面残余应力与装夹方式有关。将测量的装夹力作为计算参数输入,通过有限元分析方法测试了装夹方式对工件变形的影响。协同测量结果示出了装夹方式影响工件变形的一个主要因素,表面残余应力与工件的径向变形有关,最大的拉伸应力位于夹口位置。旋转切削试验结果表明,提高切削速度圆度会稍有增加;随着切削深度的加大,圆度呈下降趋势,尽管切削力增加了;进给量的增加会导致更高的切削力,因此圆度值也增加;常规的去应力退火可使被加工环的圆度值增加。 相似文献
76.
A model for atmospheric pollutant transport is proposed considering an advection–diffusion–reaction equation. A splitting method is used to decouple the advection, diffusion and reaction parts. A scheme based on finite volume, finite difference and backward differentiation formula is used for solving an atmospheric transport-chemistry problem. 相似文献
77.
Lourenço André Rota Bulò Samuel Rebagliati Nicola Fred Ana L. N. Figueiredo Mário A. T. Pelillo Marcello 《Machine Learning》2015,98(1-2):331-357
Machine Learning - Clustering ensemble methods produce a consensus partition of a set of data points by combining the results of a collection of base clustering algorithms. In the evidence... 相似文献
78.
79.
Bit commitment schemes are at the basis of modern cryptography. Since information-theoretic security is impossible both in the classical and in the quantum regime, we examine computationally secure commitment schemes. In this paper we study worst-case complexity assumptions that imply quantum bit commitment schemes. First, we show that QSZK \({\not\subseteq}\) QMA implies a computationally hiding and statistically binding auxiliary-input quantum commitment scheme. We then extend our result to show that the much weaker assumption QIP \({\not\subseteq}\) QMA (which is weaker than PSPACE \({\not\subseteq}\) PP) implies the existence of auxiliary-input commitment schemes with quantum advice. Finally, to strengthen the plausibility of the separation QSZK \({\not\subseteq}\) QMA, we find a quantum oracle relative to which honest-verifier QSZK is not contained in QCMA, the class of languages that can be verified using a classical proof in quantum polynomial time. 相似文献
80.
André J. Torii Rafael H. Lopez Leandro F. F. Miguel 《Structural and Multidisciplinary Optimization》2016,54(2):289-299
Truss optimization based on the ground structure approach often leads to designs that are too complex for practical purposes. In this paper we present an approach for design complexity control in truss optimization. The approach is based on design complexity measures related to the number of bars (similar to Asadpoure et al. Struct Multidisc Optim 51(2):385–396 2015) and a novel complexity measure related to the number of nodes of the structure. Both complexity measures are continuously differentiable and thus can be used together with gradient based optimization algorithms. The numerical examples show that the proposed approach is able to reduce design complexity, leading to solutions that are more fit for engineering practice. Besides, the examples also indicate that in some cases it is possible to significantly reduce design complexity with little impact on structural performance. Since the complexity measures are non convex, a global gradient based optimization algorithm is employed. Finally, a detailed comparison to a classical approach is presented. 相似文献